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Laser pulses with stable electric field waveforms establish the opportunity to achieve coherent control on attosecond timescales. We present experimental and theoretical results on the steering of electronic motion in a multi-electron…

Temporally shaping the density of electron beams using light forms the basis for a wide range of established and emerging technologies, including free-electron lasers and attosecond electron microscopy. The modulation depth of compressed…

Quantum Physics · Physics 2021-08-18 Sergey V. Yalunin , Armin Feist , Claus Ropers

A precise understanding of mechanisms governing the dynamics of electrons in atoms and molecules subjected to intense laser fields has a key importance for the description of attosecond processes such as the high-harmonic generation and…

A single-atom 'double-slit' experiment is realized by photo-ionizing Rubidium atoms using two independent low power lasers. The photoelectron wave of well-defined energy recedes to the continuum either from the 5P or 6P states in the same…

Atomic Physics · Physics 2019-01-17 James Pursehouse , Andrew James Murray , Jonas Wätzel , Jamal Berakdar

Well isolated quantum systems are exquisite sensors of electromagnetic fields. In this work, we use a single trapped ion for characterizing chirped ultraviolet (UV) picosecond laser pulses. The frequency swept pulses resonantly drive a…

Attosecond observations of coherent electron dynamics in molecules and nanostructures can be achieved by combining conventional scanning tunneling microscopy (STM) with ultrashort femtosecond laser pulses. While experimental studies in the…

Quantum Physics · Physics 2024-10-01 Boyang Ma , Michael Krüger

Full insight into the dynamics of a coupled quantum system depends on the ability to follow the effect of a local excitation in real-time. Here, we trace the coherent evolution of a pair of coupled atomic spins by means of scanning…

Massively parallel ionization of many atoms in a cluster or bio-molecule is identified as new phenomenon of light-matter interaction which becomes feasible through short and intense FEL pulses. Almost simultaneously emitted from the…

Atomic and Molecular Clusters · Physics 2012-04-25 Christian Gnodtke , Ulf Saalmann , Jan-Michael Rost

This tutorial presents an introduction to the interaction of light and matter on the attosecond timescale. Our aim is to detail the theoretical description of ultra-short time-delays, and to relate these to the phase of extreme ultraviolet…

Atomic Physics · Physics 2012-07-20 J. M. Dahlström , A. L'Huillier , A. Maquet

Parametric amplification of attosecond coherent pulses around 100 eV at the single-atom level is demonstrated for the first time by using the 3D time-dependent Schr{\"o}dinger equation in high-harmonic generation processes from excited…

Optics · Physics 2020-08-26 C. Serrat , J. Seres , E. Seres , T-H. Dinh , N. Hasegawa , M. Nishikino , S. Namba

Photon exchange due to nuclear bremsstrahlung during nuclear collisions can cause Coulomb excitation in the projectile and the target nuclei. The corresponding process originated in nuclear timescales can also be observed in atomic…

When a single quantum of electromagnetic field excitation is added to the same spatio-temporal mode of a coherent state, a new field state is generated that exhibits intermediate properties between those of the two parents. Such a…

Quantum Physics · Physics 2007-05-23 Alessandro Zavatta , Silvia Viciani , Marco Bellini

Using extreme-ultraviolet attosecond-pulse-trains, we investigate the photoionization dynamics of a Helium atom in the presence of moderately-strong (~10^12 W/cm^2) femtosecond laser pulses. The electronic structure of a laser-dressed atom…

Atomic Physics · Physics 2011-08-02 Niranjan Shivaram , Henry Timmers , Xiao-Min Tong , Arvinder S. Sandhu

Advances in light sources and time resolved spectroscopy have made it possible to excite specific atomic vibrations in solids and to observe the resulting changes in electronic properties but the mechanism by which phonon excitation causes…

Superconductivity · Physics 2017-05-05 Dante M. Kennes , Eli Y. Wilner , David R. Reichman , Andrew J. Millis

It is a straightforward result of electromagnetism that dipole oscillators radiate more strongly when they are synchronized, and that if there are $N$ dipoles, the overall emitted intensity scales with $N^2$. In atomic physics, such an…

Optics · Physics 2020-07-22 C. Braggio , F. Chiossi , G. Carugno , A. Ortolan , G. Ruoso

Attosecond x-ray pulses play a crucial role in the study of ultrafast phenomena occurring within inner and valence electrons. To achieve attosecond time-resolution studies and gain control over electronic wavefunctions, it is crucial to…

Accelerator Physics · Physics 2024-01-30 Hao Sun , Xiaofan Wang , Weiqing Zhang

Shaking (shakeup + shakeoff) probabilities accompanying ion-atom collisions are studied using hydrogenic wavefunctions for K-, L-, M- shell electrons in the sudden approximation limit. The role of recoil velocity in the shaking processes is…

Atomic Physics · Physics 2023-07-19 Prashant Sharma , Tapan Nandi

The correlated behavior of electrons determines the structure and optical properties of molecules, semiconductor and other systems. Valuable information on these correlations is provided by measuring the response to femtosecond laser…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Shaul Mukamel , Rafal Oszwaldowski , Lijun Yang

Double ionization of an atom by single-photon absorption in the presence of a neighbouring atom is studied. The latter is, first, resonantly photoexcited and, afterwards, transfers the excitation energy radiationlessly to the other atom,…

Atomic Physics · Physics 2020-02-19 A. Eckey , A. B. Voitkiv , C. Müller

We study the role of electron-electron correlation in the ground-state of Ne, as well as in photoionization dynamics induced by an attosecond XUV pulse. For a selection of central photon energies around 100 eV, we find that while the…

Atomic Physics · Physics 2018-01-31 Juan J. Omiste , Lars Bojer Madsen