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We study the effect of electron-electron correlations on the quantum state of the light emitted from high-harmonic generation (HHG). The quantum state of the emitted light is obtained by using a fully quantum mechanical description of both…

Quantum Physics · Physics 2024-03-19 Christian Saugbjerg Lange , Thomas Hansen , Lars Bojer Madsen

To study excitonic effects on high-harmonic generation (HHG) in Mott insulators, we investigate pumped nonequilibrium dynamics in the one-dimensional extended Hubbard model. By employing time-dependent calculations based on the exact…

Strongly Correlated Electrons · Physics 2022-06-14 Mina Udono , Koudai Sugimoto , Tatsuya Kaneko , Yukinori Ohta

For decades, most research on high harmonic generation (HHG) considered matter as quantum but light as classical, leaving the quantum-optical nature of the harmonics an open question. Here we explore the quantum properties of high…

Quantum Physics · Physics 2023-11-21 Matan Even Tzur , Michael Birk , Alexey Gorlach , Ido Kaminer , Michael Krueger , Oren Cohen

High-harmonic generation (HHG) is a nonlinear process in which a strong driving field interacts with a material, resulting in the frequency up-conversion of the driver into its high-order harmonics. This process is highly sensitive to the…

Quantum Physics · Physics 2025-07-04 J. Rivera-Dean , P. Stammer , M. F. Ciappina , M. Lewenstein

Proposals for solid state quantum computing are extremely promising as they can be used to built room temperature quantum computers. If such a quantum computer is ever built it would require in-built sources of nonclassical states required…

Quantum Physics · Physics 2019-07-16 Arjun Mukherjee , Biswajit Sen , Kishore Thapliyal , Swapan Mandal , Anirban Pathak

Quantum-optical descriptions of strong-field processes have attracted significant attention in recent years. Typically, the theoretical modeling has been conducted in the Schr\"odinger picture, where results are only obtainable under…

High-harmonic generation (HHG) has recently emerged as a promising method for generating non-classical states of light with frequencies spanning from the infrared up to the extreme ultraviolet regime. In this work, we theoretically…

High-harmonic generation is a light up-conversion process occurring in a strong laser field, leading to coherent bursts of extreme ultrashort broadband radiation [1]. As a new perspective, we propose that ultrafast strong-field electronic…

The strong-field process of high-harmonic generation (HHG) has, in recent years, been treated from a quantum optical perspective in the emerging research area of strong-field quantum optics. These investigations show that HHG radiation is,…

Quantum Physics · Physics 2026-02-19 Christian Saugbjerg Lange , Lars Bojer Madsen

Energy-time entangled photons provide new opportunities for controlling multiphoton absorption beyond classical limits. Here, we investigate biexciton generation in nanocrystal quantum dots driven by energy-time-entangled quantum light…

Chemical Physics · Physics 2026-05-27 Kaiyue Peng , Chieh Tsao , Hendrik Utzat , Eran Rabani

High harmonic generation is a resource of extremely broad frequency combs of ultrashort light pulses. The non-classical nature of this new quantum source has been recently evidenced in semiconductors by showing that high harmonic generation…

Preparation of nonclassical light with special quantum properties is essential for quantum technologies. High-harmonic generation (HHG) is a process which not only enables the creation of attosecond pulses but also has the potential to…

Quantum Physics · Physics 2026-03-03 Ákos Gombkötő , Péter Ádám , David Theidel , Tamás Kiss

High harmonic generation (HHG) is an extreme nonlinear process where intense pulses of light drive matter to emit high harmonics of the driving frequency, reaching the extreme ultraviolet (XUV) and x-ray spectral ranges. So far, the HHG…

We investigate the effect of nonlocal interactions on the photo-doped Mott insulating state of the two-dimensional Hubbard model using a nonequilibrium generalization of the dynamical cluster approximation. In particular, we compare the…

Strongly Correlated Electrons · Physics 2020-02-26 Nikolaj Bittner , Denis Golez , Martin Eckstein , Philipp Werner

We present a comprehensive theoretical investigation of high-order harmonic generation in H$_2^+$ molecular ions within a quantum optical framework. Our study focuses on characterizing various quantum optical and quantum information…

Excitons are vital in the photophysics of materials, especially in low-dimensional systems. The conceptual and quantitative understanding of excitonic effects in nonlinear optical (NLO) processes is more challenging compared to linear ones.…

Materials Science · Physics 2026-02-26 Jiawei Ruan , Y. -H. Chan , Steven G. Louie

The nonlinear optical response of an excitonic insulator coupled to lattice degrees of freedom is shown to depend in strong and characteristic ways on whether the insulating behavior originates primarily from electron-electron or…

Strongly Correlated Electrons · Physics 2021-01-04 Denis Golez , Zhiyuan Sun , Yuta Murakami , Antoine Georges , Andrew J. Millis

High harmonic generation(HHG) is one of the most commonly studied nonlinear optical phenomena, originating in the ultrafast dynamics of electrons in atomic gasses and semiconductors. It has attracted much attention because of its…

Optics · Physics 2023-09-08 Akira Kofuji , Robert Peters

Quantum control of the many-body wavefunction is a central challenge in quantum materials research, as it could yield a precise control knob to manipulate emergent phenomena. Floquet engineering, the coherent dressing of quantum states with…

Strong-field high-harmonic generation (HHG) is conventionally described semiclassically, with the driving laser treated as a classical field. This approximation becomes insufficient in nanoscale interaction geometries, where extreme spatial…

Quantum Physics · Physics 2026-05-22 Tsendsuren Khurelbaatar , R. T. Sang , Igor Litvinyuk
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