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Hot carrier-based energy conversion systems could double the efficiency of conventional solar energy technology or drive photochemical reactions that would not be possible using fully thermalized, ``cool'' carriers, but current strategies…

The hot carrier solar cell (HCSC) has the potential for converting solar energy into electrochemical energy with an efficiency of 85.4%. For this, in addition to an idealized light absorber, the HCSC has to be connected to the external load…

Applied Physics · Physics 2022-12-21 Antonio Martí , Elisa Antolín , Iñigo Ramiro

Hot-carrier solar cells are envisioned to utilize energy filtering to extract power from photogenerated electron-hole pairs before they thermalize with the lattice, and thus potentially offer higher power conversion efficiency compared to…

Mesoscale and Nanoscale Physics · Physics 2015-09-24 Steven Limpert , Stephen Bremner , Heiner Linke

Hot-carrier solar cells use the photon excess energy, that is, the energy exceeding the absorber bandgap, to do additional work. These devices have the potential to beat the upper limit for the photovoltaic power conversion efficiency set…

Materials Science · Physics 2025-02-21 Priya Viji , Constantin Tormann , Clemens Göhler , Martijn Kemerink

Extraction of charge carriers from a hot carrier solar cell using energy selective contacts, and the impact on limiting power conversion efficiency is analyzed. It is shown that assuming isentropic conversion of carrier heat into voltage…

Mesoscale and Nanoscale Physics · Physics 2015-09-24 Steven Limpert , Stephen Bremner

Utilizing hot carriers is the crucial approach for solar cell to exceed the thermodynamic detailed balance limit, yet effective extraction of hot carriers in absorber materials via most commonly used semiconductor acceptors has been a…

In optically excited two-dimensional phototransistors, charge transport is often affected by photodoping effects. Recently, it was shown that such effects are especially strong and persistent for graphene/h-BN heterostructures, and that…

Applied Physics · Physics 2019-03-06 Jorge Quereda , Talieh S. Ghiasi , Caspar H. van der Wal , Bart J. van Wees

Although van der Waals layered transition metal dichalcogenides from transient absorption spectroscopy have successfully demonstrated an ideal carrier multiplication (CM) performance with an onset of nearly 2Eg,interpretation of the CM…

Mesoscale and Nanoscale Physics · Physics 2021-04-20 Jun Suk Kim , Minh Dao Tran , Sung-Tae Kim , Daehan Yoo , Sang-Hyun Oh , Ji-Hee Kim , Young Hee Lee

Compared to traditional pn-junction photovoltaics, hot carrier solar cells offer potentially higher efficiency by extracting work from the kinetic energy of photogenerated "hot carriers" before they cool to the lattice temperature. Hot…

We apply an intense infrared laser pulse in order to perturb the electronic and vibrational states in the three-dimensional charge density wave material 1$T$-VSe$_2$. Ultrafast snapshots of the light-induced hot carrier dynamics and…

Photovoltaic cells usually have two terminals, one collecting electrons and the other collecting holes. Can more terminals improve such solar cells? Energy-filtering terminals could collect "hot" carriers (electrons or holes not yet relaxed…

Mesoscale and Nanoscale Physics · Physics 2025-07-18 Bruno Bertin-Johannet , Thibaut Thuégaz , Janine Splettstoesser , Robert S. Whitney

Efficient heat dissipation to the substrate is crucial for optimal device performance in nanoelectronics. We develop a theory of electronic thermal boundary conductance (TBC) mediated by remote phonon scattering for the single-layer…

Mesoscale and Nanoscale Physics · Physics 2020-09-28 Zhun-Yong Ong , Gang Zhang , Linyou Cao , Yong-Wei Zhang

An excitonic insulator phase is expected to arise from the spontaneous formation of electron-hole pairs (excitons) in semiconductors where the exciton binding energy exceeds the size of the electronic band gap. At low temperature, these…

Strongly Correlated Electrons · Physics 2022-09-02 Selene Mor , Marc Herzog , Claude Monney , Julia Stähler

Optoelectronic functionalities of photodection and light harnessing rely on the band-to-band excitation of semiconductors, thus the spectral response of the devices is dictated and limited by their bandgap. A novel approach, free from this…

Mesoscale and Nanoscale Physics · Physics 2014-06-12 F. Pelayo García de Arquer , Agustín Mihi , Gerasimos Konstantatos

The hot carrier solar cell (HCSC) concept has been proposed to overcome the Shockley Queisser limit of a single p-n junction solar cell by harvesting carriers before they have lost their surplus energy. A promising family of materials for…

Materials Science · Physics 2023-03-20 Tim Faber , Lado Filipovic , Jan Anton Koster

In this paper, we simulate the function of hot-carrier photocatalysts (HCPCs) with quantum well and quantum dot energy-selective contacts (ESCs) in the water-splitting reaction. The transport equations for these ESCs are derived by using…

Applied Physics · Physics 2024-12-25 Shuanglong Han , Zhiqiang Fan , Ousi Pan , Xiaohang Chen , Zhimin Yang , Yanchao Zhang , Jincan Chen , Shanhe Su

When plasmonic nanoparticles are coupled with semiconductors, highly energetic hot carriers can be extracted from the metal-semiconductor interface for various applications in light energy conversion. Hot charge-carrier extraction upon…

Moir\'e superlattices formed by transition metal dichalcogenide (TMD) heterobilayers provide a versatile platform for studying strongly correlated electronic, excitonic, and topological phenomena in solids. In particular, angle-aligned…

Rectification of thermal fluctuations in mesoscopic conductors is the key idea of today's attempts to build nanoscale thermoelectric energy harvesters in order to convert heat into a useful electric power. So far, most concepts make use of…

In conventional solar cell semiconductor materials (predominantly Si) photons with energy higher than the band gap initially generate hot electrons and holes, which subsequently cool down to the band edge by phonon emission. Due to the…

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