Related papers: Unraveling Specific Conditions for a Repeatable Mp…
The performance of several popular water models (TIP3P, TIP4P, TIP5P and TIP4P/2005) is analysed. For that purpose the predictions for ten different properties of water are investigated, namely: 1. vapour-liquid equilibria (VLE) and…
The x-ray absorption spectra of water and ice are calculated with a many-body approach for electron-hole excitations. The experimental features, including the small effects of temperature change in the liquid, are quantitatively reproduced…
The investigation of water's glass transition and a possible liquid-liquid transition within its supercooled state is hampered by its inevitable crystallization in a temperature range, termed "no-man's land". Here we report…
In this fluid dynamics video we show how a drop of water freezes into a singular shape when deposited on a cold surface. The process of solidification can be observed very clearly due to the change in refraction when water turns into ice.…
The propagation of surface water waves over rough topographical bottoms is investigated by the multiple scattering theory. It is shown that the waves can be localized spatially through the process of multiple scattering and wave…
Heterogeneous ice growth exhibits a maximum in freezing rate arising from the competition between kinetics and the thermodynamic driving force between the solid and liquid states. Here, we use molecular dynamics simulations to elucidate the…
The distinctive characteristics of water, evident in its thermodynamic anomalies, have implications across disciplines from biology to geophysics. Considered a valid hypothesis to rationalize its unique properties, a liquid-liquid phase…
A drop of water that freezes from the outside-in presents an intriguing problem: the expansion of water upon freezing is incompatible with the self-confinement by a rigid ice shell. Using high-speed imaging we show that this conundrum is…
Tetrahedral liquids such as water and silica-melt show unusual thermodynamic behavior such as a density maximum and an increase in specific-heat when cooled to low temperatures. There is a debate in the literature whether these phenomena…
We show that the time dependent Dielectric Hole Burning experiments performed on supercooled liquids in the commented paper should be analyzed with a much shorter time step. The results would then exhibit strong short times oscillations,…
The properties of liquid water are known to change drastically in confined geometries. A most interesting and intriguing phenomenon is that the diffusion of water is found to be strongly enhanced by the proximity of a hydrophobic confining…
Inspired by responses to the work (arXiv:1310.6514), we solved the one-dimensional, nonlinear Fourier initial and boundary condition problem using the finite element method. Examination of all possible parameters reveals the following: 1.…
Recent experiments and theoretical studies strongly indicate that water exhibits a liquid-liquid phase transition (LLPT) in the supercooled domain. An open question is how the LLPT of water can affect the properties of aqueous solutions.…
Control of cooling and heating processes is essential in many industrial and biological processes. In fact, the time evolution of an observable quantity may differ according to the previous history of the system. For example, a system that…
When drinking a cup of coffee under the morning sunshine, you may notice white membranes of steam floating on the surface of the hot water. They stay notably close to the surface and appear to almost stick to it. Although the membranes…
Acoustic levitation is a container-free method for examining novel crystallization effects, though liquid-to-solid phase change has seen little investigation for levitated nanofluids. Recent developments have allowed for examining the…
Diffusivity, a measure for how rapidly a fluid self-mixes, shows an intimate, but seemingly fragmented, connection to thermodynamics. On one hand, the "configurational" contribution to entropy (related to the number of mechanically-stable…
The mechanisms of cold- and pressure-denaturation of proteins are matter of debate and are commonly understood as due to water-mediated interactions. Here we study several cases of proteins, with or without a unique native state, with or…
In this study, we present for the first time the observations of a freezing liquid marble. In the experiment, liquid marbles are gently placed on the cold side of a Thermo-Electric Cooler (TEC) and the morphological changes are recorded and…
The Mpemba effect, an example of anomalous thermal relaxations, occurs when a system prepared at a hot temperature overtakes an identical system prepared at a warm temperature and cools down faster to the environment's temperature. We study…