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A first-principles coupled electron-nuclear dynamics simulation based on real-time, time-dependent density functional theory and Ehrenfest dynamics quantitatively repro-duces bimodal translational energy loss and angular distributions…

Chemical Physics · Physics 2025-12-05 Jialong Shi , Lingjun Zhu , Florian Nitz , Oliver Bünermann , Alec M. Wodtke , Hua Guo , Bin Jiang

In correlated compounds containing cations in high formal oxidation states (assigned by assuming that anions attain full valence shells), the energy of ligand to cation charge transfer can become small or even negative. This yields…

Strongly Correlated Electrons · Physics 2024-09-17 Robert J. Green , George A. Sawatzky

We employ time-resolved optical reflectivity to investigate the ultrafast dynamics of the charge-transfer gap (CTG) in a parent cuprate compound Ca$_2$CuO$_2$Cl$_2$ (CCOC). We observe a persistent photoinduced red shift of the CTG that…

Strongly Correlated Electrons · Physics 2025-05-23 Haiyun Huang , Xiu Zhang , Junzhi Zhu , Jianfa Zhao , Lin Zhao , Yu-Xia Duan , Jian-Qiao Meng , X. J. Zhou , Changqing Jin , Haiyun Liu

Hot electrons injection in carbon nanotubes (CNTs ) where in addition to applied dc field ($\mathbf{E}$), there exist simultaneously a quasi-static ac electric field (i.e. when the frequency $\omega$ of ac field is much less than the…

Mesoscale and Nanoscale Physics · Physics 2016-04-20 M. Amekpewu , S. Y. Mensah , R. Musah , N. G. Mensah , S. S. Abukari , K. A. Dompreh

Here, we report an alternative route to achieve two dimensional electron gas (2DEG) in a semiconductor structure. It has been shown that charge accumulation on the side facets can lead to the formation of 2DEG in a network of c-axis…

Mesoscale and Nanoscale Physics · Physics 2014-10-07 H. P. Bhasker , Varun Thakur , S. M. Shivaprasad , S. Dhar

Charge transfer is a fundamental process that underlies a multitude of phenomena in chemistry and biology. Recent advances in observing and manipulating charge and heat transport at the nanoscale, and recently developed techniques for…

Mesoscale and Nanoscale Physics · Physics 2016-07-26 Galen T. Craven , Abraham Nitzan

The non-equilibrium tunnel transport processes are considered in a square lattice of metallic nanogranules embedded into insulating host. Based on a simple model with three possible charging states (+,-, or 0) of a granule and three kinetic…

Materials Science · Physics 2007-05-23 Yu. G. Pogorelov , J. F. Polido

Nitrogen oxides are textbook class of molecular compounds, with extensive industrial applications. Nitrogen and oxygen are also among the most abundant elements in the universe. We explore the N-O system at 0 K and up to 500 GPa though ab…

Materials Science · Physics 2015-06-30 Dongxu Li , Artem R. Oganov , Xiao Dong , Xiang-Feng Zhou , Qiang Zhu , Guangrui Qian , Huafeng Dong

The discovery of high critical temperature (Tc) superconductivity in pressurized La$_3$Ni$_2$O$_7$ has ignited renewed excitement in the search of novel high-Tc superconducting compounds with 3d transition metals. Compared to other…

In the past few decades, great efforts have been devoted to studying heat transfer on the nanoscale due to its importance in multiple technologies such as thermal control and sensing applications. Heat conduction through the nanoconfined…

Computational Physics · Physics 2022-06-03 Reza Rabani , Samy Merabia , Ahmadreza Pishevar

Applying pressure around megabar is indispensable in the synthesis of high-temperature superconducting hydrides, such as SH$_3$ and LaH$_{10}$. Stabilizing the high-pressure phase of hydride around ambient condition is a severe challenge.…

Superconductivity · Physics 2023-05-17 Miao Gao , Peng-Jie Guo , Huan-Cheng Yang , Xun-Wang Yan , Fengjie Ma , Zhong-Yi Lu , Tao Xiang , Hai-Qing Lin

The charge density wave (CDW) is a condensate that often forms in layered materials. It is known to carry electric current \emph{en masse}, but the transport mechanism remains poorly understood at the microscopic level. Its quantum nature…

Mesoscale and Nanoscale Physics · Physics 2023-10-17 John H. Miller , Martha Y. Suárez-Villagrán , Johnathan O. Sanderson

We construct a fast, transferable, general purpose, machine-learning interatomic potential suitable for large-scale simulations of $N_2$. The potential is trained only on high quality quantum chemical molecule-molecule interactions, no…

Computational Physics · Physics 2024-05-10 Marcin Kirsz , Ciprian G. Pruteanu , Peter I. C. Cooke , Graeme J. Ackland

We find an unusually optimal near field heat transfer, where the maximum heat transfer is reached at experimentally feasible gap separation. We attribute this to the localized zero-energy electronic edge states, which also substantially…

Mesoscale and Nanoscale Physics · Physics 2019-03-28 Gaomin Tang , Han Hoe Yap , Jie Ren , Jian-Sheng Wang

Very recently, a new graphene-like crystalline, hole-free, 2D-single-layer carbon nitride C3N, has been fabricated by polymerization of 2,3-diaminophenazine and used to fabricate a field-effect transistor device with an on-off current ratio…

Computational Physics · Physics 2017-09-27 Yan Gao , Haifeng Wang , Maozhu Sun , Yingchun Ding , Lichun Zhang , Qingfang Li , Jidong Zhang

By means of high-pressure resistivity measurements on single crystals, we investigate the charge transport properties of Cu$_x$PdTe$_2$, notable for the combination of topological type-II Dirac semimetallic properties with superconductivity…

Superconductivity · Physics 2021-06-11 H. Yang , M. K. Hooda , C. S. Yadav , D. Hrabovsky , A. Gauzzi , Y. Klein

Exercising direct control over the unusual electronic structures arising from quantum confinement effects in graphene nanoribbons (GNRs) - atomically defined quasi one-dimensional (1D) strips of graphene - is intimately linked to geometric…

Mesoscale and Nanoscale Physics · Physics 2023-04-18 Sai Ho Pun , Aidan Delgado , Christina Dadich , Adam Cronin , Felix R. Fischer

Cesium adsorption on 2x4 GaAs (001) was studied by photoemission and low energy electron diffraction. The different Cs induced changes of the As 3d and Ga 3d core level spectra show that charge transfer is almost complete for Ga surface…

Materials Science · Physics 2015-05-14 O. E. Tereshchenko , D. Paget , P. Chiaradia , F. Wiame , A. Taleb-Ibrahimie

The prototypical phase change material GeTe shows an enigmatic phase transition at Tc ca. 650 K from rhombohedral (R3m) to cubic (Fm-3m) symmetry. While local probes see little change in bonding, in contrast, average structure probes imply…

Materials Science · Physics 2015-07-01 Jessica M. Hudspeth , Tapan Chatterji , Simon J. L. Billinge , Simon A. J. Kimber

We present first systematic studies of the photoinduced phase transition from the ground charge density wave (CDW) state to the normal metallic (M) state in the prototype quasi-1D CDW system K0.3MoO3. Ultrafast non-thermal CDW melting is…

Strongly Correlated Electrons · Physics 2009-11-13 A. Tomeljak , H. Schäfer , D. Städter , M. Beyer , K. Biljakovic , J. Demsar