Related papers: Nonlinear Spectroscopy as a Magnon Breakdown Diagn…
Non-linear magnetization dynamics is essential for the operation of many spintronics devices. For microwave assisted switching of magnetic elements the low field regime is of particular interest. In addition a large number of experiments…
The magnetic excitations of the quasi-2D spin-1/2 Heisenberg antiferromagnet on an anisotropic triangular lattice Cs2CuCl4 are explored throughout the 2D Brillouin zone using inelastic neutron scattering. In the spin liquid phase above the…
Recent studies have shown that the nonlinear optical response of crystalline systems is fundamentally a quantum geometric property. In this work, we propose two-dimensional coherent spectroscopy (2DCS), which measures the nonlinear…
Raman spectroscopy is used to study magnetic excitations in the quasi one dimensional $S=1/2$ quantum spin systems Cu(Qnx)(Cl$_{1-x}$Br$_x$)$_2$. The low energy spectrum is found to be dominated by a two-magnon continuum as expected from…
We study electric field induced two-dimensional coherent nonlinear optical spectroscopy (2DCS) in a Kitaev magnet at finite temperature. We show that 2DCS is susceptible to both types of fractional quasiparticles of this quantum…
Continuum of spin excitations observed in inelastic neutron scattering experiments are often considered as a strong evidence of quantum spin liquid formation. When quantum spin liquid is indeed the ground state of a disorder-free magnetic…
Nonlinear manipulation of nuclear and electron spins is the basis for all advanced methods in magnetic resonance including multidimensional nuclear magnetic and electron spin resonance spectroscopies, magnetic resonance imaging, and in…
We present a new method to model spin-wave excitations in magnetic solids, based on the Liouville-Lanczos approach to time-dependent density functional perturbation theory. This method avoids computationally expensive sums over empty states…
We report on terahertz spectroscopy of quantum spin dynamics in $\alpha$-RuCl$_3$, a system proximate to the Kitaev honeycomb model, as a function of temperature and magnetic field. An extended magnetic continuum develops below the…
Quantum mechanical perturbative expressions for second order dynamical magnetoelectric (ME) susceptibilities have been derived and calculated for a small molecular system using the Hubbard Hamiltonian with SU(2) symmetry breaking in the…
The Kitaev quantum spin liquid (KSL) is a theoretically predicted state of matter whose fractionalized quasiparticles are distinct from bosonic magnons, the fundamental excitation in ordered magnets. The layered honeycomb antiferromagnet…
Searching for Kitaev quantum spin liquid (QSL) is a fascinating and challenging problem. Much effort has been devoted to honeycomb lattice candidates with strong spin-orbit coupling in 5d-electron iridates and 4delectron RuCl3. Recently,…
We explain how gapped quantum spin liquids, both conventional and 'fractonic', may be unambiguously diagnosed experimentally using the technique of multidimensional coherent spectroscopy. 'Conventional' gapped quantum spin liquids (e.g.…
The leading order nonlinear (NL) susceptibility, $\chi_3$, in a paramagnet is negative and diverges as $T \rightarrow 0$. This divergence is destroyed when spins correlate and the NL response provides unique insights into magnetic order.…
For some years Lanczos moments methods have been combined with large-scale shell-model calculations in evaluations of the spectral distributions of certain operators. This technique is of great value because the alternative, a…
The pure Kitaev honeycomb model harbors a quantum spin liquid in zero magnetic fields, while applying finite magnetic fields induces a topological spin liquid with non-Abelian anyonic excitations. This latter phase has been much sought…
We present and benchmark a quantum computing approach to calculate the two-dimensional coherent spectrum (2DCS) of high-spin models. Our approach is based on simulating their real-time dynamics in the presence of several magnetic field…
Magnetic excitation spectra c"(q,w) of YBa2Cu3Oy, La2-xSrxCuO4, La2-y-xNdySrxCuO4 and Nd2-xCexCuO4 are compared with those of model calculations, where q and w are the wave vector and the energy of the excitations. In the model, the…
$^7$Li nuclear magnetic resonance (NMR) and terahertz (THz) spectroscopies are used to probe magnetic excitations and their field dependence in the hyperhoneycomb Kitaev magnet $\beta$-Li$_2$IrO$_3$. Spin-lattice relaxation rate ($1/T_1$)…
We report on magneto-oscillations in differential resistivity of a two-dimensional electron system subject to intense microwave radiation. The period of these oscillations is determined not only by microwave frequency but also by its…