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The oxidation and spin state of a metal-organic molecule determine its chemical reactivity and magnetic properties. Here, we demonstrate the reversible control of the oxidation and spin state in a single Fe-porphyrin molecule in the force…

Mesoscale and Nanoscale Physics · Physics 2018-04-09 Benjamin W. Heinrich , Christopher Ehlert , Nino Hatter , Lukas Braun , Christian Lotze , Peter Saalfrank , Katharina J. Franke

Fe3Si is a ferromagnetic material with possible applications in magnetic tunnel junctions. When doped with Mn, the material shows a complex magnetic behavior, as suggested by older experiments. We employed the Korringa-Kohn-Rostoker (KKR)…

Materials Science · Physics 2016-08-14 Marjana Ležaić , Phivos Mavropoulos , Stefan Blügel , Hubert Ebert

We study theoretically the spin dynamics of the ferric wheel, an antiferromagnetic molecular ring. For a single nuclear or impurity spin coupled to one of the electron spins of the ring, we calculate nuclear and electronic spin correlation…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Florian Meier , Daniel Loss

The design and control of atomic-scale spin structures constitute major challenges for spin-based quantum technology platforms, including quantum dots, color centers, and molecular spins. Here, we showcase a strategy for designing the…

We derive the spin-atomic vibration interaction $V_{\rm SA}$ and the spin-flip Hamiltonian $V_{\rm SF}$ of a single atomic spin in a crystal field. We here apply the perturbation theory to a model with the spin-orbit interaction and the…

Mesoscale and Nanoscale Physics · Physics 2010-11-11 Satoshi Kokado , Kikuo Harigaya , Akimasa Sakuma

A systematic microscopic theory of magnetically induced ferroelectricity and lattice modulation is presented for all electron configurations of Mott-insulating transition-metal oxides. Various mechanisms of polarization are identified in…

Strongly Correlated Electrons · Physics 2009-11-13 Chenglong Jia , Shigeki Onoda , Naoto Nagaosa , Jung Hoon Han

We propose an experimental scheme to study spin-orbit coupling effects in a of two-dimensional (2D) Fermi atomic gas cloud by coupling its internal electronic states (pseudospins) to radiation in a delta configuration. The induced…

Statistical Mechanics · Physics 2009-11-13 Xiong-Jun Liu , Mario F. Borunda , Xin Liu , Jairo Sinova

We study the magnetic interactions in atomic layers of Fe and 5d transition-metals such as Os, Ir, and Pt on the (001) surface of Rh using first-principles calculations based on density functional theory. For both stackings of the 5d-Fe…

Materials Science · Physics 2017-10-11 Sebastian Meyer , Bertrand Dupé , Paolo Ferriani , Stefan Heinze

The preferred spin orientation of a magnetic ion can be predicted on the basis of density functional theory (DFT) calculations including electron correlation and spin-orbit coupling (SOC). However, most chemists and physicists are unaware…

Strongly Correlated Electrons · Physics 2015-12-31 Myung-Hwan Whangbo , Elijah E. Gordon , Hongjun Xiang , Hyun-Joo Koo , Changhoon Lee

Proposals for novel spin-orbitronic logic1 and memory devices2 are often predicated on assumptions as to how materials with large spin-orbit coupling interact with ferromagnets when in contact. Such interactions give rise to a host of novel…

Mesoscale and Nanoscale Physics · Physics 2015-08-05 Hans T. Nembach , Justin M. Shaw , Mathias Weiler , Emilie Jué , Thomas J. Silva

We study the physics of dilute magnetic impurities in a two-dimensional altermagnetic metal. For the single impurity case, although the spin degeneracy is broken in an altermagnetic metal, we show that the antiferromagnetic Kondo coupling…

Strongly Correlated Electrons · Physics 2025-03-10 Yu-Li Lee

The kagome lattice, whose electronic valence band (VB) structure includes two Dirac bands and one flat band, offers a rich space to realise tuneable topological and strongly correlated electronic phases in two-dimensional (2D) and layered…

Strongly Correlated Electrons · Physics 2021-09-16 Dhaneesh Kumar , Jack Hellerstedt , Bernard Field , Benjamin Lowe , Yuefeng Yin , Nikhil V. Medhekar , Agustin Schiffrin

The effects of nuclear field and spin-orbit interaction on dense coding and swap operation are studied in detail for both the antiferromagnetic (AFM) and ferromagnetic (FM) coupling cases. The conditions for a valid dense coding and under…

Quantum Physics · Physics 2017-02-16 Li Jiang , Guo-Feng Zhang

Magnetic and electronic structures in LaFeAsO in the single-stripe-type antiferromagnetic (AFM) phase are studied using first-principles density-functional calculations including the spin-orbit interaction. We show that the longitudinal…

Superconductivity · Physics 2016-12-28 Sehoon Oh , Jung-Hoon Lee , Hyun Myung Jang , Hyoung Joon Choi

Based on first-principles density-functional theory calculations we investigate the electronic structure of hexanuclear "ferric wheels" M Fe_6[N(CH_2 CH_2 O)_3]_6 Cl (M = Li, Na) in their antiferromagnetic ground state. The electronic…

Materials Science · Physics 2007-05-23 A. V. Postnikov , Jens Kortus , Stefan Bluegel

Exchange couplings are fundamental to our understanding of many physical phenomena in condensed matter physics and material science. Model systems provide a controlled environment to investigate such phenomena, effectively. In this study,…

Materials Science · Physics 2024-11-26 Mahnaz Rezaei , Jahanfar Abouie , Fariba Nazari

We consider eigenmodes of a ring resonator made of a circular dielectric waveguide. Taking into account the polarization corrections, which are responsible for the interaction of polarization and orbital properties of electromagnetic waves…

Optics · Physics 2007-05-23 K. Yu. Bliokh , D. Yu. Frolov

Macroscopic assemblies of interacting spins give rise to a broad spectrum of behaviors determined by the spatial arrangement of the magnetic sites and the electronic interactions between them. Compounds of copper (II), in which each copper…

Strongly Correlated Electrons · Physics 2021-04-22 Pavel Pokhilko , Dmitry S. Bezrukov , Anna I. Krylov

We study theoretically the structure of double pionic atoms, in which two negatively charged pions ($\pi^-$) are bound in the atomic orbits. The double pionic atom is considered to be an interesting system from the point of view of the…

We present an ab-initio-based effective interaction model (EIM) for the study of magnetism, thermodynamics, and their interplay in body-centered cubic Fe-Co alloys, with Co content from 0 to 70%. The model includes explicitly both spin and…

Materials Science · Physics 2020-01-16 Van-Truong Tran , Chu-Chun Fu , Anton Schneider