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Coherence among rotational ion channels during photoionization is exploited to control the anisotropy of the resulting photoelectron angular distributions at specific photoelectron energies. The strategy refers to a robust and single…

Chemical Physics · Physics 2019-09-11 R. Chamakhi , M. Telmini , O. Atabek , E. Charron

We present the experimental observation of two-center interference in the ionization time delays of Kr2. Using attosecond electron-ion-coincidence spectroscopy, we simultaneously measure the photoionization delays of krypton monomer and…

The use of semiclassical models based on the Strong Field Approximation (SFA) is ubiquitous in strong field multi-photon ionization and underlies many key developments in attosecond science, including the description of High Harmonic…

The photoelectric effect consists in the photoexcitation of electrons above a potential barrier at a material interface and is exploited for photodetection over a wide frequency range. This three-dimensional process has an inherent…

Using a two-photon interference technique, we measure the delay for single-photon wavepackets to be transmitted through a multilayer dielectric mirror, which functions as a ``photonic bandgap'' medium. By varying the angle of incidence, we…

Quantum Physics · Physics 2016-09-08 Aephraim M. Steinberg , Raymond Y. Chiao

The phenomenon of wave packet diffraction in space and time is described. It consists in a diffraction pattern whose spatial location progresses with time. The pattern is produced by wave packet quantum scattering off an attractive or…

Quantum Physics · Physics 2008-11-26 G. Kälbermann

Using a quantum wave packet simulation including the nuclear and electronic degrees of freedom, we investigate the femtosecond and picosecond energy- and angle-resolved photoelectron spectra of the E($^1\Sigma_g^+$) electronic state of…

Chemical Physics · Physics 2019-04-04 R. Chamakhi , R. Puthumpally-Joseph , M. Telmini , E. Charron

Imaging the quantum motion of electrons not only in real-time, but also in real-space is essential to understand for example bond breaking and formation in molecules, and charge migration in peptides and biological systems. Time-resolved…

Atomic Physics · Physics 2012-07-20 Gopal Dixit , Oriol Vendrell , Robin Santra

Recent advances in the field of attosecond science hold the promise of tracking electronic processes at the shortest space and time scales. Imaging methods that combine attosecond temporal with nanometer spatial resolution are currently out…

Ultraviolet irradiation of ice is of great interest for understanding the chemistry in both atmospheric and astrophysical environments. In interstellar space, photodissociation of H2O molecules can be a driving force behind the chemistry on…

Astrophysics · Physics 2016-08-30 Stefan Andersson , Geert-Jan Kroes , Ewine F. van Dishoeck

Modulating macroscopic parameters of materials in time offers innovative avenues for manipulating electromagnetic waves. Due to such enticing prospects, the general research subject of time-varying systems is expanding today in different…

Optics · Physics 2024-12-06 M. S. Mirmoosa , T. Setälä , A. Norrman

Visualizing the electron dynamics in four dimensions of space and time is crucial to the understanding of several ubiquitous processes in nature. Hence, ultrafast X-ray and electron imaging tools have been developed to probe the dynamics of…

Mesoscale and Nanoscale Physics · Physics 2024-11-26 Mingrui Yuan , Nikolay V. Golubev

A theoretical study of the interference pattern imprinted on the doubly differential momentum distribution of the photoelectron due to atomic ionization induced by a short laser pulse is developed from a semiclassical standpoint. We use the…

Atomic Physics · Physics 2019-09-04 Sebastián D. López , Diego G. Arbó

In the last decade, the development of Ultrafast Electron Diffraction (UED) and Microscopy (UEM) has enabled the imaging of atomic motion in real time and space. These pivotal table-top tools opened the door for a vast range of applications…

Chemical Physics · Physics 2018-01-16 Mohammed Th. Hassan

Accurately determining the crystallographic structure of a material, organic or inorganic, is a critical primary step in material development and analysis. The most common practices involve analysis of diffraction patterns produced in…

We investigate an angular dependence of the photoemission time delay in helium as measured by the RABBITT (Reconstruction of Attosecond Beating By Interference of Two-photon Transitions) technique. The measured time delay $…

Atomic Physics · Physics 2016-05-17 I A Ivanov , J M Dahlström , E Lindroth , A S Kheifets

Elastic scattering of a wave can be quantified by a shift in the phase with respect to the incoming wave phase. A qualitative measure of the time during which the effect occurs is given by the Wigner time delay. The tunneling time in turn…

Quantum Physics · Physics 2024-02-08 Benjamin Schwager , Lars Meschede , Jamal Berakdar

Photoelectron angular momentum distribution of He+ driven by a few-cycle laser is investigated numerically. We simultaneously observe two dominant interference patterns with one shot of lasers by solving the 3D time-dependent Schrodinger…

Atomic and Molecular Clusters · Physics 2016-10-31 Hongchuan Du , Hongmei Wu , Huiqiao Wang , Shengjun Yue , Bitao Hu

Extracting single photoionization time delays associated with atomic (or molecular) species from attosecond time scale two-photon experiments usually relies on the theoretical description of continuum-continuum transitions. The available…

Atomic Physics · Physics 2022-08-29 D. I. R. Boll , L. Martini , O. A. Fojón

We determine and analyze the quantum phases and time delays in photoionization and photorecombination of valence 3p and 3s electrons of argon using the Kohn-Sham local density functional approach. The time-dependent local density…

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