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Entangled photon sources (EPSs) are essential building blocks for scalable quantum communication and quantum key distribution (QKD). We present a stable, highly nondegenerate EPS based on type-0 spontaneous parametric down-conversion (SPDC)…

This study presents a refined approach to computing the electronic structure of indium antimonide (InSb) using advanced \textit{ab initio} techniques with the In and Sb $4d^{10}$ semicore electrons included in the valence states. These…

Materials Science · Physics 2025-08-04 Ritwik Das , Anne-Sophie Grimault-Jacquin , Frédéric Aniel

We studied optical coherence properties of the 1.53 $\mu$m telecommunication transition in an Er$^{3+}$-doped silicate optical fiber through spectral holeburning and photon echoes. We find decoherence times of up to 3.8 $\mu$s at a magnetic…

The highly efficient photocatalytic water splitting to produce clean energy requires novel semiconductor materials to achieve high solar-to-hydrogen energy conversion efficiency. Herein, the photocatalytic properties of anisotropic…

Materials Science · Physics 2023-05-22 Pooja Jamdagni , Ashok Kumar , Sunita Srivastava , Ravindra Pandey , K. Tankeshwar

Epitaxially-grown semiconductor quantum dots (QDs) provide an attractive platform for the development of deterministic sources of high-quality quantum states of light. Such non-classical light sources are essential for quantum information…

Mesoscale and Nanoscale Physics · Physics 2023-08-30 Lucie Leguay , Abhiroop Chellu , Joonas Hilska , Esperanza Luna , Andrei Schliwa , Mircea Guina , Teemu Hakkarainen

We propose an entanglement beam splitter (EBS) using a quantum-dot spin in a double-sided optical microcavity. In contrast to the conventional optical beam splitter, the EBS can directly split a photon-spin product state into two…

Quantum Physics · Physics 2010-01-11 C. Y. Hu , W. J. Munro , J. L. O'Brien , J. G. Rarity

In the framework of four-band envelope-function formalism, developed earlier for spherical semiconductor nanocrystals, we study the electronic structure and optical properties of quantum-confined lead-salt (PbSe and PbS) nanowires (NWs)…

Materials Science · Physics 2015-05-13 Valery I. Rupasov

We investigate the properties of electronic states and optical transitions in hexagonal GaAs quantum dots within AlGaAs nanowires. Such dots are particularly interesting due to their high degree of symmetry. A streamlined postsymmetrization…

Mesoscale and Nanoscale Physics · Physics 2015-11-18 Guro K. Svendsen , Johannes Skaar , Helge Weman , Marc-André Dupertuis

We present a novel "linear combination of atomic orbitals"-type of approximation, enabling accurate electronic structure calculations for systems of up to 20 or more electronically coupled quantum dots. Using realistic single quantum dot…

Mesoscale and Nanoscale Physics · Physics 2021-03-10 Alexander Mittelstädt , Ludwig A. Th. Greif , Stefan T. Jagsch , Andrei Schliwa

Energy states below the bandgap of a semiconductor, such as trap states or charge transfer states in organic donor acceptor blends, can contribute to light absorption. Due to their low number density or ultrasmall absorption cross-section,…

Applied Physics · Physics 2019-11-27 Christina Kaiser , Stefan Zeiske , Paul Meredith , Ardalan Armin

This study analyzed the optical techniques for high resolution, low-noise spectroscopy of a hyperfine structure (HFS) made of ytterbium-isotope 171 ions ($^{171}\mathrm{Yb}^{3+}$:$\mathrm{Y}_2\mathrm{SiO}_5$). Large energy spacings in…

Optics · Physics 2024-08-21 Hee-Jin Lim , Ga-Hyun Choi , Ki Suk Hong

Halide perovskites (HPs) are widely viewed as promising photovoltaic and light-emitting materials for their suitable band gaps in the visible spectrum. Density functional theory (DFT) calculations employing (semi)local exchange-correlation…

Materials Science · Physics 2022-12-06 Jiyuan Yang , Tianyuan Zhu , Shi Liu

Here, the structural, electronic and optical properties of the GaP1-xSbx/Si tandem materials association are determined in view of its use for solar water splitting applications. The GaPSb crystalline layer is grown on Si by Molecular Beam…

We present a first-principles study of the structural, electronic, and optical properties of hydrogenated amorphous silicon (a-Si:H). To this end, atomic configurations of a-Si:H with 72 and 576 atoms respectively are generated using…

Materials Science · Physics 2017-03-31 Philippe Czaja , Urs Aeberhard , Massimo Celino , Simone Giusepponi , Michele Gusso

We report artifact-free CH3NH3PbI3 optical constants extracted from ultra-smooth perovskite layers without air exposure and assign all the optical transitions in the visible/ultraviolet region unambiguously based on density functional…

We study theoretically the performance of electrically pumped self-organized quantum dots as a gain material in the mid-IR range at room temperature. We analyze an AlGaAs/InGaAs based structure composed of dots-in-a-well sandwiched between…

Materials Science · Physics 2014-10-27 Stephan Michael , Weng W. Chow , Hans Christian Schneider

In this work, the structural, electrical, and optical properties of bilayer SiX (X= N, P, As, and Sb) are studied using density functional theory (DFT). Five different stacking orders are considered for every compound and their structural…

Materials Science · Physics 2021-07-07 Nayereh Ghobadi , Shoeib Babaee Touski

Qubits encoded in hyperfine states of trapped ions are ideal for quantum computation given their long lifetimes and low sensitivity to magnetic fields, yet they suffer from off-resonant scattering during detection often limiting their…

Quantum Physics · Physics 2021-07-28 C. L. Edmunds , T. R. Tan , A. R. Milne , A. Singh , M. J. Biercuk , C. Hempel

Two-dimensional (2D) Pb nanoisland has established an ideal platform for studying the quantum size effects on growth mechanism, electronic structures as well as high-temperature superconductivity. Here, we investigate the growth and quantum…

Materials Science · Physics 2020-10-28 Guan-Yu Chen , Chia-Hsiu Hsu , Bo-You Liu , Li-Wei Chang , Deng-Sung Lin , Feng-Chuan Chuang , Pin-Jui Hsu

The Si/SiGe heterosystem would be ideally suited for the realization of complementary metal-oxide-semiconductor (CMOS)-compatible integrated light sources, but the indirect band gap, exacerbated by a type-II band offset, makes it…