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Quantum spin liquid (QSL) represents a new class of condensed matter states characterized by the long-range many-body entanglement of topological orders. The most prominent feature of the elusive QSL state is the existence of fractionalized…

The kagome Heisenberg antiferromagnet formed by frustrated spins arranged in a lattice of corner-sharing triangles is a prime candidate for hosting a quantum spin liquid (QSL) ground state consisting of entangled spin singlets. But the…

Strongly Correlated Electrons · Physics 2022-03-09 Jiaming Wang , Weishi Yuan , Philip M. Singer , Rebecca W. Smaha , Wei He , Jiajia Wen , Young S. Lee , Takashi Imai

Spin-$1/2$ kagome antiferromagnets are leading candidates for realizing quantum spin liquid (QSL) ground states. While QSL ground states are predicted for the pure Heisenberg model, understanding the robustness of the QSL to additional…

Strongly Correlated Electrons · Physics 2026-02-16 Shengtao Jiang , Arthur C. Campello , Wei He , Jiajia Wen , Daniel M. Pajerowski , Young S. Lee , Hong-Chen Jiang

Quantum spin liquids (QSLs) represent an exotic quantum many-body state characterized by the suppression of long-range magnetic order due to strong quantum fluctuations. The kagome spin-1/2 antiferromagnet (AFM) is a prime candidate for…

Strongly Correlated Electrons · Physics 2024-07-24 S. Suetsugu , T. Asaba , S. Ikemori , Y. Sekino , Y. Kasahara , K. Totsuka , B. Li , Y. Zhao , Y. Li , Y. Kohama , Y. Matsuda

The spin-$\frac{1}{2}$ kagome antiferromagnet is considered an ideal host for a quantum spin liquid ground state. We find that when the bonds of the kagome lattice are modulated with a periodic pattern, new quantum ground states emerge.…

Synthetic barlowite, Cu4(OH)6BrF, has emerged as a new quantum spin liquid (QSL) host, containing kagome layers of S=1/2 Cu2+ ions separated by interlayer Cu2+ ions. Similar to synthetic herbertsmithite, ZnCu3(OH)6Cl2, it has been reported…

Strongly Correlated Electrons · Physics 2018-05-02 C. M. Pasco , B. A. Trump , Thao T. Tran , Z. A. Kelly , C. Hoffmann , I. Heinmaa , R. Stern , T. M. McQueen

Quantum spin liquids (QSLs) are an exotic state of matter that is subject to extensive research. However, the relationship between the ubiquitous disorder and the QSL behaviors is still unclear. Here, by performing comparative experimental…

Realizing a quantum spin liquid (QSL) ground state in a real material is a leading issue in condensed matter physics research. In this pursuit, it is crucial to fully characterize the structure and influence of defects, as these can…

A quantum spin liquid is a novel ground state that can support long-range entanglement between magnetic moments, resulting in exotic spin excitations involving fractionalized $S=\frac{1}{2}$ spinons. Here, we measure the excitations in…

Quantum spin liquid (QSL) is a novel state of matter with exotic excitations and was theoretically predicted to be realized most possibly in an S=1/2 kagome antiferromagnet. Experimentally searching for the candidate materials is a big…

Strongly Correlated Electrons · Physics 2014-09-15 Yuesheng Li , Bingying Pan , Shiyan Li , Wei Tong , Langsheng Ling , Zhaorong Yang , Junfeng Wang , Zhongjun Chen , Zhonghua Wu , Qingming Zhang

The quantum spin liquid (QSL) is a highly entangled magnetic state characterized by the absence of static magnetism in its ground state. Instead, the spins fluctuate in a highly correlated way down to the lowest temperatures. The QSL is…

Spin-1/2 kagome materials have recently attracted a resurgence of interest as they are considered an ideal host of the quantum spin liquid (QSL) state, which can underpin functionality such as superconductivity. Here we report the first…

Strongly Correlated Electrons · Physics 2023-06-27 M. Georgopoulou , D. Boldrin , B. Fåk , P. Manuel , A. Gibbs , J. Ollivier , E. Suard , A. S. Wills

Quantum fluctuations enhanced by frustration and subtle interplay between competing degrees of freedom offer an ideal ground to realize novel states with fractional quantum numbers in quantum materials that defy standard theoretical…

A quantum spin liquid (QSL) is an exotic state of matter in which electrons' spins are quantum entangled over long distances, but do not show symmetry-breaking magnetic order in the zero-temperature limit. The observation of QSL states is a…

Strongly Correlated Electrons · Physics 2017-03-08 J. A. M. Paddison , M. Daum , Z. L. Dun , G. Ehlers , Y. Liu , M. B. Stone , H. D. Zhou , M. Mourigal

Based on experimental data and our theoretical analysis, we provide a strategy for unambiguous establishing of gapless quantum spin liquid state (QSL) in herbertsmithite and other materials. To clarify the nature of QSL, we recommend…

A quantum spin liquid is an exotic quantum state of matter in which spins are highly entangled and remain disordered down to zero temperature. Such a state of matter is potentially relevant to high-temperature superconductivity and…

Recent experiments suggest a quantum spin liquid ground state in the material PbCuTe$_2$O$_6$, where $S=1/2$ moments are coupled by antiferromagnetic Heisenberg interactions into a three dimensional structure of corner sharing triangles…

Strongly Correlated Electrons · Physics 2021-09-15 Li Ern Chern , Yong Baek Kim

A quantum spin liquid (QSL) is a state of matter where unpaired electrons' spins in a solid are quantum entangled, but do not show magnetic order in the zero-temperature limit. Because such a state may be important to the microscopic origin…

Geometric frustration of magnetic ions can lead to a quantum spin liquid ground state where long range magnetic order is avoided despite strong exchange interactions. The physical realization of quantum spin liquids comprises a major…

Strongly Correlated Electrons · Physics 2023-06-07 Alex Hallett , Catalina Avarvarei , John W. Harter

Quantum spin liquids (QSLs) are exotic states of matter characterized by emergent gauge structures and fractionalized elementary excitations. The recently discovered triangular lattice antiferromagnet YbMgGaO$_4$ is a promising QSL…

Strongly Correlated Electrons · Physics 2019-09-04 Yao Shen , Yao-Dong Li , H. C. Walker , P. Steffens , M. Boehm , Xiaowen Zhang , Shoudong Shen , Hongliang Wo , Gang Chen , Jun Zhao
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