Related papers: Spin-chirality-driven second-harmonic generation i…
Second-harmonic generation (SHG) microscopy provides label-free imaging of biological tissues with unique contrast mechanisms, but its resolution is limited by the diffraction limit. Here, we present the first experimental demonstration of…
We demonstrate second harmonic generation (SHG) in an $x$-cut congruent lithium niobate (LN) whispering gallery mode resonator. We first show theoretically that independent control of the coupling of the pump and signal modes is optimal for…
Optical-field sampling using second-harmonic generation (SHG) from strong-field ionization enables ultrabroadband terahertz detection, but the microscopic origin of the SHG signal and its ultrabroadband response have been unclear. Here we…
MnBi2Te4 is a van der Waals topological insulator with intrinsic intralayer ferromagnetic exchange and A-type antiferromagnetic interlayer coupling. Theoretically, it belongs to a class of structurally centrosymmetric crystals whose layered…
We analytically investigate the effect of a non-centrosymmetric geometry in the optical second harmonic (SH) generation from a particle made of a centrosymmetric material, in the interior of which quadratic optical processes are suppressed.…
Chip-scale nonlinear optics enables strong light-matter interactions within compact devices, serving as a fundamental platform for multifunctional integrated photonics from classical optical signal processing to quantum information…
We show that the concept of coherent phonon generation by second order response to incident electric laser fields, which is a hallmark of pump-probe spectroscopy on conventional solids, can be expanded to include frustrated quantum magnets.…
On the basis of the Edward-Kornfeld formulation, we study the effective susceptibility of secondharmonic generation (SHG) in colloidal crystals, which are made of graded metallodielectric nanoparticles with an intrinsic SHG susceptibility…
Optical generation of complex spin textures is one of the most exciting challenges of modern spintronics. Here, we uncover a distinct physical mechanism for imprinting spin chirality into collinear magnets with short laser pulses. By…
Giant second-harmonic generation (SHG) in the terahertz (THz) frequency range is observed in a thin film of an s-wave superconductor NbN, where the time-reversal ($\mathcal{T}$-) and space-inversion ($\mathcal{P}$-) symmetries are…
We report the first observation of nonlinear harmonic generation and sum frequency generation (SFG) coupled with stimulated Raman scattering (SRS) via the second-order (\chi^{(2)}) and the third-order (\chi^{(3)}) nonlinearities in a silica…
The interplay of polarization and magnetism in materials with light can create rich nonlinear magneto-optical (NLMO) effects, and the recent discovery of two-dimensional (2D) van der Waals magnets provides remarkable control over NLMO…
Structured light carrying orbital angular momentum enables new regimes of nonlinear light-matter interaction. Here we develop a molecular quantum electrodynamics description of third-harmonic generation (THG) driven by focused…
Spin currents proportional to the first- and second-order of the electric field are calculated in a specific tight-binding model with time-reversal symmetry. Specifically, a tight-binding model with time-reversal symmetry is constructed…
In chiral magnets with intrinsic inversion symmetry breaking, it has been known that two spin waves moving in opposite directions can propagate at different velocities, exhibiting a phenomenon called magnetochiral nonreciprocity which…
Optical materials with centrosymmetry, such as silicon and germanium, are unfortunately absent of second-order nonlinear optical responses, hindering their developments in efficient nonlinear optical devices. Here, a design with an array of…
Chiral discrimination with high harmonic generation (cHHG method) has been introduced in the recent work by R. Cireasa et al ( Nat. Phys. 11, 654 - 658, 2015). In its original implementation, the cHHG method works by detecting high harmonic…
Chirality and topology are intimately related fundamental concepts, which are heavily explored to establish spin-textures as potential magnetic bits in information technology. However, this ambition is inhibited since electrical reading of…
Second harmonic generation (SHG) is forbidden in centrosymmetric molecular materials. However, a signal is frequently observed from interfaces where the symmetry is broken. Whereas the effect can be phenomenologically accommodated, an ab…
Diffractive neural networks (DNNs) are an emerging approach for the realization of photonic artificial intelligence, especially due to their suitability for machine-vision applications and high-dimensional photonic information processing at…