Related papers: Pyrochlore NaYbO2: A potential Quantum Spin Liquid…
A quantum spin liquid is an exotic quantum state of matter in which spins are highly entangled and remain disordered down to zero temperature. Such a state of matter is potentially relevant to high-temperature superconductivity and…
Quantum spin liquids (QSLs) form an extremely unusual magnetic state in which the spins are highly correlated and fluctuate coherently down to the lowest temperatures, but without symmetry breaking and without the formation of any static…
The ground states of the frustrated pyrochlore oxide Tb$_{2+x}$Ti$_{2-x}$O$_{7+y}$ have been studied by inelastic neutron scattering experiments. Three single-crystal samples are investigated; one shows no phase transition…
Quantum fluctuations enhanced by frustration and subtle interplay between competing degrees of freedom offer an ideal ground to realize novel states with fractional quantum numbers in quantum materials that defy standard theoretical…
Metallization of quantum spin liquid (QSL) materials has long been considered as a potential route to achieve unconventional superconductivity. Here we report our endeavor in this direction by pressurizing a three-dimensional QSL candidate,…
The synthesis and characterization of a new Yb-based material Ba3Yb2Zn5O11 are reported. This material is identified as the first model system of a pseudospin-1/2 quantum antiferromagnet on "breathing" pyrochlore lattice characterized by an…
Quantum spin liquid (QSL) is a novel state of matter which refuses the conventional spin freezing even at 0 K. Experimentally searching for the structurally perfect candidates is a big challenge in condensed matter physics. Here we report…
Quantum spin liquids (QSLs) are exotic states of matter characterized by emergent gauge structures and fractionalized elementary excitations. The recently discovered triangular lattice antiferromagnet YbMgGaO$_4$ is a promising QSL…
YbMgGaO$_{4}$, a structurally perfect two-dimensional triangular lattice with odd number of electrons per unit cell and spin-orbit entangled effective spin-1/2 local moments of Yb$^{3+}$ ions, is likely to experimentally realize the quantum…
The quantum spin liquid (QSL) is an exotic phase of magnetic materials where the spins continue to fluctuate without any symmetry breaking down to zero temperature. Among the handful reports of QSL with spin $S\ge$1, examples with magnetic…
Quantum spin liquids (QSL) are theoretical states of matter with long-range entanglement and exotic quasiparticles. However, they generally elude quantitative theory, rendering their underlying phases mysterious and hampering efforts to…
Based on the recent experiments on the triangular lattice antiferromagnet Na$_2$BaCo(PO$_4$)$_2$, we propose the easy-axis XXZ spin-1/2 model on the triangular lattice, that exhibits a quantum spin supersolid, to be a precursory Dirac spin…
One main theme in current condensed matter physics is the search of quantum spin liquid (QSL), an exotic magnetic state with strongly-fluctuating and highly-entangled spins down to zero temperature without static order. However, there is no…
Quantum spin liquid (QSL) is a novel state of matter with exotic excitations and was theoretically predicted to be realized most possibly in an S=1/2 kagome antiferromagnet. Experimentally searching for the candidate materials is a big…
Yb-based magnets, with a perfect triangular lattice of pseudospin-$1/2$ Yb$^{3+}$ ions, have emerged as candidates for realizing a quantum spin-liquid state, with NaYbS$_2$ being a prominent example. Here we present the solid-solution…
The Ce$^{3+}$ pseudospin-$\frac{1}{2}$ degrees of freedom in the pyrochlore magnet Ce$_2$Zr$_2$O$_7$ are known to possess dipole-octupole (DO) character, making it a candidate for novel quantum spin liquid (QSL) ground states at low…
The quantum pyrochlore antiferromagnet is studied by perturbative expansions and exact diagonalization of small clusters. We find that the ground state is a spin-liquid state: The spin-spin correlation functions decay exponentially with…
Geometrical frustration among interacting spins combined with strong quantum fluctuations destabilize long-range magnetic order in favour of more exotic states such as spin liquids. By following this guiding principle, a number of spin…
The Mott transition is one of the fundamental issues in condensed matter physics, especially in the system with antiferromagnetic long-range order. However the Mott transition in quantum spin liquid (QSL) systems without long-range order is…
Antiferromagnetically coupled S=1/2 spins on an isotropic triangular lattice is the paradigm of frustrated quantum magnetism, but structurally ideal realizations are rare. Here we investigate NaYbO$_2$, which hosts an ideal triangular…