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We propose cotunneling as the microscopic mechanism that makes possible inelastic electron spectroscopy of magnetic atoms in surfaces for a wide range of systems, including single magnetic adatoms, molecules and molecular stacks. We…

Mesoscale and Nanoscale Physics · Physics 2011-08-26 F. Delgado , J. Fernández-Rossier

We study a nonuniversal contribution to the dephasing rate of conduction electrons due to local vibrational modes. The inelastic scattering rate is strongly influenced by multiphonon excitations, exhibiting oscillatory behaviour. For higher…

Strongly Correlated Electrons · Physics 2009-11-13 Balázs Dóra , Miklós Gulácsi

The article presents the result of an extended in silico experiment on computational vibrational spectroscopy of graphene molecules performed using the virtual vibrational spectrometer UHF VVS, previously proposed in the first part of the…

Materials Science · Physics 2020-08-26 Elena F. Sheka , Nadezhda A. Popova

Interactions between electrons and lattice vibrations are responsible for a wide range of material properties and applications. Recently, there has been considerable interest in the development of resonant inelastic x-ray scattering (RIXS)…

We study inelastic electron tunneling through a molecular junction using the non-equilibrium Green function (NEGF) formalism. The effect of the mutual influence between the phonon and the electron subsystems on the electron tunneling…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Michael Galperin , Mark A. Ratner , Abraham Nitzan

Electron spin resonance (ESR) spectroscopy in scanning tunneling microscopy (STM) has enabled probing the electronic structure of single magnetic atoms and molecules on surfaces with unprecedented energy resolution, as well as demonstrating…

Magnetic excitations are important quantum phenomena in magnetic systems and have been widely studied in individual magnetic atoms and molecules as well as their assembled structures over the past few decades. Using scanning tunneling…

In recent measurements of tunneling transport through individual ferromagnetic Co nanograins, Deshmukh, Gu\'eron, Ralph et al. \cite{mandar,gueron} (DGR) observed a tunneling spectrum with discrete resonances, whose spacing was much smaller…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Silvia Kleff , Jan von Delft

Taking spinon excitations in the quantum antiferromagnet CaCu2O3 as an example, we demonstrate that femtosecond dynamics of magnetic excitations can be probed by direct resonant inelastic x-ray scattering (RIXS). To this end, we isolate the…

Propagating atomic vibrational waves, phonons, rule important thermal, mechanical, optoelectronic and transport characteristics of materials. Thus the knowledge of phonon dispersion, namely the dependence of vibrational energy on momentum…

Materials Science · Physics 2019-10-09 Ryosuke Senga , Kazu Suenaga , Paolo Barone , Shigeyuki Morishita , Francesco Mauri , Thomas Pichler

The paper addresses inelastic spin-flip tunneling accompanied by surface spin excitations (magnons) in ferromagnetic junctions. The inelastic tunneling current is proportional to the magnon density of states which is energy-independent for…

Mesoscale and Nanoscale Physics · Physics 2011-08-24 G. Tkachov

Tunneling-induced electronic excitations in a metallic nanograin are classified in terms of {\em generations}: subspaces of excitations containing a specific number of electron-hole pairs. This yields a hierarchy of populated excited states…

Materials Science · Physics 2009-11-10 Gustavo A. Narvaez , George Kirczenow

We present a scattering theory description for the inelastic current noise in the presence of electron-vibration interactions. In this description, we specify elastic and inelastic scattering contributions to the shot noise by examining…

Mesoscale and Nanoscale Physics · Physics 2017-09-15 Sejoong Kim

In the local or itinerant extreme, magnetic excitations can be described by the Heisenberg model which treats electron spins as localized moments, or by the itinerant-electron model where the exchange interaction between electrons leads to…

Surface states of three-dimensional topological insulators exhibit the phenomenon of spin-momentum locking, whereby the orientation of an electron spin is determined by its momentum. Probing the spin texture of these states is of critical…

Mesoscale and Nanoscale Physics · Physics 2018-07-10 Pan He , Steven S. -L. Zhang , Dapeng Zhu , Yang Liu , Yi Wang , Jiawei Yu , Giovanni Vignale , Hyunsoo Yang

Recent developments in experiments with vibrational electron energy loss spectroscopy (EELS) have revealed spectral shape variations at spatial resolutions down to sub-atomic scale. Interpretation in terms of local phonon density of states…

Materials Science · Physics 2021-09-15 Paul M. Zeiger , Ján Rusz

Focused beams of electrons, which act as both sources, and sensors of electric fields, can be used to characterise the electric response of complex photonic systems by locally probing the induced optical near fields. This functionality can…

Electrochemical Impedance Spectroscopy (EIS) is a non-invasive technique widely used for understanding charge transfer and charge transport processes in electrochemical systems and devices. Standard approaches for the interpretation of EIS…

Local moments with a spin $S>1/2$ can exhibit a rich variety of elementary quasiparticle excitations, such as quadrupolar excitations, that go beyond the dipolar magnons of conventional spin-$1/2$ systems. However, the experimental…

Strongly Correlated Electrons · Physics 2025-03-17 Yoshito Watanabe , Simon Trebst , Ciarán Hickey

Inelastic neutron scattering (INS) experiments under applied magnetic field at low temperatures show detailed low lying magnetic excitations in the so called tridiminshed iron icosahedron magnetic molecule. The magnetic molecule consists of…

Strongly Correlated Electrons · Physics 2014-06-05 David Vaknin , Franz Demmel