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The electronic and nuclear dynamics in methanol, following 156~nm photoexcitation, are investigated by combining a detailed analysis of time-resolved photoelectron spectroscopy experiments with electronic structure calculations. The…

An electron beam traversing a structured plasmonic field is shown to undergo diffraction with characteristic angular patterns of both elastic and inelastic outgoing electron components. In particular, a plasmonic {\it grating} (e.g., a…

Mesoscale and Nanoscale Physics · Physics 2016-07-20 F. Javier Garcia de Abajo , Brett Barwick , Fabrizio Carbone

Attosecond photoemission or photoionization delays are a unique probe of the structure and the electronic dynamics of matter. However, spectral congestion and spatial delocalization of valence electron wave functions set fundamental limits…

Laser-induced electron diffraction is an evolving tabletop method, which aims to image ultrafast structural changes in gas-phase polyatomic molecules with sub-{\AA}ngstr\"om spatial and femtosecond temporal resolution. Here, we provide the…

Slow-light enhanced optical detection in liquid-infiltrated photonic crystals is theoretically studied. Using a scattering-matrix approach and the Wigner-Smith delay time concept, we show that optical absorbance benefits both from…

Optics · Physics 2008-02-02 M. E. V. Pedersen , L. S. Rishoj , H. Steffensen , S. Xiao , N. A. Mortensen

For a circularly polarized single-color field at a central frequency of $2\omega$ the final electron momentum distribution upon strong field ionization does not carry any information about the phase of the initial momentum distribution.…

Quantum Physics · Physics 2020-08-17 Sebastian Eckart

A clear consensus on how long it takes a particle to tunnel through a potential barrier has never been so urgently required, since the electron dynamics in strong-field ionization can be resolved on attosecond time-scale in experiment and…

Atomic Physics · Physics 2019-03-19 Xiaolei Hao , Zheng Shu , Weidong Li , Jing Chen

When an atom or molecule absorbs a high-energy photon, an electron is emitted with a well-defined energy and a highly-symmetric angular distribution, ruled by energy quantization and parity conservation. These rules seemingly break down…

Attosecond streaking of photoelectrons emitted by extreme ultraviolet light has begun to reveal how electrons behave during their transport within simple crystalline solids. Many sample types within nanoplasmonics, thin-film physics, and…

Photoionization using attosecond pulses can lead to the formation of coherent superpositions of the electronic states of the parent ion. However, ultrafast electron ejection triggers not only electronic but also nuclear dynamics---leading…

Chemical Physics · Physics 2017-03-29 Caroline Arnold , Oriol Vendrell , Robin Santra

Time delays in photoemission are on the order of attoseconds and have been experimentally determined in atoms, molecules and solids. Their magnitude and energy dependence are expected to yield fundamental insights into the properties of the…

The dissociative ionization of H2+ interacting with intense, femtosecond extreme-ultraviolet laser pulses is investigated theoretically. This is done by numerical propagation of the time-dependent Schr\"{o}dinger equation for a colinear…

Atomic Physics · Physics 2015-02-25 Lun Yue , Lars Bojer Madsen

We present analytical expressions of momentum-resolved core-level photoemission time delay in a molecular frame of a heteronuclear diatomic molecule upon photoionization by a linearly polarized soft x-rays attosecond pulse. For this…

Chemical Physics · Physics 2022-05-31 Y. Tamura , K. Yamazaki , K. Ueda , K. Hatada

Photoelectron holography constitutes a powerful tool for the ultrafast imaging of matter, as it combines high electron currents with subfemtosecond resolution, and gives information about transition amplitudes and phase shifts. Similarly to…

Atomic Physics · Physics 2020-02-19 C. Figueira de Morisson Faria , A. S. Maxwell

Statistical properties of Wigner delay times and the effect of evanescent modes on the deterministic scattering of an electron matter wave from a classically chaotic 2-d electron waveguide are studied for the case of 2, 6, and 16…

Chaotic Dynamics · Physics 2009-10-31 G. B. Akguc , L. E. Reichl

We calculate the transient absorption of an isolated attosecond pulse by helium atoms subject to a delayed infrared (\ir) laser pulse. With the central frequency of the broad attosecond spectrum near the ionization threshold, the absorption…

Atomic Physics · Physics 2015-06-12 Shaohao Chen , Mengxi Wu , Mette B. Gaarde , Kenneth J. Schafer

Wireless signals are integral to modern society, enabling both communication and increasingly, environmental sensing. While various propagation models exist, ranging from empirical methods to full-wave simulations, the phenomenon of…

Signal Processing · Electrical Eng. & Systems 2025-09-10 Anurag Pallaprolu , Winston Hurst , Yasamin Mostofi

Exotic forms of wave control have been emerging by engineering matter in space and time. In this framework, temporal photonic interfaces, i.e., abrupt changes in the electromagnetic properties of a material, have been shown to induce…

We analyze two-center interference effects in the yields of ionization of a dissociating hydrogen molecular ion by an ultrashort VUV laser pulse. To this end, we performed numerical simulations of the time-dependent Schr\"odinger equation…

Quantum Physics · Physics 2015-05-27 A. Picón , A. Bahabad , H. C. Kapteyn , M. M. Murnane , A. Becker

Using a spectrally resolved electron interferometry technique, we measure photoionization time delays between the $3s$ and $3p$ subshells of argon over a large 34-eV energy range covering the Cooper minima in both subshells. The observed…

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