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A coupled oscillator system displays enhanced sensitivity of its saturated steady-state (SS) oscillation frequency to small parameter perturbations near an exceptional point degeneracy (EPD), a property that can be used to realize EPD-based…

Applied Physics · Physics 2026-02-03 Benjamin Bradshaw , Amin Hakimi , Filippo Capolino

We present a model for Desorption Induce by (Multiple) Electronic Transitions (DIET/DIMET) based on potential energy surfaces calculated with the Delta Self-Consistent Field extension of Density Functional Theory. We calculate potential…

Chemical Physics · Physics 2009-11-13 Thomas Olsen , Jeppe Gavnholt , Jakob Schiøtz

We extend ground-state density-functional theory to excited states and provide the theoretical formulation for the widely used $\Delta SCF$ method for calculating excited-state energies and densities. As the electron density alone is…

Chemical Physics · Physics 2024-03-08 Weitao Yang , Paul W. Ayers

The $k\cdot p$ effective mass approximation (EMA) predicts large, nearly size-independent exciton oscillator strengths in quantum confined semiconductors. Yet, experimental reports have concluded that the total oscillator strength of the…

Mesoscale and Nanoscale Physics · Physics 2017-03-06 Yanhao Tang , Mersedeh Saniepay , Chenjia Mi , Rémi Beaulac , John A. McGuire

Exciton Scattering (ES) theory attributes excited electronic states to standing waves in quasi-one-dimensional molecular materials by assuming a quasi-particle picture of optical excitations. The quasi-particle properties at branching…

Chemical Physics · Physics 2016-12-13 Michael J. Catanzaro , Tian Shi , Sergei Tretiak , Vladimir Y. Chernyak

Following our previous work focussing on compounds containing up to 3 non-hydrogen atoms [\emph{J. Chem. Theory Comput.} {\bfseries 14} (2018) 4360--4379], we present here highly-accurate vertical transition energies obtained for 27…

We present a linear-response formulation of density cumulant theory (DCT) that provides a balanced and accurate description of many electronic states simultaneously. In the original DCT formulation, only information about a single…

Chemical Physics · Physics 2018-09-10 Andreas V. Copan , Alexander Yu. Sokolov

We study the excitation spectroscopy of few-electron, parallel coupled double quantum dots (QDs). By applying a finite source drain voltage to a double QD (DQD), the first excited states observed in nonequilibrium charging diagrams can be…

Mesoscale and Nanoscale Physics · Physics 2013-07-01 T. Hatano , Y. Tokura , S. Amaha , T. Kubo , S. Teraoka , S. Tarucha

Quantum calculations are performed for an anion water cluster representing the first hydration shell of the solvated electron in solution. The absorption spectra from the ground state, the instant excited states and the relaxed excited…

Soft Condensed Matter · Physics 2009-11-11 P. O. J. Scherer , Sighart F. Fischer

We study theoretically the noise-assisted quantum exciton (electron) transfer (ET) in bio-complexes consisting of a single-level electron donor and an acceptor which has a complicated internal structure, and is modeled by many electron…

Biological Physics · Physics 2017-09-12 Shmuel Gurvitz , Alexander I. Nesterov , Gennady P. Berman

We examine some excited state energies in the non-unitary integrable quantum field theory obtained from the perturbation of the minimal conformal field theory model $M_{3,5}$ by its operator $\phi_{2,1}$. Using the correspondence of this…

High Energy Physics - Theory · Physics 2011-02-11 R. M. Ellem , V. V. Bazhanov

Thermally activated delayed fluorescence (TADF) emitters consisting of donor and acceptor molecules are potentially highly interesting for electroluminescence (EL) applications. Their strong fluorescence emission is considered to be due to…

While the variational principle for excited-state energies leads to a route to obtaining excited-state densities from time-dependent density functional theory, relatively little attention has been paid to the quality of the resulting…

Chemical Physics · Physics 2025-09-12 Anna Baranova , Neepa T. Maitra

Electron-stimulated desorption (ESD) of cryosorbed molecules on surfaces is a process of relevance to fields as varied as vacuum dynamics in accelerators and astrochemistry. While desorption from such molecular systems induced by keV…

Chemical Physics · Physics 2020-11-05 Rémi Dupuy , Michal Haubner , Bernard Henrist , Jean-Hugues Fillion , Vincent Baglin

A precise determination of the ground state $^{111}$In ($9/2^+$) electron capture to ground state of $^{111}$Cd ($1/2^+$) $Q$ value has been performed utilizing the double Penning trap mass spectrometer, JYFLTRAP. A value of 857.63(17) keV…

The electronic absorption (EA), circular dichroism (ECD), and anisotropy spectra of the L-valine zwitterion and D-glyceraldehyde are calculated by time-dependent density functional theory (TDDFT) with the M06-2X and B3LYP functionals. It is…

Chemical Physics · Physics 2021-01-27 Jie Su , Bingbing Suo , Patrick Cassam-Chenaï

We reexamine $\Delta$CCSD, a state-specific coupled-cluster (CC) with single and double excitations (CCSD) approach that targets excited states through the utilization of non-Aufbau determinants. This methodology is particularly efficient…

Chemical Physics · Physics 2024-06-13 Yann Damour , Anthony Scemama , Denis Jacquemin , Fábris Kossoski , Pierre-François Loos

In this work we propose a chemically-informed data-driven approach to benchmark the approximate density-functional tight-binding (DFTB) excited state (ES) methods that are currently available within the DFTB+ suite. By taking advantage of…

Chemical Physics · Physics 2023-01-02 Andrés I. Bertoni , Cristián G. Sánchez

Excited-state intramolecular proton transfer (ESIPT) is a fundamental photochemical process in which photoexcitation induces proton transfer within a molecule, leading to the formation of a tautomeric excited state. It was observed…

Chemical Physics · Physics 2026-03-03 Alessandro Nicola Nardi , Morgane Vacher

It is known that ensembles of interacting oscillators or qubits can exhibit the phenomenon of quantum synchronization. In this work we consider a set of $N$ identical two-state systems that we call ``harmonic qubits'', because the kinetic…

General Physics · Physics 2025-09-18 L. Gamberale , G. Modanese