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On a lattice composed of triangular plaquettes where antiferromagnetic exchange interactions between localized spins cannot be simultaneously satisfied, the system becomes geometrically frustrated with magnetically disordered phases…

Crystal structure and thermodynamic properties of Na$_2$SrCo(PO$_4$)$_2$, the chemical sibling of the triangular quantum spin-liquid candidate Na$_2$BaCo(PO$_4$)$_2$, are reported. From single crystal x-ray diffraction and high-resolution…

Strongly Correlated Electrons · Physics 2022-08-12 Vera P. Bader , Jan Langmann , Philipp Gegenwart , Alexander A. Tsirlin

Quantum spin liquids (QSLs) are topologically ordered exotic states of matter that host fractionalized excitations. Kitaev proposed a particular route towards a QSL via strongly bond-dependent interactions on the hexagonal lattice. A number…

Strongly Correlated Electrons · Physics 2022-12-06 Xinshu Zhang , Yuanyuan Xu , T. Halloran , Ruidan Zhong , R. J. Cava , C. Broholm , N. Drichko , N. P. Armitage

The quantum spin liquid (QSL) state is an exotic state of matter featuring a high degree of entanglement and lack of long-range magnetic order in the zero-temperature limit. The triangular antiferromagnet YbMgGaO4 is a candidate QSL host,…

Kitaev quantum spin liquid, massively quantum entangled states, is so scarce in nature that searching for new candidate systems remains a great challenge. Honeycomb heterostructure could be a promising route to realize and utilize such an…

A quantum spin liquid (QSL) is a state of matter in which magnetic spins interact strongly, but quantum fluctuations inhibit long-range magnetic order even at zero temperature. A QSL has been predicted to have a host of exotic properties,…

Quantum materials exhibiting magnetic frustration are connected to diverse phenomena including high-Tc superconductivity, topological order and quantum spin liquids (QSLs). A QSL is a quantum phase (QP) related to a quantum-entangled…

Strongly Correlated Electrons · Physics 2021-08-03 Samuel Mañas-Valero , Benjamin Huddart , Tom Lancaster , Eugenio Coronado , Francis Pratt

The molecular triangular lattice system, beta'-EtMe3Sb[Pd(dmit)2]2, is considered as a candidate material for the quantum spin liquid (QSL) state, although ongoing debates arise from recent controversial results. Here, the results of…

Strongly Correlated Electrons · Physics 2024-12-05 Yugo Oshima , Yasuyuki Ishii , Francis L. Pratt , Isao Watanabe , Hitoshi Seo , Takao Tsumuraya , Tsuyoshi Miyazaki , Reizo Kato

Quantum spin liquids (QSL) have generated considerable excitement as phases of matter with emergent gauge structures and fractionalized excitations. In this context, phase transitions out of QSLs have been widely discussed as Higgs…

Strongly Correlated Electrons · Physics 2021-09-15 Hyeok-Jun Yang , Nic Shannon , SungBin Lee

The most fascinating feature of certain two-dimensional (2D) gapless quantum spin liquid (QSL) is that their spinon excitations behave like the fermionic carriers of a paramagnetic metal. The spinon Fermi surface is then expected to produce…

Strongly Correlated Electrons · Physics 2020-09-17 N. Li , Q. Huang , X. Y. Yue , W. J. Chu , Q. Chen , E. S. Choi , X. Zhao , H. D. Zhou , X. F. Sun

Quantum spin liquid (QSL) phases exist in theory, but real candidate QSL materials are often extraordinarily sensitive to structural defects which disrupt the ground state. Here, we investigate candidate triangular QSL material…

We demonstrate that the insulating one-band Hubbard model on the pyrochlore lattice contains, for realistic parameters, an extended quantum spin-liquid phase. This is a three-dimensional spin liquid formed from a highly degenerate manifold…

Strongly Correlated Electrons · Physics 2014-05-28 B. Normand , Z. Nussinov

Symmetry plays a fundamental role in our understanding of both conventional symmetry breaking phases and the more exotic quantum and topological phases of matter. We explore the experimental signatures of symmetry enriched U(1) quantum spin…

Strongly Correlated Electrons · Physics 2017-01-25 Yao Dong Li , Gang Chen

Recent excitement in the quantum spin ice community has come from the experimental discovery of pseudospin-$1/2$ breathing pyrochlores, including Ba$_3$Yb$_2$Zn$_5$O$_{11}$, in which inversion symmetry is broken by the `up' and `down'…

Strongly Correlated Electrons · Physics 2024-05-14 Alaric Sanders , Claudio Castelnovo

The dipolar-octupolar pyrochlore oxides R$_2$M$_2$O$_7$ (R=Ce, Sm, Nd) represent an important opportunity in the search for three dimensional Quantum Spin Liquid (QSL) ground states. Their low energy physics is governed by an alluringly…

Strongly Correlated Electrons · Physics 2020-09-15 Owen Benton

A quantum spin liquid (QSL) arises from a highly entangled superposition of many degenerate classical ground states in a frustrated magnet, and is characterized by emergent gauge fields and deconfined fractionalized excitations (spinons).…

Strongly Correlated Electrons · Physics 2025-06-24 Bin Gao , Félix Desrochers , David W. Tam , Paul Steffens , Arno Hiess , Yixi Su , Sang-Wook Cheong , Yong Baek Kim , Pengcheng Dai

Beyond the conventional electron pairing mediated by phonons, high-temperature superconductivity in cuprates is believed to stem from quantum spin liquid (QSL). The unconventional superconductivity by doping a spin liquid/Mott insulator, is…

The quasi-2D Shastry-Sutherland model has remained topical in the field of condensed matter physics for the last two decades, following the experimental realization of the model in the material SrCu$_2$(BO$_3$)$_2$. Since then, research…

Strongly Correlated Electrons · Physics 2024-07-11 M. Pula , S. Sharma , J. Gautreau , Sajilesh K. P. , A. Kanigel , M. D. Frontzek , T. N. Dolling , L. Clark , S. Dunsiger , A. Ghara , G. M. Luke

The search for Kitaev's quantum spin liquid (KQSL) state in real materials has recently expanded with the prediction that honeycomb lattices of divalent, high-spin cobalt ions could host the dominant bond-dependent exchange interactions…

Organic solids host various electronic phases. Especially, a milestone compound of organic solid, $\beta'$-$X$[Pd(dmit)$_2$]$_2$ with $X$=EtMe$_3$Sb shows quantum spin-liquid (QSL) properties suggesting a novel state of matter. However,…

Strongly Correlated Electrons · Physics 2022-04-29 Kota Ido , Kazuyoshi Yoshimi , Takahiro Misawa , Masatoshi Imada