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We propose the application of laser cooling to a number of transition-metal atoms, allowing numerous bosonic and fermionic atomic gases to be cooled to ultra-low temperatures. The non-zero electron orbital angular momentum of these atoms…

Atomic Physics · Physics 2020-12-03 Scott Eustice , Kayleigh Cassella , Dan Stamper-Kurn

We measure the complete set of transition frequencies necessary to laser cool and trap MgF molecules. Specifically, we report the frequency of multiple low $J$ transitions of the $X^2\Sigma^+(v^{\prime\prime}=0,1) \rightarrow…

Hyperfine interactions with a nuclear spin environment fundamentally limit the coherence properties of confined electron spins in the solid-state. Here, we show that a quantum interference effect in optical absorption from two electronic…

Mesoscale and Nanoscale Physics · Physics 2012-05-16 Mena Issler , Eric Kessler , Geza Giedke , Susanne Yelin , Ignacio Cirac , Mikhail Lukin , Atac Imamoglu

Precision spectroscopy of atomic systems is an invaluable tool for the advancement of our understanding of fundamental interactions and symmetries. Recently, highly charged ions (HCI) have been proposed for sensitive tests of physics beyond…

YbF has been identified as a molecule that can be used to investigate charge-parity symmetry violations that are beyond the Standard Model of particle physics. Cooling to sub-milli-Kelvin is advantageous for experiments that probe…

Chemical Physics · Physics 2022-12-14 Thomas D. Persinger , Jiande Han , Anh T. Le , Timothy C. Steimle , Michael C. Heaven

We report the electromagnetically-induced-transparency (EIT) cooling of $^{137}\mathrm{Ba}^{+}$ ions with a nuclear spin of $I=3/2$, which are a good candidate of qubits for future large-scale trapped ion quantum computing. EIT cooling of…

Direct laser cooling of molecules has made significant progress in recent years. However, the selective cooling and manipulation of molecules based on their isotopic composition, which is ubiquitous in atomic laser cooling, has not yet been…

We report on magneto-optical trapping of the two fermionic isotopes of atomic titanium, $^{47}$Ti and $^{49}$Ti. Unlike the even mass-number isotopes, which were recently laser cooled, $^{47}$Ti and $^{49}$Ti have nonzero nuclear spins and,…

Algorithmic cooling methods manipulate an open quantum system in order to lower its temperature below that of the environment. We show that significant cooling is achieved on an ensemble of spin-pair systems by exploiting the long-lived…

Only bosonic molecular species have been directly laser cooled to date, primarily due to an abundance of bosonic isotopes in nature and to their simpler hyperfine structure. Fermionic molecules provide new opportunities for ultracold…

Atomic Physics · Physics 2024-08-07 Jinyu Dai , Qi Sun , Benjamin C. Riley , Debayan Mitra , Tanya Zelevinsky

Molecular laser cooling and trapping requires addressing all spontaneous decays to excited vibrational states that occur at the $\gtrsim 10^{-4} - 10^{-5}$ level, which is accomplished by driving repumping transitions out of these states.…

Atomic Physics · Physics 2023-06-06 Nickolas H. Pilgram , Arian Jadbabaie , Chandler J. Conn , Nicholas R. Hutzler

We investigated the optical cycling effect of the $\mathrm{X}^2\Sigma(v=0,\ N=1^-) - \mathrm{A}^2\Pi_{1/2}(v'=0,\ J'=1/2^+)$ band of MgF molecules, specifically the $\mathrm{P_1/Q_{12}(1)}$ transition, which serves as the main transition in…

Atomic and Molecular Clusters · Physics 2025-07-08 Kikyeong Kwon , Seunghwan Roh , Youngju Cho , Yongwoong Lee , Eunmi Chae

Optical cycling transitions and direct laser cooling have recently been demonstrated for a number of alkaline-earth dimers and trimer molecules. This is made possible by diagonal Franck-Condon factors between the vibrational modes of the…

Chemical Physics · Physics 2020-04-08 Jacek Kłos , Svetlana Kotochigova

We demonstrate a quasi optical cycling for the $X(v=0)\to A(v'=0)$ transition and a radiative force induced deflection on the buffer-gas cooled BaF molecular beam. The laser induced fluorescence enhancement with additional sidebands and a…

Atomic Physics · Physics 2017-11-15 Tao Chen , Wenhao Bu , Bo Yan

We demonstrate buffer-gas cooling, high-resolution spectroscopy and cycling fluorescence of cold barium monofluoride (BaF) molecules. Our source produces an intense and internally cold molecular beam containing the different BaF…

Atomic Physics · Physics 2020-01-13 Ralf Albrecht , Michael Scharwaechter , Tobias Sixt , Lucas Hofer , Tim Langen

We propose a method for laser cooling group-II-like atoms without changing the quantum state of their nuclear spins, thus preserving coherences that are usually destroyed by optical pumping. As group-II-like atoms have a $^1S_0$…

Quantum Physics · Physics 2009-11-13 Iris Reichenbach , Ivan H. Deutsch

It has been roughly three decades since laser cooling techniques produced ultracold atoms, leading to rapid advances in a vast array of fields. Unfortunately laser cooling has not yet been extended to molecules because of their complex…

Atomic Physics · Physics 2015-05-27 E. S. Shuman , J. F. Barry , D. DeMille

A {\gamma}-ray linear polarization measurement has been performed to directly determine the parities for the levels in 146Gd nucleus. High-spin states in this nucleus were populated in a reaction 115In + 34S at 140 MeV incident energy.…

Rapid and repeated photon cycling has enabled precision metrology and the development of quantum information systems using a variety of atoms and simple molecules. Extending optical cycling to structurally complex molecules would provide…

We investigate the prospect of using ultracold alkali diatomic molecules to implement many-body quantum systems with SU($N$) symmetry. Experimentally accessible molecules offer large $N$ for both bosonic and fermionic systems, with both…

Quantum Physics · Physics 2025-02-04 Bijit Mukherjee , Jeremy M. Hutson