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An optical coherent control scheme has been proposed and theoretically investigated where an extreme ultraviolet single attosecond pulse (SAP) propagates through a dense helium gas dressed by a time-delayed femtosecond laser pulse. The…

Atomic Physics · Physics 2012-09-26 Wei-Chun Chu , C. D. Lin

Resonance fluorescence of natural or artificial atoms constitutes a prime method for generating non-classical light. While most efforts have focused on producing single-photons, multi-photon emission is unavoidably present in the resonant…

The photon-ion merged-beams technique was used at a synchrotron light source for measuring absolute cross sections of double and triple photodetachment of O$^{-}$ ions. The experimental photon energy range of 524-543 eV comprised the…

Atomic Physics · Physics 2016-10-07 S. Schippers , R. Beerwerth , L. Abrok , S. Bari , T. Buhr , M. Martins , S. Ricz , J. Viefhaus , S. Fritzsche , A. Müller

We study the classical dynamics of a Paul-trapped ion in a low-density bath of atoms above 1 $\mu\textrm{K}$. We find that lower energy collisions with more massive atoms, especially at energies less than the initial micromotion heating,…

Atomic Physics · Physics 2025-12-29 Saajid Chowdhury , Jesús Pérez Ríos

In a joint experimental and theoretical endeavour, photoionization of metastable C4+(1s 2s 3S1) ions via intermediate levels with hollow, double-K-vacancy configurations 2s2p, 2s3p, 2p3s, 2p3d, 2s4p, 2p4s and 2p4d has been investigated.…

A universal mechanism of ultrafast two-electron orbital swap is discovered through two-photon sequential double ionization of Li. After a $1s$ electron in Li is ionized by absorbing an EUV photon, the other two bound electrons located on…

Atomic Physics · Physics 2022-11-30 Hui Jiang , Zhao-Han Zhang , Yang Li , Camilo Ruiz , Feng He

For several decades, the interest of the scientific community in aneutronic fusion reactions such as proton-Boron fusion has grown because of potential applications in different fields. Recently, many scientific teams in the world have…

Plasma Physics · Physics 2021-09-27 X. Ribeyre , R. Capdessus , E. d'Humières , J. Wheeler , G. Mourou

Attochemistry aims to exploit the properties of coherent electronic wavepackets excited via attosecond pulses, to control the formation of photoproducts. Such molecular processes can in principle be simulated with various nonadiabatic…

Chemical Physics · Physics 2024-05-28 Thierry Tran , Anthony Ferté , Morgane Vacher

Nuclear orbiting resonances have been revealed at the sub-barrier energies as an atomic phenomenon by means of x-ray spectroscopy experiments. This interpretation is supported by several phenomenological models and theoretical estimates of…

Attosecond ionization time-delays at photoelectron energies above typically 10 eV are usually interpreted using the so called asymptotic approximation as a sum of the atomic or molecular delays with a universal laser-induced contribution.…

The swing-up of quantum emitter population (SUPER) scheme allows to populate the excited state of a quantum emitter with near-unity fidelity using two red-detuned laser pulses. Its off-resonant, yet fully coherent nature has attracted…

Quantum Physics · Physics 2024-09-19 Luca Vannucci , Niels Gregersen

Solitary waves have consistently captured the imagination of scientists, ranging from fundamental breakthroughs in spectroscopy and metrology enabled by supercontinuum light, to gap solitons for dispersionless slow-light, and discrete…

The pump-probe experiments enabled by X-ray free-electron lasers (XFEL) will allow us to directly observe correlated electronic motion with attosecond time resolution by detecting photoelectron pairs in coincidence. In helium, the…

We photoionize nitrogen molecules with a train of extreme ultraviolet attosecond pulses together with a weak infrared field. We measure the phase of the two-color two-photon ionization transition (molecular phase) for different states of…

We develop a first-principles simulation method for attosecond time-resolved photoelectron spectroscopy. This method enables us to directly simulate the whole experimental processes, including excitation, emission and detection on equal…

Atomic Physics · Physics 2018-08-01 Shunsuke A. Sato , Hannes Hübener , Angel Rubio , Umberto De Giovannini

The present review addresses the technical advances and the theoretical developments to realize and rationalize attosecond-science experiments that reveal a new dynamical time scale ($10^{-15}$-$10^{-18}$ s), with a particular emphasis on…

Chemical Physics · Physics 2020-02-07 Denitsa Baykusheva , Hans Jakob Wörner

Sympathetic cooling is the process of energy exchange between a system and a colder bath. We investigate this fundamental process in an atom-ion experiment where the system is composed of a single ion, trapped in a radio-frequency Paul…

Atomic Physics · Physics 2018-08-08 Ziv Meir , Meirav Pinkas , Tomas Sikorsky , Ruti Ben-shlomi , Nitzan Akerman , Roee Ozeri

The existence of electronic coherence can fundamentally change the scenario of nonlinear interaction of light with quantum systems such as atoms and molecules, which, however, has escaped from observation in the investigations of strong…

Attosecond spectroscopy of materials has provided invaluable insight into light-driven coherent electron dynamics. However, attosecond spectroscopies have so far been focused on weakly-correlated materials. As a result, the behavior of…

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