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High-order harmonic generation (HHG) is a powerful tool for probing electronic structure and ultrafast dynamics in matter. Traditionally studied in atomic and molecular gases, HHG has recently been extended to condensed matter, enabling…

Light carrying transverse orbital angular momentum (T-OAM) in the form of spatiotemporal optical vortices (STOVs) is opening new degrees of freedom for structured light manipulation. Such spatiotemporal wavepackets hold significant…

Optics · Physics 2025-11-25 Jinxin Wu , Dan Wang , Qingqing Liang , Jianhua Hu , Jiahao Dong , Jijun Feng , Yi Liu

We investigate the high harmonic generation (HHG) in solids driven by laser fields with different ellipticities. The HHG spectra show a two-plateau structure within the energy gap between the valence band and the first conduction band.…

Optics · Physics 2018-06-01 Liang Li , Pengfei Lan , Xiaosong Zhu , Tengfei Huang , Peixiang Lu

High harmonic generation (HHG) is an established means of producing coherent, short wavelength, ultrafast pulses from a compact set-up. Table-top high-harmonic sources are increasingly being used to image physical and biological systems…

We present theoretical studies of high-order harmonic generation (HHG) produced by non-homogeneous fields as resulting from the illumination of plasmonic nanostructures with a short laser pulse. We show that both the inhomogeneity of the…

Atomic Physics · Physics 2012-04-27 M. F. Ciappina , J. Biegert , R. Quidant , M. Lewenstein

Symmetries essentially provide conservation rules in nonlinear light-matter interactions, that facilitate control and understanding of photon conversion processes or electron dynamics. Since anisotropic solids have rich symmetries, they are…

We study high-order harmonic generation (HHG) resulting from the illumination of plasmonic nanostructures with a short laser pulse. We show that both the inhomogeneities of the local electric field and the confinement of the electron motion…

Atomic Physics · Physics 2012-04-27 M. F. Ciappina , Srdjan S. Acimovic , T. Shaaran , J. Biegert , R. Quidant , M. Lewenstein

High harmonic generation (HHG) is an extreme nonlinear process where intense pulses of light drive matter to emit high harmonics of the driving frequency, reaching the extreme ultraviolet (XUV) and x-ray spectral ranges. So far, the HHG…

Accelerating and colliding particles has been a key strategy to explore the texture of matter. Strong lightwaves can control and recollide electronic wavepackets, generating high-harmonic (HH) radiation which encodes the structure and…

Mesoscale and Nanoscale Physics · Physics 2016-04-14 M. Hohenleutner , F. Langer , O. Schubert , M. Knorr , U. Huttner , S. W. Koch , M. Kira , R. Huber

We present a comprehensive theoretical investigation of high-order harmonic generation in H$_2^+$ molecular ions within a quantum optical framework. Our study focuses on characterizing various quantum optical and quantum information…

High-harmonic generation (HHG) in the two topological phases of a finite, one-dimensional, periodic structure is investigated using a self-consistent time-dependent density functional theory (TDDFT) approach. For harmonic photon energies…

Optics · Physics 2018-04-26 Dieter Bauer , Kenneth K. Hansen

We experimentally disentangle the contributions of different quantum paths in high-order harmonic generation (HHG) from the spectrally and spatially resolved harmonic spectra. By adjusting the laser intensity and focusing position, we…

Atomic Physics · Physics 2015-10-08 Lixin He , Pengfei Lan , Qingbin Zhang , Chunyang Zhai , Feng Wang , Wenjing Shi , Peixiang Lu

Recently nonlocal spatial-mirror-symmetry-breaking metasurfaces have been proposed to generate spatiotemporal optical vortices (STOVs), which carry transverse orbital angular momenta. Here we investigate the topological property of the STOV…

Optics · Physics 2023-10-10 Junyi Huang , Hongliang Zhang , Tengfeng Zhu , Zhichao Ruan

We observe non-perturbative high harmonic generation in solids driven by a macroscopic quantum state of light, bright squeezed vacuum (BSV), which we generate in a single spatiotemporal mode. The BSV-driven process is considerably more…

High-order harmonic generation (HHG) in isolated atoms and molecules has been widely utilized in extreme ultraviolet (XUV) photonics and attosecond pulse metrology. Recently, HHG has also been observed in solids, which could lead to…

We develop a numerical scheme to investigate the high-order harmonic generation (HHG) in intense laser-matter interactions. Tracing the time evolution of every electronic laser-field-free state, we "observe" the HHG in a time-integrated…

Atomic Physics · Physics 2008-11-14 Y. J. Chen , J. Liu , Bambi Hu

Spatiotemporal Optical Vortices (STOVs) are structured electromagnetic fields propagating in free space with phase singularities in the space-time domain. Depending on the tilt of the helical phase front, STOVs can carry both longitudinal…

Optics · Physics 2024-03-26 Pronoy Das , Sathwik Bharadwaj , Zubin Jacob

We experimentally demonstrate how spatiotemporal optical vortices (STOVs) control long-range atmospheric filamentation of intense laser pulses. High-power pulses long enough to overlap with the delayed rotational nonlinearity of air…

Optics · Physics 2026-03-11 A. Goffin , L. Railing , G. Babic , H. M. Milchberg

We present the first experimental evidence, supported by theory and simulation, of spatiotemporal optical vortices (STOVs). Quantized STOVs are a fundamental element of the nonlinear collapse and subsequent propagation of short optical…

We study numerically the Bloch electron wavepacket dynamics in periodic potentials to simulate laser-solid interactions. We introduce a new perspective in the coordinate space combined with the motion of the Bloch electron wavepackets…

Optics · Physics 2018-01-12 Tao-Yuan Du , Xiao-Huan Huang , Xue-Bin Bian