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Related papers: Interplanar magnetic exchange in CoPS$_3$

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Igniting interface magnetic ordering of magnetic topological insulators by building a van der Waals heterostructure can help to reveal novel quantum states and design functional devices. Here, we observe an interesting exchange bias effect,…

Compounds with two-dimensional (2D) layers of magnetic ions weakly connected by van der Waals bonding offer routes to enhance quantum behavior, stimulating both fundamental and applied interest. CrPS4 is one such magnetic van der Waals…

Strongly Correlated Electrons · Physics 2020-07-07 S. Calder , A. V. Haglund , Y. Liu , D. M. Pajerowski , H. B. Cao , T. J. Williams , V. O. Garlea , D. Mandrus

FePS$_3$ is a prototype van der Waals layered antiferromagnet and a Mott insulator under ambient conditions, which has been recently reported to go through a pressure-induced dimensionality crossover and an insulator-to-metal transition.…

Strongly Correlated Electrons · Physics 2023-07-19 Shiyu Deng , Siyu Chen , Bartomeu Monserrat , Emilio Artacho , Siddharth S Saxena

Two-dimensional antiferromagnetism has long attracted significant interest in many areas of condensed matter physics, but only recently has experimental exploration become feasible due to the isolation of van der Waals antiferromagnetic…

Mesoscale and Nanoscale Physics · Physics 2025-11-21 Cheol-Yeon Cheon , Volodymyr Multian , Kenji Watanabe , Takashi Taniguchi , Alberto F. Morpurgo , Dmitry Lebedev

Two-dimensional van der Waals magnetic materials are of great current interest for their promising applications in spintronics. In this work, using density functional theory calculations in combination with the maximally localized Wannier…

Materials Science · Physics 2024-01-30 Guangyu Wang , Ke Yang , Yaozhenghang Ma , Lu Liu , Di Lu , Yuxuan Zhou , Hua Wu

Magneto-spectroscopy methods have been employed to study the zero-wavevector magnon excitations in MnPSe$_3$. Experiments carried out as a function of temperature and the applied magnetic field show that two low-energy magnon branches of…

Lamellar structures of transition metal phosphorus trisulfides possess strong intralayer bonding, albeit adjacent layers are held by weak van der Waals interactions. Those compounds received enormous interest due to their unique combination…

We calculate the magnon dispersion spectra of the two-dimensional zigzag van der Waals antiferromagnet NiPS$_3$ for monolayer, bilayer, and bulk systems as a function of an external magnetic field. We calculate the exchange and anisotropy…

Layered van-der-Waals 2D magnetic materials are of great interest in fundamental condensed-matter physics research, as well as for potential applications in spintronics and device physics. We present neutron powder diffraction data using…

We have performed electrochemical treatment of the van der Waals antiferromagnetic materials FePS$_3$ and NiPS$_3$ with the ionic liquid EMIM-BF$_4$, achieving significant molecular intercalation. Mass analysis of the intercalated…

Strongly Correlated Electrons · Physics 2024-05-07 Cong Li , Ze Hu , Xiaofei Hou , Sheng Xu , Zhanlong Wu , Kefan Du , Shuo Li , Xiaoyu Xu , Ying Chen , Zeyu Wang , Tiancheng Mu , Tian-Long Xia , Yanfeng Guo , B. Normand , Weiqiang Yu , Yi Cui

Antiferromagnetic van der Waals family $\rm \textit{M}P\textit{X}_{3}\ (M=Fe,\ Mn,\ Co,\text{ and}\ Ni; X=S\text{ and}\ Se)$ have attracted significant research attention due to the possibility of realizing long-range magnetic order down to…

Strongly Correlated Electrons · Physics 2024-06-11 Junbo Liao , Zhentao Huang , Yanyan Shangguan , Bo Zhang , Shufan Cheng , Hao Xu , Ryoichi Kajimoto , Kazuya Kamazawa , Song Bao , Jinsheng Wen

The exchange bias (EB) effect, pivotal in magnetic data storage and sensing devices, has been observed not only in interfacial regions but also in intrinsic ferromagnetic materials. Here, we've uncovered a robust and stable exchange bias…

Materials Science · Physics 2023-12-29 Xi Zhang , Xiuquan Xia , Qiye Liu , Yonggang He , Le Wang , Junhao Lin , Jia-Wei Mei , Yingchun Cheng , Jun-Feng Dai

NiPS3 is an exfoliable van-der-Waals intralayer antiferromagnet with zigzag-type spin arrangement. It is distinct from other TMPS3 (TM: transition metal) materials by optical excitations into a strongly correlated state that is tied to the…

Magnon gap excitations selectively coupled to phonon modes have been studied in FePSe$_3$ layered antiferromagnet with magneto-Raman scattering experiments performed at different temperatures. The bare magnon excitation in this material has…

Recent developments in two-dimensional (2D) magnetism have motivated the search for novel van-der Waals (vdWs) magnetic materials to explore new magnetic phenomenon in the 2D limit. Metal thiophosphates, MPX3, is a class of magnetic vdWs…

Materials Science · Physics 2021-06-30 Rabindra Basnet , Aaron Wegner , Krishna Pandey , Stephen Storment , Jin Hu

How to electrically control magnetic properties of a magnetic material is promising towards spintronic applications, where the investigation of carrier doping effects on antiferromagnetic (AFM) materials remains challenging due to their…

We present comprehensive measurements of the structural, magnetic and electronic properties of layered van-der-Waals ferromagnet VI$_3$ down to low temperatures. Despite belonging to a well studied family of transition metal trihalides,…

Van der Waals (vdW) magnetic heterostructures offer a versatile platform for engineering interfacial spin interactions with atomic precision, enabling nontrivial spin textures and dynamic behaviors. In this work, we report robust asymmetric…

We studied magnetic states and phase transitions in the van der Waals antiferromagnet VBr3 by specific heat and magnetization measurements of single crystals in high magnetic fields and by ab initio density functional theory calculations…

Magnetic anisotropy is a key parameter to describe the exchange bias effect in heterostructures. In this paper, we describe explicit density functional calculations of the magnetic structure of an interface between the industrially…

Materials Science · Physics 2025-09-03 Robert A. Lawrence , Matt I. J. Probert