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We report terahertz spectroscopic measurements of quantum spin dynamics in the spin-1/2 honeycomb magnet Na$_2$Co$_2$TeO$_6$ as a function of applied magnetic field with different terahertz polarizations. Distinct field dependencies of the…

Strongly Correlated Electrons · Physics 2023-10-12 Patrick Pilch , Laur Peedu , Anup Kumar Bera , S. M. Yusuf , Urmas Nagel , Toomas Rõõm , Zhe Wang

We present a comprehensive study of single crystals of Na2Co2TeO6, a putative Kitaev honeycomb magnet, focusing on its low-temperature phase behaviors. A new thermal phase transition is identified at 31.0 K, below which the system develops…

Strongly Correlated Electrons · Physics 2021-05-26 Wenjie Chen , Xintong Li , Zhenhai Hu , Ze Hu , Li Yue , Ronny Sutarto , Feizhou He , Kazuki Iida , Kazuya Kamazawa , Weiqiang Yu , Xi Lin , Yuan Li

The honeycomb magnet $\alpha-$RuCl$_3$ is a prime candidate material for realizing the Kitaev quantum spin liquid (QSL), but it shows long-range magnetic order at low temperature. Nevertheless, its broad inelastic neutron scattering (INS)…

Strongly Correlated Electrons · Physics 2022-11-23 Oliver Franke , Dumitru Călugăru , Andreas Nunnenkamp , Johannes Knolle

We report on terahertz spectroscopy of quantum spin dynamics in $\alpha$-RuCl$_3$, a system proximate to the Kitaev honeycomb model, as a function of temperature and magnetic field. An extended magnetic continuum develops below the…

Strongly Correlated Electrons · Physics 2017-11-30 Zhe Wang , S. Reschke , D. Hüvonen , S. -H. Do , K. -Y. Choi , M. Gensch , U. Nage , T. Rõõm , A. Loidl

We report on the results of 23Na NMR in the honeycomb lattice magnet Na2Co2TeO6 which has been nominated as a Kitaev material. Measurements of magnetic shift and width of the NMR line as functions of temperature and magnetic field show that…

Strongly Correlated Electrons · Physics 2022-12-21 Jun Kikuchi , Takayuki Kamoda , Nobuyoshi Mera , Yodai Takahashi , Kouji Okumura , Yukio Yasui

Spin-orbit coupled honeycomb magnets with the Kitaev interaction have received a lot of attention due to their potential of hosting exotic quantum states including quantum spin liquids. Thus far, the most studied Kitaev systems are…

We have investigated the magnetic properties and mapped out the phase diagram of the honeycomb magnet Na2Co2TeO6 with Co 3d7 in out-of-plane magnetic fields. This material has previously been proposed to show nearest-neighbor Kitaev…

Strongly Correlated Electrons · Physics 2024-06-03 Shengzhi Zhang , Sangyun Lee , Eric Brosha , Qing Huang , Haidong Zhou , Vivien S. Zapf , Minseong Lee

Na2Co2TeO6 is a proposed approximate Kitaev magnet, yet its actual magnetic interactions are elusive due to a lack of knowledge on the full excitation spectrum. Here, using inelastic neutron scattering and single crystals, we determine the…

Strongly Correlated Electrons · Physics 2022-10-04 Weiliang Yao , Kazuki Iida , Kazuya Kamazawa , Yuan Li

The honeycomb magnet Na$_3$Co$_2$SbO$_6$ recently emerged as a promising candidate for realizing Kitaev quantum spin liquid with relatively low levels of structural disorder. While the precise spin Hamiltonian remains controversial, the…

Strongly Correlated Electrons · Physics 2025-07-16 Rongsheng Li , Liyu Shi , Yuchen Gu , Yue Chen , Xintong Li , Qiong Wu , Shuxiang Xu , Dong Wu , Yuan Li , Fa Wang , Tao Dong , Nanlin Wang

The layered honeycomb iridate $\alpha$-Li$_2$IrO$_3$ displays an incommensurate magnetic structure with counterrotating moments on nearest-neighbor sites, proposed to be stabilized by strongly-frustrated anisotropic Kitaev interactions…

Strongly Correlated Electrons · Physics 2019-03-06 Sungkyun Choi , S. Manni , J. Singleton , C. V. Topping , T. Lancaster , S. J. Blundell , D. T. Adroja , V. Zapf , P. Gegenwart , R. Coldea

Na$_2$Co$_2$TeO$_6$ has recently been proposed to be a Kitaev-like honeycomb magnet. To assess how close it is to realizing Kitaev quantum spin liquids, we have measured magnetization and specific heat on high-quality single crystals in…

Strongly Correlated Electrons · Physics 2020-02-19 Weiliang Yao , Yuan Li

$^7$Li nuclear magnetic resonance (NMR) and terahertz (THz) spectroscopies are used to probe magnetic excitations and their field dependence in the hyperhoneycomb Kitaev magnet $\beta$-Li$_2$IrO$_3$. Spin-lattice relaxation rate ($1/T_1$)…

Strongly Correlated Electrons · Physics 2020-06-16 M. Majumder , M. Prinz-Zwick , S. Reschke , A. Zubtsovskii , T. Dey , F. Freund , N. Büttgen , A. Jesche , I. Kézsmárki , A. A. Tsirlin , P. Gegenwart

The 3$d^7$ Co$^{2+}$-based insulating magnet \NCTO{} has recently been reported to have strong Kitaev interactions on a honeycomb lattice, and is thus being considered as a Kitaev quantum spin liquid candidate. However, due to the existence…

We report vibrating coil magnetometry of the spin ice system Ho2Ti2O7 down to ~0.04 K for magnetic fields up to 5 T applied parallel to the [111] axis. History dependent behavior emerges below T*_0 ~ 0.6 K near zero magnetic field, in…

Strongly Correlated Electrons · Physics 2012-06-25 C. Krey , S. Legl , S. R. Dunsiger , M. Meven , J. S. Gardner , J. M. Roper , C. Pfleiderer

The intriguing interplay between competing degrees of freedom in frustrated magnets can lead to non-trivial magnetic phenomena with exotic low-energy excitations that are highly relevant for addressing some of the fundamental questions in…

Strongly Correlated Electrons · Physics 2026-03-20 A. Yadav , U. Jena , A. Pradhan , Satish K. , P. Khuntia

A polycrystalline sample of the hyperhoneycomb iridate $\beta$-ZnIrO$_3$ was synthesized via a topochemical reaction, and its structural, magnetic, and thermodynamic properties were investigated. The magnetization and heat capacity data…

Strongly Correlated Electrons · Physics 2022-02-17 Yuya Haraguchi , Akira Matsuo , Koichi Kindo , Hiroko Aruga Katori

We consider the quasi-two-dimensional pseudo-spin-1/2 Kitaev - Heisenberg model proposed for A2IrO3 (A=Li, Na) compounds. The spin-wave excitation spectrum, the sublattice magnetization, and the transition temperatures are calculated in the…

Strongly Correlated Electrons · Physics 2016-08-24 A. A. Vladimirov , D. Ihle , N. M. Plakida

The magnetic phase diagram of CuFeO2 as a function of applied magnetic field and temperature is thoroughly explored and expanded, both for magnetic fields applied parallel and perpendicular to the material's c-axis. Pulsed field…

Materials Science · Physics 2015-05-18 Tom T. A. Lummen , Cornelius Strohm , Harison Rakoto , Paul H. M. van Loosdrecht

Despite exhibiting magnetic long-range order below $T_\mathrm{N} = 26.7\,\mathrm{K}$, the honeycomb cobaltate Na$_2$Co$_2$TeO$_6$ is predicted to enter a Kitaev spin liquid state when subjected to small external perturbations. While most of…

Strongly Correlated Electrons · Physics 2026-03-04 J. Arneth , R. Kalaivanan , R. Sankar , K. -Y. Choi , R. Klingeler

In the quest to find quantum spin liquids, layered cobalt oxides Na2Co2TeO6 and Na3Co2SbO6 have been proposed as promising candidates for approximating the Kitaev honeycomb model. Yet, their suitability has been thrown into question due to…

Strongly Correlated Electrons · Physics 2024-04-25 Ping Miao , Xianghong Jin , Weiliang Yao , Yue Chen , Akihiro Koda , Zhenhong Tan , Wu Xie , Wenhai Ji , Takashi Kamiyama , Yuan Li
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