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Two-dimensional (2D) intrinsic magnetic materials with high Curie temperature (Tc) coexisting with 100% spin-polarization are highly desirable for realizing promising spintronic devices. In the present work, the intrinsic magnetism of…

Materials Science · Physics 2024-06-12 Fei Li , Yulu Ren , Wenhui Wan , Yong Liu , Yanfeng Ge

Two-dimensional (2D) half-metallic materials are highly desirable for nanoscale spintronic applications. Here, we propose a new mechanism that can achieve half-metallicity in 2D ferromagnetic (FM) material with two-layer magnetic atoms by…

Materials Science · Physics 2023-08-08 Hao-Tian Guo , San-Dong Guo , Yee Sin Ang

Two-dimensional chromium ditelluride (CrTe2) is a promising ferromagnetic layered material that exhibits long-range ferromagnetic ordering in the monolayer limit. The formation energies of the different possible structural phases (1T, 1H,…

Materials Science · Physics 2023-05-02 Yuhang Liu , Sohee Kwon , George J. de Coster , Roger K. Lake , Mahesh R. Neupane

Room temperature two-dimensional (2D) ferromagnetism is highly desired in practical spintronics applications. Recently, 1T phase CrTe2 (1T-CrTe2) nanosheets with five and thicker layers have been successfully synthesized, which all exhibit…

Materials Science · Physics 2021-06-16 Pengfei Gao , Xingxing Li , Jinlong Yang

The structural, electronic and magnetic properties of single layers of Iron Dichloride (FeCl$_{2}$) were calculated using first principles calculations. We found that the 1T phase of the single layer FeCl$_{2}$ is 0.17 eV/unit cell more…

Materials Science · Physics 2015-07-31 E. Torun , H. Sahin , S. K. Singh , F. M. Peeters

Lateral heterostructures of two-dimensional (2D) materials, integrating different phases or materials into a single piece of nanosheet, have attracted intensive research interests in the past few years for high-performance electronic and…

Materials Science · Physics 2020-05-04 Kaiyun Chen , Junkai Deng , Yuan Yan , Qian Shi , Tieyan Chang , Xiangdong Ding , Jun Sun , Sen Yang , Jefferson Zhe Liu

Due to the high magnetic coupling strength between the Cr elements, the bulk phase CrO2 is one of several ferromagnetic oxides known to have the highest Curie temperature. When the dimensionality of the material is reduced from 3D to 2D,…

Materials Science · Physics 2024-03-14 Yang Zhang , Xianggong Bo , Jimeng Jing , Lixia Wang , Shiqian Qiao , Hong Wu , Yong Pu , Feng Li

We investigate magnetic properties of CrTe$_2$ within the density functional theory (DFT) approach in ferromagnetic phase and combination of DFT and dynamical mean field theory (DFT+DMFT) approach in paramagnetic phase. We show that few…

Strongly Correlated Electrons · Physics 2026-03-03 A. A. Katanin , E. M. Agapov

Two-dimensional CrI3 has attracted much attention as it is reported to be a ferromagnetic semiconductor with the Curie temperature around 45K. By performing first-principles calculations, we find that the magnetic ground state of CrI3 is…

Computational Physics · Physics 2019-01-09 Zewen Wu , Jin Yu , Shengjun Yuan

Monolithic realization of metallic 1T and semiconducting 2H polymorphic phases makes MoS2 a potential candidate for future microelectronic circuits. Though co-existence of these phases has been reported, a method for engineering a stable 1T…

Mesoscale and Nanoscale Physics · Physics 2018-08-22 Chithra H. Sharma , Ananthu P. Surendran , Abin Varghese , Madhu Thalakulam*

Recently, two-dimensional ferromagnetic semiconductors have been an important class of materials for many potential applications in spintronic devices. Based on density functional theory, we systematically explore the magnetic and…

Materials Science · Physics 2020-01-14 Yulu Ren , Yanfeng Ge , Wenhui Wan , Qiaoqiao Li , Yong Liu

Ferromagnetism in the two-dimensional materials is of great significance and has become an emerging topic. The ferromagnetic VS$_2$ and VSe$_2$ monolayers have been experimentally synthesized, and O element belongs to the same group as S…

Materials Science · Physics 2025-03-14 Lihui Han , Lujia Tian , Bing-Xin Liu , Zong-liang Li , Miao Gao , Fengjie Ma , Xun-Wang Yan

We study magnetic properties of CrO$_2$ within the density functional theory plus dynamical mean-field theory (DFT+DMFT) approach in the paramagnetic phase. We consider the 3-orbital (per Cr site) model, containing only $t_{2g}$ states, the…

Strongly Correlated Electrons · Physics 2024-10-15 A. A. Katanin

Interfaces and low dimensionality are sources of strong modifications of electronic, structural, and magnetic properties of materials. FeRh alloys are an excellent example because of the first-order phase transition taking place at…

The dynamical and thermodynamic phase stabilities of the stoichiometric compound CrN including different structural and magnetic configurations are comprehensively investigated using a first-principles density-functional-theory (DFT) plus U…

The electronic and magnetic properties of pristine CrPSe$_3$ and mixed Cr$_{1\textrm{-}x}$M$_x$PSe$_3$ (M = Zn, Cd, Hg) monolayers were studied using density functional theory including an on-site Coulomb term (DFT$+U$) and tight-binding…

Materials Science · Physics 2021-12-23 Juntao Yang , Yong Zhou , Yuriy Dedkov , Elena Voloshina

Two-dimensional (2D) 1T-VSe$_2$ has prompted significant interest due to the discrepancies regarding alleged ferromagnetism (FM) at room temperature, charge density wave (CDW) states and the interplay between the two. We employed a combined…

An accurate density-functional method is used to study systematically half-metallic ferromagnetism and stability of zincblende phases of 3d-transition-metal chalcogenides. The zincblende CrTe, CrSe, and VTe phases are found to be excellent…

Materials Science · Physics 2009-11-10 Wen-Hui Xie , Ya-Qiong Xu , Bang-Gui Liu , D G Pettifor

We apply the density-functional theory to study various phases (including non-magnetic (NM), anti-ferromagnetic (AFM), and ferromagnetic (FM)) in monolayer magnetic chromium triiodide (CrI$_3$), a recently fabricated 2D magnetic material.…

Mesoscale and Nanoscale Physics · Physics 2018-10-17 Lucas Webster , Liangbo Liang , Jia-An Yan

Using Density Functional Theory (DFT) calculations and Monte-Carlo (MC) simulations, we investigate the recently reported magnetic transition in B2 Al-Cr-Co alloys. The Cr sublattice is alloyed with different amounts of Co in the…

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