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Using a combination of density functional theory (DFT) and spin-wave theory methods, we investigate the magnetic interactions and spin excitations in semiconducting VI$_3$. Exchange parameters of monolayer, bilayer, and bulk forms are…

Materials Science · Physics 2021-09-24 Elijah Gordon , V. V. Mkhitaryan , Haijun Zhao , Y. Lee , Liqin Ke

alpha-UTe3, a van der Waals (vdW) actinide compound with a monoclinic ZrSe3-type structure, is a narrow-gap semiconductor with 5f moments. 125Te NMR reveals strongly anisotropic, layer-confined spin fluctuations below about 20 K, with the…

Strongly Correlated Electrons · Physics 2025-10-14 H. Sakai , C. Tabata , K. Kaneko , Y. Tokiwa , T. Kitazawa , S. Kambe , Y. Tokunaga , Y. Haga

Two-dimensional materials have proven to be a prolific breeding ground of new and unstudied forms of magnetism and unusual metallic states, particularly when tuned between their insulating and metallic phases. In this paper we present work…

Strongly Correlated Electrons · Physics 2019-01-02 C. R. S. Haines , M. J. Coak , G. I. Lampronti , C. Liu , H. Hamidov , A. R. Wildes , D. Daisenberger , P. Nahai-Williamson , S. S. Saxena

Recent experimental work shows that FePS$_3$ undergoes phase transitions from $C2/m$ ($\beta\sim107^{\circ}$) to $C2/m$ ($\beta\sim90^{\circ}$) at $6$ GPa and then to metallic $P\bar{3}1m$ at $14$ GPa, with the magnetic ordering wave vector…

Materials Science · Physics 2022-12-12 Yijie Zeng , Dao-Xin Yao , Man-Rong Li

Interest in van der Waals materials often stems from a desire to miniaturise existing technologies by exploiting their intrinsic layered structure to create near atomically-thin components that do not suffer from surface defects. One…

Mesoscale and Nanoscale Physics · Physics 2022-08-22 A. J. Healey , S. Rahman , S. C. Scholten , I. O. Robertson , G. J. Abrahams , N. Dontschuk , B. Liu , L. C. L. Hollenberg , Y. Lu , J. -P. Tetienne

Nonlocal magnon transport can provide valuable insight into the magnetic properties of magnetic insulators (MIs). A spin-flop transition, a typical magnetic reorientation in antiferromagnets, is expected to affect mag non transport, but…

Mesoscale and Nanoscale Physics · Physics 2025-05-30 Peisen Yuan , Beatriz Martín-García , Evgeny Modin , M. Xochitl Aguilar-Pujol , Fèlix Casanova , Luis E. Hueso

Electric-field switching of magnetic order is of significant physical interest and holds great potential for spintronic applications. However, it has rarely been reported in two-dimensional (2D) van der Waals (vdW) magnets due to the…

Materials Science · Physics 2025-02-06 Chengxi Huang , Jinzhe Han , Jing Wang , Jintao Jiang , Ziyang Qu , Fang Wu , Ang Li , Yi Wan , Kaiyou Wang , Erjun Kan

The unique discovery of magnetic exciton in van der Waals antiferromagnet NiPS3 arises between two quantum many-body states of a Zhang-Rice singlet excited state and a Zhang-Rice triplet ground state. Simultaneously, the spectral width of…

Two-dimensional multiferroic van der Waals heterostructures provide a promising platform for the simultaneous control of distinct ferroic orders, with potential applications in magnetoelectric devices and spintronics. The practical…

Materials Science · Physics 2025-09-03 Priyanshu Raj , Sourav Mal , Rana Saha , Prasenjit Sen

We provide a complete and systematic first-principles study of the thermodynamic stability, structural parameters, and magnetic properties of the T1 non-collinear antiferromagnetic L1$_2$-IrMn$_3$ surface and L1$_2$-IrMn$_3$/Fe…

Materials Science · Physics 2020-10-16 Daniel Maldonado-Lopez , Noboru Takeuchi , Jonathan Guerrero-Sanchez

Magnetic van der Waals (vdW) materials have opened new frontiers for realizing novel many-body phenomena. Recently NiPS3 has received intense interest since it hosts an excitonic quasiparticle whose properties appear to be intimately linked…

Strongly Correlated Electrons · Physics 2024-04-29 W. He , Y. Shen , K. Wohlfeld , J. Sears , J. Li , J. Pelliciari , M. Walicki , S. Johnston , E. Baldini , V. Bisogni , M. Mitrano , M. P. M. Dean

Van der Waals magnets provide opportunities for exploring low-dimensional magnetism and spintronic phenomena. The Mermin-Wagner theorem states that long-range correlations in reduced dimensions are stabilized and controlled by magnetic…

Electrical gate-manipulated exchange bias (EB) effect is a long-term goal for spintronics applications. Meanwhile, the emergence of van der Waals (vdW) magnetic heterostructures provides ideal platforms for the study of interlayer magnetic…

Two-dimensional van der Waals (vdW) heterostructures are an attractive platform for studying exchange bias due to their defect free and atomically flat interfaces. Chromium thiophosphate (CrPS4), an antiferromagnetic material, possesses…

We present a computational study to explore the potential of different experimental approaches to tune the magnetic interactions in two-dimensional van der Waals magnets. We selected CrGeSe$_3$, CrGeTe$_3$, and Janus Cr$_2$Ge$_2$(Se,Te)$_3$…

Mesoscale and Nanoscale Physics · Physics 2024-11-14 Gabriel Martínez-Carracedo , Amador García-Fuente , László Oroszlány , László Szunyogh , Jaime Ferrer

Optical magneto-spectroscopy methods (Raman scattering, far-infrared transmission, and photoluminescence) have been applied to investigate the properties of the NiPS3 semiconducting antiferromagnet. The fundamental magnon gap excitation in…

Mesoscale and Nanoscale Physics · Physics 2023-06-14 Dipankar Jana , P. Kapuscinski , I. Mohelsky , D. Vaclavkova , I. Breslavetz , M. Orlita , C. Faugeras , M. Potemski

Studying antiferromagnetic domains is essential for fundamental physics and potential spintronics applications. Despite its importance, few systematic studies have been performed on van der Waals (vdW) antiferromagnets (AFMs) domains with…

Despite extensive research, the precise spin Hamiltonian of the van der Waals antiferromagnet NiPS$_3$ -- which hosts a zigzag-ordered ground state -- remains debated. While consensus has emerged on ferromagnetic nearest-neighbor ($J_1$)…

Strongly Correlated Electrons · Physics 2026-03-27 Qiang Luo , Shuhang Yang , Xiaoying Wang , Zhengyu Jiang , Chunlan Ma , Yan Zhu

Manipulating the interlayer magnetic coupling in van der Waals magnetic materials and heterostructures is the key to tailoring their magnetic and electronic properties for various electronic applications and fundamental studies in condensed…

Materials Science · Physics 2020-08-19 Zhe Li , Jiaheng Li , Ke He , Xiangang Wan , Wenhui Duan , Yong Xu

Fe3-xGeTe2 is a layered magnetic van der Waals material of interest for both fundamental and applied research. Despite the observation of intriguing physical properties, open questions exist even on the basic features related to magnetism:…