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The interplay between collective optical response and molecular static and dynamic disorder is studied using simple effective Hamiltonians for an ensemble of two-level emitters inside and outside a single-mode cavity. We model environmental…

Chemical Physics · Physics 2022-11-30 Zeyu Zhou , Hsing-Ta Chen , Joseph E. Subotnik , Abraham Nitzan

The notion of strong light-matter coupling is typically associated with the observation of Rabi splitting, corresponding to the formation of the hybrid light-matter states known as polaritons. However, this relationship is derived based on…

Chemical Physics · Physics 2025-12-03 Wei-Kuo Li , Hsing-Ta Chen

The strong coupling between molecules and photonic modes in a Fabry-P\'{e}rot optical cavity, which forms hybrid light-matter states called polaritons, has been demonstrated as a promising route to control the rates of chemical reactions.…

Quantum Physics · Physics 2025-05-22 Kunyang Sun , Matthew Du , Joel Yuen-Zhou

The effect of disorder in the intensity of the driving laser on a coupled array of cavities described by a Bose-Hubbard Hamiltonian for dark-state polaritons is investigated. A canonically-transformed Gutzwiller wave function is used to…

Other Condensed Matter · Physics 2020-05-15 Abuenameh Aiyejina , Roger Andrews

We consider molecules confined to a microcavity whose dimensions are such that an excitation of the molecule is nearly resonant with a cavity mode. We investigate the situation where the excitation energies of the molecules are randomly…

Quantum Physics · Physics 2022-06-01 Tarun Gera , K. L. Sebastian

We study the dependence of the vacuum Rabi splitting (VRS) on frequency disorder, vibrations, near-field effects and density in molecular polaritonics. In the mesoscopic limit, static frequency disorder alone can already introduce a loss…

Quantum Physics · Physics 2021-08-23 Christian Sommer , Michael Reitz , Francesca Mineo , Claudiu Genes

This study investigates the dynamic behavior of polaritons in an optical cavity containing one million molecules, emphasizing the influence of molecular rotation and level disorder on the coupling between molecules and photons. Through…

Optics · Physics 2024-02-22 Wei Liu , Jingqi Chen , Wenjie Dou

We investigate the effect of disorder in the laser intensity on the dynamics of dark-state polaritons in an array of 20 cavities, each containing an ensemble of four-level atoms that is described by a Bose-Hubbard Hamiltonian. We examine…

Mesoscale and Nanoscale Physics · Physics 2020-05-15 Abuenameh Aiyejina , Roger Andrews

Cavity quantum electrodynamics advances the coherent control of a single quantum emitter with a quantized radiation field mode, typically piecewise engineered for the highest finesse and confinement in the cavity field. This enables the…

Coherent light-matter interaction at the single photon and electronic qubit level promises the remarkable potential for nonclassical information processing. Against the efforts of improving the figure of merit of the cavities, here we…

Quantum Physics · Physics 2015-06-19 Yong-Chun Liu , Xingsheng Luan , Hao-Kun Li , Qihuang Gong , Chee Wei Wong , Yun-Feng Xiao

The manipulation of molecular excited state processes through strong coupling has attracted significant interest for its potential to provide precise control of photochemical phenomena. However, the key limiting factor for achieving this…

We present a comprehensive investigation of the light-matter interaction dynamics in two-dimensional materials coupled with a spectrally isolated cavity mode in the strong coupling regime. The interaction between light and matter breaks the…

Mesoscale and Nanoscale Physics · Physics 2023-12-18 Maria Vittoria Gurrieri , Emil V. Denning , Kristian Seegert , Philip T. Kristensen , Jesper Mørk

In this article we report about linear and nonlinear optical properties of intersubband cavity polariton samples, where the resonant photonic mode is a defect state in a metallo-dielectric photonic crystal slab. By tuning a single geometric…

Mesoscale and Nanoscale Physics · Physics 2016-05-31 Simone Zanotto , Federica Bianco , Giorgio Biasiol , Lucia Sorba , Alessandro Tredicucci

The interplay between static and dynamic disorder and collective optical response in molecular ensembles is an important characteristic of nanoplasmonic and nanophotonic molecular systems. Here we investigate the cooperative superradiant…

Many types of dissipative processes can be found in nature or be engineered, and their interplay with a system can give rise to interesting phases of matter. Here we study the interplay among interaction, tunneling, and disorder in the…

Quantum Gases · Physics 2018-04-18 Xiansong Xu , Chu Guo , Dario Poletti

The dynamics of arbitrary-order quantum correlations in a cavity magnon-polariton system are investigated based on the quantum master equation in the coherent state representation. The phenomena of Rabi-like oscillation and level repulsion…

Quantum Physics · Physics 2021-10-25 Guogan Zhao , Yong Wang , X. -F. Qian

When the interaction between a molecular system and confined light modes in an optical or plasmonic cavity is strong enough to overcome the dissipative process, hybrid light-matter states (polaritons) become the fundamental excitations in…

Mesoscale and Nanoscale Physics · Physics 2020-01-08 Yu Zhang , Tammie Nelson , Sergei Tretiak

We study ultracold atoms in a finite size one-dimensional optical lattice prepared in the Mott insulator phase and commonly coupled to a single cavity mode. Due to resonance dipole-dipole interactions among the atoms, electronic excitations…

Quantum Physics · Physics 2009-08-10 Hashem Zoubi , Helmut Ritsch

Strong coupling in the conventional sense requires that the Rabi cycling process between two interacting states is faster than other dissipation rates. Some recent experimental findings show intriguing properties that were attributed to…

Materials Science · Physics 2026-03-09 Ben Johns , Nitin Yadav , Anand Vinod , Kuljeet Kaur , Jino George

We study the interplay between disorder and light-matter coupling by considering a disordered one-dimensional chain of lossy dipoles coupled to a multimode optical cavity, through a microscopically derived Hamiltonian. Such a system,…

Mesoscale and Nanoscale Physics · Physics 2023-01-04 Thomas F. Allard , Guillaume Weick
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