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We propose to evaluate the contribution of polycyclic aromatic hydrocarbon molecules that carry side groups to the mid-infrared emission spectra. Within this framework, the IR absorption spectra of 2- and 9-vinylanthracene were measured in…

Solar and Stellar Astrophysics · Physics 2015-06-05 Anju Maurya , Shantanu Rastogi , G. Rouillé , Friedrich Huisken , Thomas Henning

Super-Resolution Ultrasound (SRUS) through localizing spatially isolated microbubbles has been demonstrated to overcome the wave diffraction limit and reveal the microvascular structure and flow information at the microscopic scale.…

Signal Processing · Electrical Eng. & Systems 2022-06-09 B. Wang , K. Riemer , M. Toulemonde , J. Yan , X. Zhou , M. Tang

We combine different wavelengths from an intense high-order harmonics source with variable delay at the focus of a split-mirror interferometer to conduct pump-probe experiments on gas-phase molecules. We report measurements of the time…

Chemical Physics · Physics 2015-05-27 T. K. Allison , T. W. Wright , A. M. Stooke , C. Khurmi , J. van Tilborg , Y. Liu , R. W. Falcone , A. Belkacem

Quantum cascade laser (QCL) frequency combs have revolutionized mid-infrared (MIR) spectroscopy by their high brightness and fast temporal resolution, and are a promising technology for fully-integrated and cost-effective sensors. As for…

Hyperspectral microscopy is an imaging technique that provides spectroscopic information with high spatial resolution. When applied in the relevant wavelength region, such as in the infrared (IR), it can reveal a rich spectral fingerprint…

Optical phase-spaces represent fields of any spatial coherence, and are typically measured through phase-retrieval methods involving a computational inversion, interference, or a resolution-limiting lenslet array. Recently, a weak-values…

Optics · Physics 2018-09-12 Samuel H. Knarr , Daniel J. Lum , James Schneeloch , John C. Howell

Dual Comb Spectroscopy proved its versatile capabilities in molecular fingerprinting in different spectral regions, but not yet in the ultraviolet (UV). Unlocking this spectral window would expand fingerprinting to the electronic energy…

Increasing the sweep rate of mid-infrared (MIR) frequency-swept sources offers significant potential for various high-speed spectroscopy-based applications. While continuous-wave frequency-swept lasers have achieved sweep rates up to 1 MHz,…

Two frequency combs can be used to measure the full complex response of a sample in a configuration which can be alternatively viewed as the equivalent of a dispersive Fourier transform spectrometer, infrared time domain spectrometer, or a…

Optics · Physics 2015-05-18 I. Coddington , W. C. Swann , N. R. Newbury

We present a study of water vapour in the Venus troposphere obtained by modelling specific water vapour absorption bands within the 1.18 \mu m window. We compare the results with the normal technique of obtaining the abundance by matching…

Earth and Planetary Astrophysics · Physics 2012-12-06 S. Chamberlain , J. A. Bailey , D. Crisp , V. S. Meadows

We describe a new method which achieves high precision Very Long Baseline Interferometry (VLBI) astrometry in observations at millimeter wavelengths. It combines fast frequency-switching observations, to correct for the dominant…

Instrumentation and Methods for Astrophysics · Physics 2015-05-27 Maria J. Rioja , Richard Dodson

Many areas of optical science require an accurate measurement of optical spectra. Devices based on laser speckle promise compact wavelength measurement, with attometer-level sensitivity demonstrated for single wavelength laser fields. The…

High-resolution gas phase spectroscopy techniques in the microwave, millimeter-wave and terahertz spectral ranges can be used to study complex organic molecules desorbed from interstellar ice analogues surface with a high sensitivity.…

Instrumentation and Methods for Astrophysics · Physics 2019-12-23 Patrice Theulé , Christian Endres , Marius Hermanns , Jean-Baptiste Bossa , Alexey Potapov

Dual-comb spectroscopy has been proven a powerful tool in molecular characterization, which remains challenging to implement in the mid-infrared region due to difficulties in the realization of two mutually locked comb sources and efficient…

High-performance integrated optical phased arrays (OPAs) are crucial for building up energy-efficient solid-state beam steering systems on a chip. This work demonstrates a first heterogeneous III-V/Si phase-shifter based OPA that utilizes…

Applied Physics · Physics 2019-04-03 Weiqiang Xie , Tin Komljenovic , Jinxi Huang , Michael L. Davenport , John E. Bowers

Photo-acoustic spectroscopy (PAS) is one of the most sensitive non-destructive analysis techniques for gases, fluids and solids. It can operate background-free at any wavelength and is applicable to microscopic and even non-transparent…

Precise astronomical spectroscopic analyses routinely assume that individual pixels in charge-coupled devices (CCDs) have uniform sensitivity to photons. Intra-pixel sensitivity (IPS) variations may already cause small systematic errors in,…

Instrumentation and Methods for Astrophysics · Physics 2015-06-04 Michael T. Murphy , Clayton R. Locke , Philip S. Light , Andre N. Luiten , Jon S. Lawrence

Single-photon avalanche diode (SPAD) arrays have transformed optical imaging by enabling photon-counting sensitivity, picosecond resolution, and high frame-rate operation. These capabilities, however, have remained confined to the visible…

Measuring microcombs in amplitude and phase provides unique insight into the nonlinear cavity dynamics but spectral phase measurements are experimentally challenging. Here, we report a linear heterodyne technique assisted by electro-optic…

Cavity-enhanced direct frequency comb spectroscopy combines broad spectral bandwidth, high spectral resolution, precise frequency calibration, and ultrahigh detection sensitivity, all in one experimental platform based on an optical…

Optics · Physics 2009-11-13 Michael J. Thorpe , Jun Ye