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We show that the relaxation dynamics near a glass transition with continuous ergodicity breaking can be endowed with a geometric interpretation based on percolation theory. At mean-field level this approach is consistent with the…

Statistical Mechanics · Physics 2014-09-05 Jeferson J. Arenzon , Antonio Coniglio , Annalisa Fierro , Mauro Sellitto

In this work, the single-component Cu metallic glass was fabricated by the physical vapor deposition on the Zr (0001) crystal substrate at 100 K using the classical molecular dynamic simulation. The same deposition process was performed on…

Materials Science · Physics 2016-07-21 Yang Yu , Yunyun Chen , Fenping Cui

Glass-to-glass and liquid-to-liquid phase transitions were observed many years ago in bulk and confined water with or without applied pressure. It is shown that they result from the competition of two-liquid phases separated by an enthalpy…

Disordered Systems and Neural Networks · Physics 2017-03-21 Robert F Tournier

To experimentally clarify the changes in structural and dynamic heterogeneities in a metallic glass (MG), Gd65Co35, by rejuvenation with a temperature cycling (cryogenic rejuvenation), high-energy x-ray diffraction (HEXRD), anomalous x-ray…

By systematically investigating the relaxation behavior of a model metallic glass based on the extensive molecular dynamics (MD) simulations combined with the dynamic mechanical spectroscopy method, a pronounced ultra-low temperature peak…

Materials Science · Physics 2020-02-25 B. Wang , L. J. Wang , B. S. Shang , X. Q. Gao , Y. Yang , H. Y. Bai , M. X. Pan , W. H. Wang , P. F. Guan

The immense dependence of the glass transition temperature $T_g$ on molecular weight $M$ is one of the most fundamentally and practically important features of polymer glass formation. Here, we report on molecular dynamics simulation of…

Soft Condensed Matter · Physics 2024-05-30 William F. Drayer , David S. Simmons

We review the recently proposed elastic approach to glass transition. This approach is based on a simple and a physically transparent idea of elastic interactions between local relaxation events in a liquid. Central to this picture is the…

Soft Condensed Matter · Physics 2008-07-25 Kostya Trachenko

We use coherent X-rays to probe the aging dynamics of a metallic glass directly on the atomic level. Contrary to the common assumption of a steady slowing down of the dynamics usually observed in macroscopic studies, we show that the…

Materials Science · Physics 2015-10-23 Zach Evenson , Beatrice Ruta , Simon Hechler , Moritz Stolpe , Eloi Pineda , Isabella Gallino , Ralf Busch

Dynamical heterogeneities -- strong fluctuations near the glass transition -- are believed to be crucial to explain much of the glass transition phenomenology. One possible hypothesis for their origin is that they emerge from soft…

Soft Condensed Matter · Physics 2012-01-10 Karina E. Avila , Horacio E. Castillo , Azita Parsaeian

The enhancement of surface diffusion (DS) over the bulk (DV) in metallic glasses (MGs) is well documented and likely to strongly influence the properties of glasses grown by vapor deposition. Here, we use classical molecular dynamics…

Materials Science · Physics 2021-08-20 Ajay Annamareddy , Yuhui Li , Lian Yu , Paul M. Voyles , Dane Morgan

We investigate multi-component metallic glass systems using a hybrid Molecular Dynamics (MD) and Variance-Constrained Semi-Grand Canonical approach. This method enables us to generate samples with properties consistent with experimental…

Disordered Systems and Neural Networks · Physics 2025-10-10 Filip Kaskosz , Rene Alvarez-Donado , Mikko Alava , Anshul D. S. Parmar , Silvia Bonfanti

Tackling the low-temperature fate of supercooled liquids is challenging due to the immense timescales involved, which prevent equilibration and lead to the operational glass transition. Relating glassy behaviour to an underlying,…

Statistical Mechanics · Physics 2017-08-16 Francesco Turci , C. Patrick Royall , Thomas Speck

The correlations of the free-energy landscape of mean-field spin glasses at different temperatures are investigated, concentrating on models with a first order freezing transition. Using a ``potential function'' we follow the metastable…

Disordered Systems and Neural Networks · Physics 2009-10-30 A. Barrat , S. Franz , G. Parisi

In this work we use molecular simulations to examine methods of controlling mechanical properties of polymeric glass materials such as elastic moduli, mechanical heterogeneity as well as their glass transition temperature. We study filled…

Soft Condensed Matter · Physics 2016-10-13 George J. Papakonstantopoulos , Juan J. de Pablo

We investigate the Johari-Goldstein (JG) $\beta$-relaxation process in a model metallic glass-forming (GF) material (Al90Sm10), previously studied extensively by both frequency-dependent mechanical measurements and simulation studies…

Materials Science · Physics 2021-03-09 Hao Zhang , Xinyi Wang , Hai-Bin Yu , Jack F. Douglas

An equilibrated model glass-forming liquid is studied by mapping successive configurations produced by molecular dynamics simulation onto a time series of inherent structures (local minima in the potential energy). Using this ``inherent…

Soft Condensed Matter · Physics 2012-03-27 Thomas B. Schroeder , Srikanth Sastry , Jeppe C. Dyre , Sharon C. Glotzer

Glass-forming liquids have been extensively studied in recent decades, but there is still no theory that fully describes these systems, and the diversity of treatments is in itself a barrier to understanding. Here we introduce a new simple…

Disordered Systems and Neural Networks · Physics 2011-03-28 Davide Cellai , Andrzej Z. Fima , Aonghus Lawlor , Kenneth A. Dawson

Specific heat and linear thermal expansivity are fundamental thermal dynamics and have been proven as interesting relaxing quantities to investigate in glass transition and glassy state. However, their possibility has much less been…

Soft Condensed Matter · Physics 2021-09-06 Pengfei Zhang , Marco Gandolfi , Francesco Banfi , Christ Glorieux , Liwang Liu

The existence of multiple amorphous states, or polyamorphism, remains one of the most debated phenomena in disordered matter, particularly regarding its microscopic origin and impact on glassy dynamics. Profiting of the enhanced data…

The glassy dynamics in confluent epithelial monolayers is crucial for several biological processes, such as wound healing, embryogenesis, cancer progression, etc. Several experiments have indicated that, unlike particulate systems, the…

Soft Condensed Matter · Physics 2024-07-24 Satyam Pandey , Soumitra Kolya , Padmashree Devendran , Souvik Sadhukhan , Tamal Das , Saroj Kumar Nandi