Related papers: Creating attosecond breathing ions by coherent sha…
We propose a new technique to fully characterize the temporal structure of extreme ultraviolet pulses by ionizing a bound coherent electronic wavepacket. The populated energy levels make it possible to interfere different spectral…
Time-resolved investigations of ultrafast electronic and molecular dynamics were not possible until recently. The typical time scale of these processes is in the picosecond to attosecond realm. The tremendous technological progress in…
Traditionally double neutrinoless electronic capture is considered as a resonance process. We have fulfilled shake-off probability calculations, leading to ionization of the electron shell, in the case of $^{164}$Er. Allowance for the…
We investigate dynamics of atomic and molecular systems exposed to intense, shaped chaotic fields and a weak femtosecond laser pulse theoretically. As a prototype example, the photoionization of a hydrogen atom is considered in detail. The…
Double photoionization by a single photon is often discussed in terms of two contributing mechanisms, {\it knock-out} (two-step-one) and {\it shake-off} with the latter being a pure quantum effect. It is shown that a quasi-classical…
Coupling between electrons and phonons (lattice vibrations) drives the formation of the electron pairs responsible for conventional superconductivity. The lack of direct evidence for electron-phonon coupling in the electron dynamics of the…
We theoretically study time-resolved photoemission in atoms as probed by attosecond streaking. We review recent advances in the study of the photoelectric effect in the time domain and show that the experimentally accessible time shifts can…
The implementation of attosecond photoelectron-photoion coincidence spectroscopy for the investigation of atomic and molecular dynamics calls for a high-repetition-rate driving source combined with experimental setups characterized by…
A pair of coherent femtosecond pulse excitations applied to a molecule with strong electron-phonon coupling creates a coherent superposition of a low momentum and a high momentum wavepacket in the vibrational states of both the excited…
Time-resolved photoelectron spectroscopy provides access to the electronic structure and non-equilibrium electron dynamics in matter. At solid surfaces photoemission dynamics can be investigated on its natural time scale by measuring…
Strong-field ionization generally produces ions in a superposition of ionic eigenstates. This superposition is generally not fully coherent und must be described in terms of a density matrix. A recent experiment [E. Goulielmakis et al.,…
The photoelectric effect is not truly instantaneous, but exhibits attosecond delays that can reveal complex molecular dynamics. Sub-femtosecond duration light pulses provide the requisite tools to resolve the dynamics of photoionization.…
We study four- and higher-order wave mixing of continuous coherent waves on a single superconducting artificial atom. Narrow side peaks of different orders of nonlinearity resulting from elastic multi-photon scattering on the atom are…
Coherence among rotational ion channels during photoionization is exploited to control the anisotropy of the resulting photoelectron angular distributions at specific photoelectron energies. The strategy refers to a robust and single…
Twenty-five years have passed since the first experimental demonstration of attosecond pulses, marking the advent of our ability to resolve and control electron motion in real time. What began as a technological breakthrough - generating…
Radiative nonlinear four-wave mixing can monitor the evolution of electronic wave packets, providing access to lifetimes and quantifies the light induced couplings between excited states. We report the observation of quantum beats in an…
Two emerging areas of research, attosecond and nanoscale physics, have recently started to merge. Attosecond physics deals with phenomena occurring when ultrashort laser pulses, with duration on the femto- and sub-femtosecond time scales,…
State-of-the-art attosecond metrology deals with the detection and characterization of photon pulses with typical energies up to the hundreds of eV and time resolution of several tens of attoseconds. Such short pulses are used for example…
The interaction between relativistic electron beams and intense laser fields has been extensively studied for generating high-energy radiation. However, achieving coherent radiation from such interactions needs to precisely control the…
When intense light irradiates a quantum system, an ionizing electron recollides with its parent ion within the same light cycle and, during that very brief (few femtosecond) encounter, its kinetic energy sweeps from low to high energy and…