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We have detected second-order nonlinear optical response from an amphoteric mega-saccharides named sacran under a needle/ring electrode stimulus by using an optical second harmonic generation (SHG) microscope. SHG was observed from sacran…

Second-harmonic generation allows for coherently bridging distant regions of the optical spectrum, with applications ranging from laser technology to self-referencing of frequency combs. However, accessing the nonlinear response of a medium…

Chirality characterizes the asymmetry between a structure and its mirror image and underlies a wide range of chiral functionalities. In crystallographically chiral materials, phonons with non-zero linear momentum $\textbf{k}$ can acquire a…

Strongly Correlated Electrons · Physics 2025-12-02 J. Okamoto , C. Y. Mou , H. Y. Huang , G. Channagowdra , C. Won , K. Du , X. Fang , E. V. Komleva , C. T. Chen , S. V. Streltsov , A. Fujimori , S-W. Cheong , D. J. Huang

Second harmonic generation (SHG) is a nonlinear optical response arising exclusively from broken inversion symmetry in the electric-dipole limit. Recently, SHG has attracted widespread interest as a versatile and noninvasive tool for…

A comprehensive analysis of second harmonic generation (SHG) in a diatomic zincblende crystal based on the Simplified Bond Hyperpolarizability Model (SBHM), Group Theory (GT) is presented. The third rank tensor between the two approaches…

Controlling magnetic order via external fields or heterostructures enables precise manipulation and tracking of spin and exciton information, facilitating the development of high-performance optical spin valves. However, the weak…

Materials Science · Physics 2024-09-30 Jia Shi , Dan Wang , Nai Jiang , Ziqian Xin , Houzhi Zheng , Chao Shen , Xinping Zhang , Xinfeng Liu

Polar textures have attracted significant attention in recent years as a promising analog to spin-based textures in ferromagnets. Here, using optical second harmonic generation based circular dichroism, we demonstrate deterministic and…

Magnetization-induced optical third-harmonic generation (MTHG) is observed in magnetic nanostructures: Co and Fe nanolayers and granular films containing Co nanoparticles. Magnetization-induced variations of the MTHG characteristics in…

Materials Science · Physics 2013-05-29 O. A. Aktsipetrov , E. M. Kim , R. V. Kapra , T. V. Murzina

Understanding the mechanisms and spatial correlations of crystallographic symmetry breaking in ferroelectric materials is essential to tuning their functional properties. While optical second harmonic generation (SHG) has long been utilized…

Materials Science · Physics 2022-08-10 Wei Li , Yunpeng Ma , Tianyi Feng , Sergei V. Kalinin , Jing-Feng Li , Qian Li

We have investigated second harmonic generation (SHG) from Ag-coated LiNbO3 (LN) core-shell nanocuboids and found that giant SHG can occur via deliberately designed double plasmonic resonances. By controlling the aspect ratio, we can tune…

Optics · Physics 2014-11-19 Ming-Liang Ren , Si-Yuan Liu , Ben-Li Wang , Bao-Qin Chen , Jiafang Li , Zhi-Yuan Li

Generation of second-harmonic waves is one of the universal nonlinear phenomena that have found numerous technical applications in many modern technologies, in particular, in photonics. This phenomenon also has great potential in the field…

Mesoscale and Nanoscale Physics · Physics 2024-03-01 K. O. Nikolaev , S. R. Lake , G. Schmidt , S. O. Demokritov , V. E. Demidov

We demonstrate pronounced electric-field-induced second-harmonic generation in naturally inversion symmetric 2H stacked bilayer MoS$_{2}$ embedded into microcapacitor devices. By applying strong external electric field perturbations ($|F| =…

We report the first application of pump-probe second harmonic generation (SHG) measurements to characterize optically-induced magnetization in non-magnetic multilayer semiconductors. In the experiment, coherent spins are selectively excited…

Condensed Matter · Physics 2009-11-07 Yu. D. Glinka , T. V. Shahbazyan , I. E. Perakis , N. H. Tolk , X. Liu , Y. Sasaki , J. K. Furdyna

High harmonic generation (HHG) records the ultrafast electronic response of matter to light, encoding key properties of the interrogated quantum system, such as chirality. The first implementation of chiral HHG [Cireasa et al. Nat. Phys.…

Imaging antiferromagnetic 180{\deg} domains with actively controlled visibility is vital for both fundamental science and sophisticated applications. While optical second-harmonic generation (SHG) is a well-known technique for…

Strongly Correlated Electrons · Physics 2024-09-02 Ziqian Wang , Meng Wang , Jannis Lehmann , Yuki Shiomi , Taka-hisa Arima , Naoto Nagaosa , Yoshinori Tokura , Naoki Ogawa

In the past decade, chiral materials have drawn significant attention because it is widely claimed that they can act as spin injectors/detectors due to the chirality-induced spin selectivity (CISS) effect. Nevertheless, the microscopic…

Mesoscale and Nanoscale Physics · Physics 2024-09-30 Sytze H. Tirion , Bart J. van Wees

The emerging field of silicon photonics seeks to unify the high bandwidth of optical communications with CMOS microelectronic circuits. Many components have been demonstrated for on-chip optical communications, including those that utilize…

Optics · Physics 2015-05-20 Jacob S. Levy , Mark A. Foster , Alexander L. Gaeta , Michal Lipson

Chiral phonons are desirable for applications in spintronics but their generation and control remains a challenge.Here we demonstrate the emergence of truly chiral phonons from selective magnon-phonon coupling in inversion-symmetric…

We report the observation of optical second harmonic generation (SHG) in single-layer indium selenide (InSe). We measure a second harmonic signal of $>10^3$ $\textrm{cts/s}$ under nonresonant excitation using a home-built confocal…

Chirality is breaking of mirror symmetry in matter. In the fields of biology and chemistry, this is particularly important because some of the essential molecules in life such as amino acids and DNA have chirality. It is a long-standing…

Strongly Correlated Electrons · Physics 2019-07-04 N. Jiang , Y. Nii , H. Arisawa , E. Saitoh , Y. Onose
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