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We develop a generic strategy and simple numerical models for multi-component metallic glasses for which the swap Monte Carlo algorithm can produce highly stable equilibrium configurations equivalent to experimental systems cooled more than…

Statistical Mechanics · Physics 2020-10-09 Anshul D. S. Parmar , Misaki Ozawa , Ludovic Berthier

Using molecular dynamics computer simulations we investigate how the glass transition and the properties of the resulting glass depend on the cooling rate with which the sample has been quenched. This is done by studying a two component…

Condensed Matter · Physics 2009-10-28 Katharina Vollmayr , Walter Kob , Kurt Binder

The mean-square displacement (MSD) was measured by neutron scattering at various temperatures and pressures for a number of molecular glass-forming liquids. The MSD is invariant along the glass-transition line at the pressure studied, thus…

Soft Condensed Matter · Physics 2012-03-27 K. Niss , C. Dalle-Ferrier , B. Frick , D. Russo , J. Dyre , C. Alba-Simionesco

In this paper we investigate, both analytically and numerically, the emergence of a kinetic glass transition in two different model systems: a uniformly heated granular gas and a molecular fluid with nonlinear drag. Despite the profound…

Soft Condensed Matter · Physics 2024-04-25 A. Patrón , B. Sánchez-Rey , A. Prados

Melting is well understood in terms of the Lindemann criterion, essentially stating that crystalline materials melt when the thermal vibrations of their atoms become such vigorous that they shake themselves free of the binding forces.…

Disordered Systems and Neural Networks · Physics 2023-05-17 P. Lunkenheimer , A. Loidl , B. Riechers , A. Zaccone , K. Samwer

The effect of cyclic loading on relaxation dynamics and mechanical properties of metallic glasses is studied using molecular dynamics simulations. We consider the Kob-Andersen three-dimensional binary mixture rapidly cooled across the glass…

Soft Condensed Matter · Physics 2018-07-09 Nikolai V. Priezjev

We use large-scale molecular dynamics simulations to study the kinetics of the liquid-gas phase separation if the temperature is lowered across the glass transition of the dense phase. We observe a gradual change from phase separated…

Statistical Mechanics · Physics 2011-06-01 Vincent Testard , Ludovic Berthier , Walter Kob

We study theoretically and numerically a family of multi-point dynamic susceptibilities that quantify the strength and characteristic lengthscales of dynamic heterogeneities in glass-forming materials. We use general theoretical arguments…

This review deals with the kinetic and thermodynamic fragility of bulk metallic glass forming liquids. The experimental methods to determine the kinetic fragility, relaxation behavior and thermodynamic functions of undercooled metallic…

Materials Science · Physics 2014-05-12 Ralf Busch , Zach Evenson , Isabella Gallino , Shuai Wei

A model glass is considered with one type of fast ($\beta$-type) of processes, and one type of slow processes ($\alpha$-type). On time-scales where the fast ones are in equilibrium, the slow ones have a dynamics that resembles the one of…

Statistical Mechanics · Physics 2009-11-07 Luca Leuzzi , Theo M. Nieuwenhuizen

Analytical relations for the glass transition temperature, $T_g$, and the crystal melting temperature, $T_m$, are developed on the basis of nonaffine lattice dynamics. The proposed relations explain: (i) the seemingly universal factor of…

Soft Condensed Matter · Physics 2025-03-18 Alessio Zaccone , Konrad Samwer

We applied an efficient methodology to separate vibrational and configurational entropies in bulk metallic glasses by means of molecular dynamics simulation based on a combination of non-equilibrium adiabatic switching and reversible…

Soft Condensed Matter · Physics 2020-07-03 René Alvarez-Donado , Alex Antonelli

Establishing the composition-structure-property relationships for amorphous materials is critical for many important natural and engineering processes, including the dissolution of highly complex volcanic glasses. In this investigation, we…

Materials Science · Physics 2021-08-02 Kai Gong , Elsa Olivetti

Unraveling the structural factors influencing the dynamics of amorphous solids is crucial. While deep learning aids in navigating these complexities, transparency issues persist. Inspired by the successful application of prototype neural…

Soft Condensed Matter · Physics 2024-03-19 Xiao Jiang , Zean Tian , Kenli Li , Wangyu Hu

Control of the crystallization process at the microscopic level makes it possible to generate the nanocrystalline samples with the desired structural and morphological properties, that is of great importance for modern industry. In the…

Materials Science · Physics 2019-03-25 Bulat N. Galimzyanov , Dinar T. Yarullin , Anatolii V. Mokshin

The dynamic structure factor of glassy and liquid glycerol has been measured by inelastic X-ray scattering in the exchanged momentum ($Q$) region $Q$=2$\div$23 nm$^{-1}$ and in the temperature range 80$\div$570 K. Beside the propagating…

Disordered Systems and Neural Networks · Physics 2007-05-23 T. Scopigno , E. Pontecorvo , R. Di Leonardo , M. Krisch , G. Monaco , G. Ruocco , B. Ruzicka , F. Sette

A new relaxation mechanism is shown to arise from overdamped two-level systems above a critical temperature $T^*\approx 5$ K, thus yielding an explanation for experimental observations in dielectric glasses in the temperature range between…

Condensed Matter · Physics 2009-10-22 Peter Neu , Alois Würger

We consider the stationary state of a fluid comprised of inelastic hard spheres or disks under the influence of a random, momentum-conserving external force. Starting from the microscopic description of the dynamics, we derive a nonlinear…

Statistical Mechanics · Physics 2013-02-25 W. T. Kranz , M. Sperl , A. Zippelius

Despite two decades of studies, the formation of metallic glasses, very promising systems for industrial applications, still remains mostly unexplained. This lack of knowledge hinders the search for new systems, still performed with…

Thermodynamics and kinetics are thought to be linked in glass transitions. The quantitative predictions of -relaxation activation barriers provided by the theory of glasses based on random first order transitions are compared with…

Soft Condensed Matter · Physics 2007-05-23 Jacob D. Stevenson , Peter G. Wolynes
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