Related papers: Chemistry in a Cryogenic Buffer Gas Cell
The design and performance of a cryogenic buffer gas beam (CBGB) source with a load-lock system is presented. The ACME III electron electric dipole moment (eEDM) search experiment uses this source to produce a beam of cold, slow thorium…
At low temperatures, the main coolant in primordial gas is molecular hydrogen, H2. Recent work has shown that primordial gas that is not collapsing gravitationally but is cooling from an initially ionized state forms hydrogen deuteride, HD,…
The reactions of cold H atoms with solid O2 molecules were investigated at 10 K. The formation of H2O2 and H2O has been confirmed by in-situ infrared spectroscopy. We found that the reaction proceeds very efficiently and obtained the…
The interactions of atomic and molecular hydrogen with bare interstellar dust grain surfaces are important for understanding H2 formation at relatively high temperatures (>20 K). We investigate the diffusion of physisorbed H atoms and the…
Here we report the results of an experimental and theoretical study of the gas-phase reactions between O($^1$D) and H$_2$O and O($^1$D) and D$_2$O at room temperature and below. On the experimental side, the kinetics of these reactions have…
We describe a helium source cell for use in cryogenic experiments that is hermetically sealed $in$ $situ$ on the cold plate of a cryostat. The source cell is filled with helium gas at room temperature and subsequently sealed using a cold…
We present a CSO and BIMA molecular line survey of the dense, quiescent molecular environment ahead of HH2. The molecular gas is cold, 13 K, and moderately dense, 3x10^5 cm^-3. A total of 14 species has been detected (including different…
A method for calibration of cryogenic liquid argon detector response to recoils with certain energy -8.2 keV - is proposed. The method utilizes a process of inelastic scattering of monoenergetic neutrons produced by fusion DD neutron…
We introduce a method for classical trajectory calculations to simulate collisions between atoms and large rigid asymmetric-top molecules. Using this method, we investigate the formation of molecule-helium complexes in buffer-gas cooling…
Ultracold molecules represent a fascinating research frontier in physics and chemistry, but it has proven challenging to prepare dense samples at low velocities. Here we present a solution to this goal by a non-conventional approach dubbed…
We investigate the role of non-thermal electrons in the formation regions of Halpha, Hbeta, and Hgamma lines in order to unfold their influence on the formation of these lines. We concentrate on pulse-beam heating varying on a subsecond…
The bulk of the molecular component in galaxies is made of cold H2, which is not observed directly, but which abundance is derived from indirect tracers such as CO emission. The CO to H2 conversion ratio remains uncertain, and may vary by…
This work is concerned with the theoretical study of nuclear reactions between light charged ions at incident energies around and below the reactants Coulomb barrier, with a focus on the energy range of astrophysical interest for Big Bang…
We present a rigorous theoretical study of low-temperature collisions of polyatomic molecular radicals with ^1S_0 atoms in the presence of an external magnetic field. Accurate quantum scattering calculations based on ab initio and scaled…
We argue that hadron multiplicities in central high energy nucleus-nucleus collisions are established very close to the phase boundary between hadronic and quark matter. In the hadronic picture this can be described by multi-particle…
Because chemical reactions on/in cosmic ice dust grains covered by amorphous solid water (ASW) play important roles in generating a variety of molecules, many experimental and theoretical studies have focused on the chemical processes…
We demonstrate a novel method to determine the longitudinal phase-space distribution of a cryogenic buffer gas beam of barium-fluoride molecules based on a two-step laser excitation scheme. The spatial resolution is achieved by a…
We demonstrate remarkably enhanced yield of C60 fullerenes in an aerosol discharge chamber due to the additional presence of a strong spatial temperature gradient. The role of the temperature gradients in the increased yield of C60 and…
This paper presents one of the case studies of the Gamma Factory initiative -- a proposal of a new operation scheme of ion beams in the CERN accelerator complex. Its goal is to extend the scope and precision of the LHC-based research by…
We measure chemical reactions between a single trapped $^{174}$Yb$^+$ ion immersed in an ultracold bath of $^6$Li atoms containing trace amounts of Li$_2$ dimers. This produces LiYb$^+$ molecular ions that we detect via mass spectrometry.…