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We perform a quantum-theoretical treatment of cavity linewidth narrowing with intracavity electromagnetically induced transparency (EIT). By means of intracavity EIT, the photons in the cavity are in the form of cavity polaritons:…

Quantum Physics · Physics 2015-04-10 G. W. Lin , J. Yang , X. M. Lin , Y. P. Niu , S. Q. Gong

Interactions between atoms and light in optical cavities provide a means of investigating collective (many-body) quantum physics in controlled environments. Such ensembles of atoms in cavities have been proposed for studying collective…

We realize a ring cavity strongly interacting with an atom array with configurable spatial structures. By preparing the atom array with a maximized structure factor, we observe the emergence of a cavity dark mode, where the standing-wave…

Quantum Physics · Physics 2024-10-29 Xiaotian Zhang , Zhanhai Yu , Hongrui Zhang , Di Xiang , Hao Zhang

From the high vibrational dipolar strength offered by molecular liquids, we demonstrate that a molecular vibration can be ultra-strongly coupled to multiple IR cavity modes, with Rabi splittings reaching $24\%$ of the vibration frequencies.…

Strong coupling of molecules to the vacuum field of micro cavities can modify the potential energy surfaces opening new photophysical and photochemical reaction pathways. While the influence of laser fields is usually described in terms of…

Quantum Physics · Physics 2016-02-08 Markus Kowalewski , Kochise Bennett , Shaul Mukamel

Molecular polaritons arise when molecules interact so strongly with light that they become entangled with each other. This light-matter hybridization alters the chemical and physical properties of the molecular system and allows chemical…

Chemical Physics · Physics 2023-07-28 Tor S. Haugland , John P. Philbin , Tushar K. Ghosh , Ming Chen , Henrik Koch , Prineha Narang

We study the tunable photonic distribution in an optical molecule consisting of two linearly coupled single-mode cavities. With the inter-cavity coupling and two driving fields, the energy levels of the optical-molecule system form a closed…

Quantum Physics · Physics 2017-01-18 Z. H. Wang , Y. Li

The optical emission spectrum of a quantum dot in strong coupling with the single mode of a microcavity is obtained in the nonlinear regime. We study how exciton-exciton interactions alter the emission spectrum of the system, bringing the…

Mesoscale and Nanoscale Physics · Physics 2009-07-09 E. del Valle , F. P. Laussy , F. M. Souza , I. A. Shelykh

We demonstrate a new type of transition within the strong coupling regime, which alters the coupling mechanism in multimode cavities. We show that this transition drastically modifies the Hamiltonian describing the polaritons, such that…

Mesoscale and Nanoscale Physics · Physics 2021-06-16 M. Balasubrahmaniyam , C. Genet , T. Schwartz

Recent experiments and theory demonstrate that the the ground state properties and chemical reactivity of molecules can be modified inside an optical cavity. The vibrational strong or ultrastrong coupling results in the formation of…

Chemical Physics · Physics 2022-12-01 Qi Yu

Harnessing strong light-matter interactions to control chemical reactions in confined electromagnetic fields offers a promising route toward deepening our understanding of chemical dynamics at the collective quantum-mechanical level, with…

Chemical Physics · Physics 2026-01-21 Yaling Ke

An ensemble of identical, intrinsically non-interacting molecules exposed to quantum light is discussed. Their interaction with the quantum light induces interactions between the molecules. The resulting hybrid light-matter states exhibit…

Chemical Physics · Physics 2024-06-19 Lorenz S. Cederbaum

We analyze equilibrium properties of coupled-doped cavities described by the Jaynes-Cummings- Hubbard Hamiltonian. In particular, we characterize the entanglement of the system in relation to the insulating-superfluid phase transition. We…

Quantum Physics · Physics 2012-04-26 Eduardo Mascarenhas , Libby Heaney , M. C. O. Aguiar , Marcelo França Santos

Ionization phenomena are widely studied for decades. With the advent of cavity technology, the question arises how quantum light affects molecular ionization. As the ionization spectrum is recorded from the neutral ground state, it is…

Chemical Physics · Physics 2024-04-23 Csaba Fábri , Gábor J. Halász , Lorenz S. Cederbaum , Ágnes Vibók

A model designed to mimic the implications of the collective optical response of molecular ensembles in optical cavities on molecular vibronic dynamics is investigated. Strong molecule-radiation field coupling is often reached when a large…

Chemical Physics · Physics 2022-10-05 Bingyu Cui , Abraham Nitzan

Dark states are excited quantum states that decouple from their environment in such a way that they do not emit or absorb external photons. These states are found in a variety of different open quantum systems and can be derived from the…

Quantum Physics · Physics 2026-05-06 Christopher Campbell , Matti Silveri

We investigate optical nonlinear interactions in a dynamic environment by studying generation of photons in spontaneous parametric down conversion inside a nonlinear cavity where the optical path length is periodically modulated in time. We…

Optics · Physics 2019-10-16 Usman A. Javid , Qiang Lin

The control of light transmission through a Fabry-Perot cavity containing atoms is theoretically investigated, when the cavity mode beam and an intersecting control beam are both close to specific atomic resonances. A four-level atomic…

Optics · Physics 2016-02-10 Rahul Sawant , S. A. Rangwala

Polaritons are usually described within single-mode cavity QED models. However, nanophotonic environments typically involve several modes that spectrally overlap and interfere, giving rise to sharp dip features such as Fano profiles in the…

Recent experiments have observed that the chemical and photophysical properties of molecules can be modified inside an optical Fabry-Perot microcavity under collective vibrational strong coupling (VSC) conditions, and such modification is…

Mesoscale and Nanoscale Physics · Physics 2021-03-09 Tao E. Li , Abraham Nitzan , Joseph E. Subotnik