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Using a first principles approach, we studied the hydrogen evolution reaction activity of newly synthesized biphenylene and B, N, P decorated biphenylene sheet. hydrogen evolution reaction activity of pristine biphenylene sheet is not…

Materials Science · Physics 2023-12-29 Mukesh Singh , Alok Shukla , Brahmananda Charkraborty

The photocatalytic production of hydrogen peroxide (H$_2$O$_2$) from water is a promising strategy for solar-to-chemical energy conversion. Herein, we investigate the effect of metal-free heteroatom doping (B, O, P, and S) on the…

The hybrid nanostructures of nitrogen doped carbon materials and nonprecious transition metals are among the most promising electrocatalysts to replace noble metal catalysts for renewable energy applications. However, the fundamental…

Materials Science · Physics 2018-05-14 Wei Pei , Si Zhou , Yizhen Bai , Jijun Zhao

Metal heteroatoms dispersed in nitrogen-doped graphene display promising catalytic activity for fuel cell reactions such as the hydrogen evolution reaction (HER). Here we explore the effects of dopant concentration on the synergistic…

The present study investigates the catalytic performance of a $hg-C_{3}N_{4}$ quantum dot aimed at enhancing electrochemical water splitting, using the first-principles density functional theory. The size of the considered quantum dot lies…

Materials Science · Physics 2024-08-08 Khushboo Dange , Vaishali Roondhe , Alok Shukla

Introduction of interstitial dopants has opened a new pathway to optimize nanoparticle catalytic activity for, e.g., hydrogen evolution/oxidation and other reactions. Here, we discuss the stability of a property-enhancing dopant, B,…

The ability to efficiently evolve hydrogen via electrocatalysis at low overpotentials holds tremendous promise for clean energy. Hydrogen evolution reaction (HER) can be easily achieved from water if a voltage above the thermodynamic…

Designing efficient, metal free, and in-expensive catalyst for electrochemical hydrogen evolution reaction (HER) is crucial for large scale clean and green energy production. Recently synthesized 1D Biphenylene nanoribbons (BPRs) display…

Materials Science · Physics 2024-05-29 Radha N Somaiya , Zicong Marvin Wong , Brahmananda Chakraborty , Teck Leong Tan , Aftab Alam

In the present paper, we investigate the structural, thermodynamic, dynamic, elastic, and electronic properties of doped 2D diamond C$_4$X$_2$ (X = B or N) nanosheets in both AA$'$A$''$ and ABC stacking configurations, by first-principles…

Materials Science · Physics 2024-01-10 Bruno Ipaves , João F. Justo , Biplab Sanyal , Lucy V. C. Assali

A first-principles investigation of the electronic and quantum transport properties of double-walled carbon nanotubes doped with nitrogen and boron atoms is presented. Concentric nanotube sidewalls separated by the typical graphitic van der…

Materials Science · Physics 2016-03-24 Alejandro Lopez-Bezanilla

BiVO4, a visible-light response photocatalyst, has shown tremendous potential because of abundant raw material sources, good stability and low cost. There exist some limitations for further applicaitions due to poor capability to separate…

Applied Physics · Physics 2021-07-07 Can Fu , Baoyun Xu , Lingling Dong , Jinguo Zhai , Xuefei Wang , De-Yi Wang

Identifying a nanostructure suitable for hydrogen storage presents a promising avenue for the secure and cost-effective utilization of hydrogen as a green energy source. This study introduces a systematic approach for selecting optimal…

Materials Science · Physics 2023-12-08 Shima Rezaie , Azahara Luna-Triguero

Since hydrogen fuel involves the highest energy density among all fuels, production of this gas through the solar water splitting approach has been suggested as a green remedy for greenhouse environmental issues due to extensive consumption…

Computational Physics · Physics 2018-03-22 Meysam Makaremi , Sean Grixti , Keith T. Butler , Geoffrey A. Ozin , Chandra Veer Singh

Graphynes offer a chemically heterogeneous $sp/sp^{2}$ carbon framework with distinct electronic regimes and site-selective reactivity. Here, Density Functional Theory and Reactive Molecular Dynamics Simulations are combined to evaluate…

Controlling the dynamics of DNA translocation is a central issue in the emerging nanopore-based DNA sequencing. To address the potential of heteroatom doping of carbon nanostructures to achieve this goal, herein we carry out atomistic…

Mesoscale and Nanoscale Physics · Physics 2018-08-13 Sang Won Jung , Han Seul Kim , Art E. Cho , Yong-Hoon Kim

With the global transition towards cleaner energy and sustainable processes, the demand for efficient catalysts, especially for the oxygen reduction reaction, has gained attention from the scientific community. This research work…

Materials Science · Physics 2025-05-12 Lanna E. B. Lucchetti , Pedro A. S. Autreto , Mauro C. Santos , James M. de Almeida

Using first-principles calculations, we perform a search for high-capacity hydrogen storage media based on individually dispersed calcium atoms on doped or defective carbon nanotubes. We find that up to six H2 molecules can bind to a Ca…

Materials Science · Physics 2009-01-20 Hoonkyung Lee , Jisoon Ihm , Marvin L. Cohen , Steven G. Louie

Electrochemical CO2 reduction reaction (CO2RR) using 2D nanomaterials has emerged as a sophisticated approach to mitigate industrial CO2 emissions. In this work, the potential application of pristine as well as strategically Fe, Co,…

Materials Science · Physics 2025-09-23 Md. Mostaqul Islam , Ahmed Zubair

Two-dimensional (2D) heterostructuring is a versatile methodology for designing nanoarchitecture catalytic systems that allow for reconstruction and modulation of interfaces and electronic structures. However, catalysts with such structures…

We present ab initio calculations on the band structure and density of states of single wall semiconducting carbon nanotubes with high degrees (up to 25%) of B, Si and N substitution. The doping process consists of two phases: different…

Mesoscale and Nanoscale Physics · Physics 2015-01-13 E. Tetik
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