English

Algorithmic Cooling of Nuclear Spin Pairs using a Long-Lived Singlet State

Quantum Physics 2020-05-20 v1 Applied Physics Chemical Physics

Abstract

Algorithmic cooling methods manipulate an open quantum system in order to lower its temperature below that of the environment. We show that significant cooling is achieved on an ensemble of spin-pair systems by exploiting the long-lived nuclear singlet state, which is an antisymmetric quantum superposition of the "up" and "down" qubit states. The effect is demonstrated by nuclear magnetic resonance (NMR) experiments on a molecular system containing a coupled pair of near-equivalent 13C nuclei. The populations of the system are subjected to a repeating sequence of cyclic permutations separated by relaxation intervals. The long-lived nuclear singlet order is pumped well beyond the unitary limit, and the nuclear magnetization is enhanced by 21% relative to its thermal equilibrium value. To our knowledge this is the first demonstration of algorithmic cooling using a quantum superposition state and without making a distinction between rapidly and slowly relaxing qubits.

Keywords

Cite

@article{arxiv.1912.13246,
  title  = {Algorithmic Cooling of Nuclear Spin Pairs using a Long-Lived Singlet State},
  author = {Bogdan A. Rodin and Christian Bengs and Lynda J. Brown and Kirill F. Sheberstov and Alexey S. Kiryutin and Richard C. D. Brown and Alexandra V. Yurkovskaya and Konstantin L. Ivanov and Malcolm H. Levitt},
  journal= {arXiv preprint arXiv:1912.13246},
  year   = {2020}
}

Comments

22 pages, 6 figures

R2 v1 2026-06-23T12:59:38.588Z