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The hydrogen atom is a system amenable to an exact treatment within Schroedinger's formulation of quantum mechanics according to coordinates in four systems -- spherical polar, paraboloidal, ellipsoidal and spheroconical coordinates; the…

General Physics · Physics 2017-07-20 J. F. Ogilvie

The calculation time for the energy of atoms and molecules scales exponentially with system size on a classical computer but polynomially using quantum algorithms. We demonstrate that such algorithms can be applied to problems of chemical…

Quantum Physics · Physics 2007-05-23 Alán Aspuru-Guzik , Anthony D. Dutoi , Peter J. Love , Martin Head-Gordon

We developed a deep generative model-based variational free energy approach to the equations of state of dense hydrogen. We employ a normalizing flow network to model the proton Boltzmann distribution and a fermionic neural network to model…

Strongly Correlated Electrons · Physics 2023-09-26 Hao Xie , Zi-Hang Li , Han Wang , Linfeng Zhang , Lei Wang

We derive the wave function for N-dimensional hydrogen atom in the momentum representation with the phase factor using the generating function method and Hankel's integral.

Mathematical Physics · Physics 2009-04-01 Mehdi Hage-Hassan

The hydrogen phase diagram has a number of unusual features which are generally well reproduced by density functional calculations. Unfortunately, these calculations fail to provide good physical insights into why those features occur. In…

Materials Science · Physics 2020-10-28 Hongxiang Zong , Heather Wiebe , Graeme J. Ackland

We consider general theoretical models of water and in particular the nature of the motions of the hydrogen nuclei. If the motion of hydrogen nuclei is classical, then the thermodynamic pressure equation of state for heavy water wherein the…

Other Condensed Matter · Physics 2015-12-11 A. Widom , J. Swain , S. Sivasubramanian , D. Drosdoff , Y. N. Srivastava

Strongly interacting quantum systems described by non-stoquastic Hamiltonians exhibit rich low-temperature physics. Yet, their study poses a formidable challenge, even for state-of-the-art numerical techniques. Here, we investigate…

Computational Physics · Physics 2021-06-18 Marin Bukov , Markus Schmitt , Maxime Dupont

The states of hydrogen atom with principal quantum number $n\le3$ and zero magnetic quantum number in constant homogeneous magnetic field ${\cal H}$ are considered. The coefficients of energy eigenvalues expansion up to 75th order in powers…

Atomic Physics · Physics 2015-08-06 V. A. Gani , A. E. Kudryavtsev , V. M. Weinberg

Quantum mechanics is considered to arise from an underlying classical structure (``hidden variable theory'', ``sub-quantum mechanics''), where quantum fluctuations follow from a physical noise mechanism. The stability of the hydrogen ground…

Quantum Physics · Physics 2009-11-11 Th. M. Nieuwenhuizen

In this note, variational Monte Carlo method based on neural quantum states for spin systems is reviewed. Using a neural network as the wave function allows for a more generalized expression of various types of interactions, including…

Strongly Correlated Electrons · Physics 2024-06-04 Yuntai Song

A basis set of generalized nonspherical Gaussian functions (GGTOs) is presented and discussed. As a first example we report on Born-Oppenheimer energies of the hydrogen molecule. Although accurate results have been obtained, we conclude…

Chemical Physics · Physics 2009-10-31 T. Detmer , P. Schmelcher , L. S. Cederbaum

It is shown that all of the basic properties of the hydrogen atom can be consistently described in terms of classical electrodynamics instead of taking the electron to be a particle; we consider an electrically charged classical wave field,…

General Physics · Physics 2017-03-08 Sergey Rashkovskiy

Hydrogen has been the subject of intense research following the discovery of high-temperature superconductivity in hydrides, and as a result of continuous efforts to produce solid hydrogen. The Born-Oppenheimer approximation is the central…

Materials Science · Physics 2023-11-13 Ville J. Härkönen

We report on highly accurate calculations of Born-Oppenheimer potentials for excited $n\,\Sigma^{+}$ states of the hydrogen molecule for all possible combinations of singlet/triplet and gerade/ungerade symmetries up to $n=7$. A relative…

Atomic Physics · Physics 2023-02-28 Michał Siłkowski , Magdalena Zientkiewicz , Krzysztof Pachucki

The ground-state properties of spin polarized hydrogen H$\downarrow$ are obtained by means of diffusion Monte Carlo calculations. Using the most accurate to date ab initio H$\downarrow$-H$\downarrow$ interatomic potential we have studied…

Other Condensed Matter · Physics 2007-05-23 L. Vranjes Markic , J. Boronat , J. Casulleras

We consider a non-relativistic two-dimensional (2D) hydrogen-like atom in a weak, static, uniform magnetic field perpendicular to the atomic plane. Within the framework of the Rayleigh-Schr\"odinger perturbation theory, using the Sturmian…

Quantum Physics · Physics 2018-06-12 Radosław Szmytkowski

We present an accurate theoretical determination of rovibrational energy levels of the hydrogen molecule and its isotopologues in its electronic ground state. We consider all significant corrections to the Born-Oppenheimer approximation,…

We present an efficient quantum algorithm for beyond-Born-Oppenheimer molecular energy computations. Our approach combines the quantum full configuration interaction method with the nuclear orbital plus molecular orbital (NOMO) method. We…

Quantum Physics · Physics 2016-02-24 Libor Veis , Jakub Višňák , Hiroaki Nishizawa , Hiromi Nakai , Jiří Pittner

An interatomic potential for high-pressure high-temperature (HPHT) crystalline and liquid phases of sodium is created using a neural-network (NN) representation of the ab initio potential energy surface. It is demonstrated that the NN…

Materials Science · Physics 2015-05-18 Hagai Eshet , Rustam Z. Khaliullin , Thomas D. Kuhne , Jorg Behler , Michele Parrinello

We construct a system of coherent states for the hydrogen atom that is expressed in terms of elementary functions. Unlike to the previous attempts in this direction, this system possesses the properties equivalent to the most of those for…

Quantum Physics · Physics 2009-11-06 Semyon Pol'shin