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This paper investigates the identifiability and estimation of the parameters of the single particle model (SPM) for lithium-ion battery simulation. Identifiability is addressed both in principle and in practice. The approach begins by…

Systems and Control · Computer Science 2018-10-03 Adrien M. Bizeray , Jin-Ho Kim , Stephen R. Duncan , David A. Howey

In this work we analyse the local nonlinear electrochemical impedance spectroscopy (NLEIS) response of a lithium-ion battery and estimate model parameters from measured NLEIS data. The analysis assumes a single-particle model including…

Chemical Physics · Physics 2023-04-24 T. L. Kirk , A. Lewis-Douglas , D. A. Howey , C. P. Please , S. J. Chapman

Advanced battery management systems rely on mathematical models to guarantee optimal functioning of Lithium-ion batteries. The Pseudo-Two Dimensional (P2D) model is a very detailed electrochemical model suitable for simulations. On the…

Systems and Control · Computer Science 2019-10-01 Andrea Pozzi , Gabriele Ciaramella , Stefan Volkwein , Davide M. Raimondo

This paper presents a Bayesian parameter estimation approach and identifiability analysis for a lithium-ion battery model, to determine the uniqueness, evaluate the sensitivity and quantify the uncertainty of a subset of the model…

Systems and Control · Electrical Eng. & Systems 2023-09-04 Antti Aitio , Scott G. Marquis , Pedro Ascencio , David Howey

Physics-based electrochemical battery models derived from porous electrode theory are a very powerful tool for understanding lithium-ion batteries, as well as for improving their design and management. Different model fidelity, and thus…

Growing demand for fast charging and optimised battery designs is fuelling significant interest in electrochemical models of Li-ion batteries. However, estimating parameter values for these models remains a major challenge. In this paper, a…

Systems and Control · Electrical Eng. & Systems 2020-12-04 Ross Drummond , Stephen R. Duncan

Battery short-term electrical impedance behavior varies between linear, linear time-varying, or nonlinear at different operating conditions. Data-based electrical impedance modeling techniques often model the battery as a linear…

Systems and Control · Computer Science 2018-05-17 Rishi Relan , Koen Tiels , Jean-Marc Timmermans , Johan Schoukens

To plan and optimize energy storage demands that account for Li-ion battery aging dynamics, techniques need to be developed to diagnose battery internal states accurately and rapidly. This study seeks to reduce the computational resources…

Lithium-ion batteries are widely used in transportation, energy storage, and consumer electronics, driving the need for reliable battery management systems (BMS) for state estimation and control. The Single Particle Model (SPM) balances…

Systems and Control · Electrical Eng. & Systems 2025-05-28 Feng Guo , Luis D. Couto

The Python Battery Optimisation and Parameterisation (PyBOP) package provides methods for estimating and optimising battery model parameters, offering both deterministic and stochastic approaches with example workflows to assist users.…

Systems and Control · Electrical Eng. & Systems 2026-01-16 Brady Planden , Nicola E. Courtier , Martin Robinson , Agriya Khetarpal , Ferran Brosa Planella , David A. Howey

Efficient parameter identification of electrochemical models is crucial for accurate monitoring and control of lithium-ion cells. This process becomes challenging when applied to complex models that rely on a considerable number of…

Systems and Control · Electrical Eng. & Systems 2024-05-20 Jianzong Pi , Samuel Filgueira da Silva , Mehmet Fatih Ozkan , Abhishek Gupta , Marcello Canova

The impedance of a Li-ion battery contains information about its state of charge (SOC), state of health (SOH) and remaining useful life (RUL). Commonly, electrochemical impedance spectroscopy (EIS) is used as a nonparametric data-driven…

The rapid spread of Lithium-ions batteries (LiBs) for electric vehicles calls for the development of accurate physical models for Battery Management Systems (BMSs). In this work, the electrochemical Single Particle Model (SPM) for a…

Systems and Control · Electrical Eng. & Systems 2023-11-30 Andrea Trivella , Matteo Corno , Stefano Radrizzani , Sergio M. Savaresi

The Single-Particle Model (SPM) of Li ion cell \cite{Santhanagopalan06, Guo2011} is a computationally efficient and fairly accurate model for simulating Li ion cell cycling behavior at weak to moderate currents. The model depends on a large…

Computational Physics · Physics 2019-12-13 Michael Khasin , Chetan S. Kulkarni , Kai Goebel

Modeling of Li-ion cells is used in battery management systems (BMS) to determine key states such as state-of-charge (SoC), state-of-health (SoH), etc. Accurate models are also useful in developing a cell-level digital-twin that can be used…

Systems and Control · Electrical Eng. & Systems 2024-05-27 Abhijit Kulkarni , Ahsan Nadeem , Roberta Di Fonso , Yusheng Zheng , Remus Teodorescu

Achieving Li-S batteries' promise of significantly higher gravimetric energy density and lower cost than Li-ion batteries requires researchers to delineate the most important factors affecting the performance of this technology. By encoding…

Chemical Physics · Physics 2021-12-17 Michael Cornish , Monica Marinescu

Monitoring battery health is essential for ensuring safe and efficient operation. However, there is an inherent trade-off between assessment speed and diagnostic depth-specifically, between rapid overall health estimation and precise…

Systems and Control · Electrical Eng. & Systems 2026-04-08 Xubo Gu , Xun Huan , Yao Ren , Wenqing Zhou , Weiran Jiang , Ziyou Song

Electrochemical Impedance Spectroscopy (EIS) and Equivalent Circuit Models (ECMs) are widely used to characterize the impedance and estimate parameters of electrochemical systems such as batteries. We use a generic ECM with ten parameters…

Systems and Control · Electrical Eng. & Systems 2024-03-18 Vladimir Sovljanski , Mario Paolone

This paper proposes the linearized physics-based model of a lithium-ion battery that can be incorporated into the optimization framework for power system economic studies. The proposed model is a linear approximation of the single particle…

Systems and Control · Electrical Eng. & Systems 2022-07-08 Anton V. Vykhodtsev , Darren Jang , Qianpu Wang , William Rosehart , Hamidreza Zareipour

This paper develops a comprehensive physics-based model (PBM) that spans a wide operational range, including varying temperatures, charge/discharge conditions, and real-world field data cycles. The PBM incorporates key factors such as…

Systems and Control · Electrical Eng. & Systems 2024-11-20 Guodong Fan , Boru Zhou , Chengwen Meng , Tengwei Pang , Xi Zhang , Mingshu Du , Wei Zhao
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