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Oxide semimetals exhibiting both nontrivial topological characteristics stand as exemplary parent compounds and multiple degrees of freedom, offering great promise for the realization of novel electronic states. In this study, we present…

The nuclear magnetic resonance (NMR) spectrum of spin-3/2 nuclei in a static magnetic field aligned with one of the electric field gradient (EFG) principal axes is developed analytically, based on fictitious spin-1/2 formalism. Compact…

Superconductivity · Physics 2024-12-17 Jaafar N. Ansari , Karen L. Sauer

The protonation of N2 bound to the active center of nitrogenase has been investigated using state-of-the-art DFT calculations. Dinitrogen in the bridging mode is activated by forming two bonds to Fe sites, which results in a reduction of…

Biomolecules · Quantitative Biology 2007-05-23 Johannes Kaestner , Sascha Hemmen , Peter E. Bloechl

Designing efficient, metal free, and in-expensive catalyst for electrochemical hydrogen evolution reaction (HER) is crucial for large scale clean and green energy production. Recently synthesized 1D Biphenylene nanoribbons (BPRs) display…

Materials Science · Physics 2024-05-29 Radha N Somaiya , Zicong Marvin Wong , Brahmananda Chakraborty , Teck Leong Tan , Aftab Alam

Nitrogen doping study on niobium (Nb) samples used for the fabrication of the superconducting radio frequency (SRF) cavities has been carried out. The samples' surface treatment was attempted to replicate that of the SRF cavities, which…

Accelerator Physics · Physics 2018-04-23 Ziqin Yang , Xiangyang Lu , Yuan He , Weiwei Tan , Shichun Huang , Hao Guo

We present a density functional theory study of the oxygen reduction reaction (ORR) on a single atom catalyst embedded in graphene, namely, TM-N$_{4}$-C (TM = Fe and Co), using the effective screening medium method combined with the…

Materials Science · Physics 2024-02-28 Azim Fitri Zainul Abidin , Ikutaro Hamada

Chemical substitution during growth is a well-established method to manipulate electronic states of quantum materials, and leads to rich spectra of phase diagrams in cuprate and iron-based superconductors. Here we report a novel and generic…

Developing advanced catalysts for acidic oxygen evolution reaction (OER) is crucial for sustainable hydrogen production. This study introduces a novel, multi-stage machine learning (ML) approach to streamline the discovery and optimization…

Materials Science · Physics 2024-07-09 Rui Ding , Jianguo Liu , Kang Hua , Xuebin Wang , Xiaoben Zhang , Minhua Shao , Yuxin Chen , Junhong Chen

Currently, the fundamental factors that control the oxygen reduction reaction (ORR) activity of graphene itself, in particular the dependence of the ORR activity on the number of exposed edge sites remain elusive, mainly due to limited…

Materials Science · Physics 2014-11-18 John Benson , Qian Xu , Peng Wang , Yuting Shen , Litao Sun , Tanyuan Wang , Meixian Li , Pagona Papakonstantinou

Controlling the dynamics of DNA translocation is a central issue in the emerging nanopore-based DNA sequencing. To address the potential of heteroatom doping of carbon nanostructures to achieve this goal, herein we carry out atomistic…

Mesoscale and Nanoscale Physics · Physics 2018-08-13 Sang Won Jung , Han Seul Kim , Art E. Cho , Yong-Hoon Kim

Ammonia poses significant environmental challenges due to its role in water pollution, contributing to eutrophication and several detrimental environmental and ecological issues. Addressing the efficient removal or conversion of ammonia is,…

Fuel cells offer an alternative to burning fossil fuels, but use platinum as a catalyst which is expensive and scarce. Cheap, alternative catalysts could enable fuel cells to become serious contenders in the green energy sector. One…

Kohn-Sham density functional theory and plane wave basis set based ab initio molecular dynamics (AIMD) simulation is a powerful tool for studying complex reactions in solutions, such as electron transfer (ET) reactions involving…

Chemical Physics · Physics 2022-09-07 Sagarmoy Mandal , Ritama Kar , Bernd Meyer , Nisanth N. Nair

Metal heteroatoms dispersed in nitrogen-doped graphene display promising catalytic activity for fuel cell reactions such as the hydrogen evolution reaction (HER). Here we explore the effects of dopant concentration on the synergistic…

The adsorption and desorption of carbon dioxide (CO2) molecule by alkaline earth metal (AEM) (Mg+2, Ca+2, Sr+2 and Ba+2) functionalized on graphitic boron nitride (g-B4N3) nanosheet have been analyzed by using density functional theory…

Mesoscale and Nanoscale Physics · Physics 2018-05-30 Shivam Kansara , Sanjeev K. Gupta , Yogesh Sonvane , Anurag Srivastava

Oxygen evolution reaction (OER) electrolysis, as an important reaction involved in water splitting and rechargeable metal-air battery, has attracted increasing attention for clean energy generation and efficient energy storage. Nickel/iron…

Materials Science · Physics 2014-11-19 Ming Gong , Hongjie Dai

Nb3O2(OH) has emerged as a highly attractive photocatalyst based on its chemical stability, energetic band positions, and large active lattice sites. Compared to other various photocatalytic semiconductors, it can be synthesized easily.…

Materials Science · Physics 2025-02-17 Wilayat Khan , Alishba Tariq , Jan Minar , Sawera Durrani , Abdul Raziq , Sikander Azam , Khalid Saeed

Precious-metal-free spinel oxide electrocatalysts are promising candidates for catalyzing the oxygen reduction reaction (ORR) in alkaline fuel cells. In this theory-driven study, we use joint density-functional theory in tandem with…

In this work, hybridization of nonmetal nitrogen-doped carbon dots (NCQDs) with ZnO nanorods (NRs) is utilized towards better photocatalytic degradation of rhodamine B under ultraviolet (UV) irradiation. The structural characterization is…

Materials Science · Physics 2021-08-11 Sujoy Kumar Mandal , Sumana Paul , Sujoy Datta , Debnarayan Jana

The current work studies the electrocatalytic performance of NaNbO$_3$ microcubes decorated with WO$_3$ nanoparticles on Printex L6 at varying concentrations (1%, 3%, 5%, and 10% by weight) for H$_2$O$_2$ electrogeneration aiming for future…

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