Related papers: Phase-matching of high harmonic generation in twis…
High-harmonic generation (HHG) is widely used for up-conversion of amplified (near) infrared ultrafast laser pulses to short wavelengths. We demonstrate that Ramsey-comb spectroscopy, based on two such pulses derived from a frequency-comb…
Highly-efficient optical generation of narrowband terahertz (THz) radiation enables unexplored technologies and sciences from compact electron acceleration to charge manipulation in solids. State-of-the-art conversion efficiencies are…
In this report, a novel methodology based on the static coherent states approach is introduced with the capability of calculating various strong-field laser-induced nonlinearities in full dimensional single-electron molecular systems; an…
High-order harmonic generation (HHG) from crystals offers a new source of coherent extreme ultraviolet (XUV) attosecond radiation.
We study high order harmonics generation (HHG) in crystalline silicon and diamond subjected to near and mid-infrared laser pulses. We employ time-dependent density functional theory and solve the time-dependent Kohn-Sham equation in the…
Fourth-generation storage-ring light sources have achieved transverse emittances approaching the diffraction limit at x-ray wavelengths, while their longitudinal coherence remains limited. Existing laser-modulation schemes can induce strong…
Vigorous efforts to harness the topological properties of light have enabled a multitude of novel applications. Translating the applications of structured light to higher spatial and temporal resolutions mandates their controlled…
In moir\'e crystals resulting from the stacking of twisted two-dimensional (2D) layered materials, a subtle adjustment in the twist angle surprisingly gives rise to a wide range of correlated optical and electrical properties. Herein, we…
Applying time-dependent local density approximation (TDLDA), we study the high-order harmonic generation (HHG) of ethylene subjected to the one-color ($\omega=2.72$ eV) and the two-color ($\omega_1=2.72$ eV and $\omega_2=5.44$ eV)…
High-quality ultrafast light sources are critical for developing advanced time- and angle-resolved photoemission spectroscopy (TrARPES). While the application of high harmonic generation (HHG) light sources in TrARPES has increased…
Metasurfaces have emerged as a promising platform for integrated nonlinear optics. Nonlocal metasurfaces enable high nonlinear conversion efficiency, while the local ones can offer versatile wavefront control, yet achieving both within a…
Collinear double-pulse seeding of the High-Gain Harmonic Generation (HGHG) process in a free-electron laser (FEL) is a promising approach to facilitate various coherent nonlinear spectroscopy schemes in the extreme ultraviolet (XUV)…
Phosphorene, a well-studied 2D allotrope of phosphorus, features unique properties such as widely tunable bandgap, high carrier mobility, and remarkable intrinsic in-plane anisotropy. Utilizing these structural and electronic properties, we…
High-order harmonic generation (HHG) in aligned linear molecules can offer valuable information about strong-field interactions in lower-lying molecular orbitals, but extracting this information is difficult for three-dimensional molecular…
Light beams carrying orbital angular momentum (OAM) have led to stunning applications in various fields from quantum information to microscopy. In this letter, we examine OAM from the recently discovered high-harmonic generation (HHG) in…
The strong ellipticity dependence of high-harmonic generation in gases enables numerous experimental techniques that are nowadays routinely used, for instance, to create isolated attosecond pulses. Extending such techniques to high-harmonic…
A scheme for quasi-phase-matching high-harmonic generation is proposed in which polarization beating within a hollow core birefringent waveguide modulates the generation of harmonics. The evolution of the polarization of a laser pulse…
We theoretically investigate the orientation dependence of high-harmonic generation (HHG) in monolayer transition metal dichalcogenides (TMDCs). We find that, unlike conventional solid-state and atomic layered materials such as graphene,…
High-harmonic generation (HHG) in liquids is opening new opportunities for attosecond light sources and attosecond time-resolved studies of dynamics in the liquid phase. In gas-phase HHG, few-cycle pulses are routinely used to create…
We theoretically demonstrate x-ray second harmonic generation (SHG) with strong-field-driven high harmonic generation (HHG) from core electrons in gas-phase atoms, highlighting its potential as a powerful spectroscopic tool for studying…