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Utilizing the excess energy of photoexcitation that is otherwise lost as thermal effects can improve the efficiency of next-generation light-harvesting devices. Multiple exciton generation (MEG) in semiconducting materials yields two or…

Materials Science · Physics 2022-12-06 Ashish Soni , Dushyant Kushavah , Li-Syuan Lu , Wen-Hao Chang , Suman Kalyan Pal

In future solar cell technologies, the thermodynamic Shockley-Queisser limit for solar-to-current conversion in traditional p-n junctions could potentially be overcome with a bulk photovoltaic effect by creating an inversion broken symmetry…

The efficiencies of solar cells based on kesterite Cu$_2$ZnSnS$_4$ (CZTS) and Cu$_2$ZnSnSe$_4$ (CZTSe) are limited by a low open-circuit voltage due to high rates of non-radiative electron-hole recombination. To probe the origin of this…

Materials Science · Physics 2018-05-11 Bartomeu Monserrat , Ji-Sang Park , Sunghyun Kim , Aron Walsh

Extraction of hot carriers (HCs) over the band-edge is a key to harvest solar energy beyond Shockley-Queisser limit1. Graphene is known as a HC-layered material due to phonon bottleneck effect near Dirac point, but limited by low…

Applied Physics · Physics 2024-11-11 Kamal Kumar Paul , Ashok Mondal , Jae Woo Kim , Ji-Hee Kim , Young Hee Lee

Hot carrier solar cells allow potential efficiency close to the thermodynamical limit in ideal conditions. However, the feasability of such devices has not been clearly stated so far and only ideal cells were considered in previous studies.…

Controlling excitons and their transport in two-dimensional (2D) transition metal dichalcogenides (TMDs) heterostructures is central to advancing photonics and electronics on-chip integration. We investigate the controlled generation and…

The conversion efficiency of ultra-thin solar cells based on layered materials has been limited by their open-circuit voltage, which is typically pinned to a value under 0.6 V. Here we report an open-circuit voltage of 1.02 V in a 120…

P-n junctions based on vertically stacked single or few layer transition metal dichalcogenides (TMDCs) have attracted substantial scientific interest. Due to the propensity of TMDCs to show exclusively one type of conductivity, n- or…

A systematic survey and subsequent research have been made on MoTe2-based n-CdS/p-MoTe2/p+-CGS device in solar cell and photodetector field. The optimization has been established by altering the various properties of each constituent layer…

Absorbed sunlight in a solar cell produces electrons and holes. But, at the open circuit condition, the carriers have no place to go. They build up in density and, ideally, they emit external fluorescence that exactly balances the incoming…

Optics · Physics 2013-08-02 Owen D. Miller , Eli Yablonovitch , Sarah R. Kurtz

Independent current extraction in multi-junction solar cells has gained attention in recent years because it can deliver higher annual energy yield and can work for more semiconductor material combinations than the more established…

We propose a nanoscale heat engine that utilizes the physics of resonant tunneling in quantum dots in order to transfer electrons only at specific energies. The nanoengine converts heat into electrical current in a multiterminal geometry…

Mesoscale and Nanoscale Physics · Physics 2013-02-15 Andrew N. Jordan , Björn Sothmann , Rafael Sánchez , Markus Büttiker

We demonstrate for the first time that impact ionization (II) [the inverse of Auger recombination (AR)] occurs with very high efficiency in semiconductor nanocrystals (NCs). Interband optical excitation of PbSe NCs at low pump intensities,…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 R. D. Schaller , V. I. Klimov

In this report we review recent experimental results on photoexcited carrier relaxation dynamics on high temperature superconductors (HTSC) probed by a femtosecond time-resolved optical spectroscopy, and compare the results with the data…

Superconductivity · Physics 2015-06-24 Jure Demsar , Dragan Mihailovic , Viktor V. Kabanov

Prototypes for hot-carrier solar cells based on type-II InAs/AlAsSb multiple quantum wells are examined for AC photoconductivity as a function of lattice temperature and photoexcitation energy to determine the photoexcited charge carrier…

Mesoscale and Nanoscale Physics · Physics 2022-04-12 H. P. Piyathilaka , R. Sooriyagoda , V. R. Whiteside , T. D. Mishima , M. B. Santos , I. R. Sellers , A. D. Bristow

Moir\'e superlattices created by stacking atomic layers of transition metal dichalcogenide semiconductors have emerged as a class of fascinating artificial photonic and electronic materials. An appealing attribute of these structures is the…

Mesoscale and Nanoscale Physics · Physics 2025-03-11 Yueh-Chun Wu , Matthew DeCapua , ZhongChen Xu , Takashi Taniguchi , Kenji Watanabe , YouGuo Shi , Jun Yan

Harvesting hot carriers before they lose energy to the lattice is a critical route toward surpassing the conventional thermodynamic limit in optical-to-electrical (O-E) conversion. However, photocurrent from such hot carriers has remained…

Mesoscale and Nanoscale Physics · Physics 2025-06-18 Katsumasa Yoshioka , Taro Wakamura , Takuya Okamoto , Norio Kumada

Heterostructures (HSs) formed by the transition-metal dichalcogenides (TMDCs) materials have shown great promise in next-generation optoelectronic and photonic applications. An artificially twisted HS, allows us to manipulate the optical,…

The separation of hot carriers in semiconductors is of interest for applications such as thermovoltaic photodetection and third-generation photovoltaics. Semiconductor nanowires offer several potential advantages for effective hot-carrier…

We evaluate the limiting efficiency of full and partial solar spectrum harvesting via the process of internal photoemission in Au-semiconductor Schottky junctions. Our results based on the ab initio calculations of the electron density of…

Optics · Physics 2015-09-09 Svetlana V. Boriskina , Jiawei Zhou , Wei-Chun Hsu , Bolin Liao , Gang Chen