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Moving the detection wavelength in vibrational sum-frequency generation (VSFG) spectroscopy to the near-infrared (> 700 nm) can potentially enable the study of molecular interfaces absorbing in the visible and give access to buried…

Optics · Physics 2024-05-10 Zsuzsanna Heiner , Valentin Petrov , Mark Mero

Phased array feeds (PAFs) for reflector antennas offer the potential for increased reflector field of view and faster survey speeds. To address some of the development challenges that remain for scientifically useful PAFs, including…

Instrumentation and Methods for Astrophysics · Physics 2015-05-14 Jonathan Landon , Michael Elmer , Jacob Waldron , David Jones , Alan Stemmons , Brian D. Jeffs , Karl F. Warnick , J. Richard Fisher , Roger D. Norrod

We present broadband dual frequency comb laser absorption measurements of 2% H$_2$O (natural isotopic abundance of 99.7% H$_2^{16}$O) in air from 6600-7650 cm$^{-1}$ (1307-1515 nm) with a spectral point spacing of 0.0068 cm$^{-1}$.…

Atmospheric and Oceanic Physics · Physics 2024-02-29 Scott C. Egbert , Keeyoon Sung , Sean C. Coburn , Brian J. Drouin , Gregory B. Rieker

The increasing availability of high-power Yb-based ultrafast laser-amplifier systems has opened the possibility of air filamentation at high repetition rates >1 kHz. In this new regime, accumulation effects cannot be ruled out, therefore,…

Dual-frequency comb spectroscopy permits broadband precision spectroscopic measurements with short acquisition time. A dramatic improvement of the maximal spectral bandwidth and the minimal measurement time can be expected when the lasers'…

We report here an experimental setup to perform three-pulse pump-probe measurements over a wide wavelength and temperature range. By combining two pump pulses in the visible (650-900 nm) and mid-IR (5-20 $\mu$m) range, with a broadband…

We report the development of a new instrument for cavity-enhanced absorption spectroscopy of the fundamental rovibrational transitions of molecules in the long-wave mid-infrared (LWIR) region from 6500 to 10000 nm. Our setup combines a LWIR…

One of the essential goals of molecular spectroscopy is to measure all fundamental molecular vibrations simultaneously. To this end, one needs to measure broadband infrared (IR) absorption and Raman scattering spectra, which provide…

The development of optical fibers has revolutionized telecommunications by enabling long-distance broad-band transmission with minimal loss. In turn, the ubiquity of high-quality low-cost fibers enabled a number of additional applications,…

Optics · Physics 2017-03-30 Brandon Redding , Mansoor Alam , Martin Seifert , Hui Cao

The NRAO Very Long Baseline Array (VLBA) was used at 1.4 GHz to image 20 compact sources in the inner 1-degree radius of the Spitzer VLA First-Look Survey. Twelve sources were detected with the VLBA, with peak flux densities above 2 mJy at…

Astrophysics · Physics 2009-11-10 J. M. Wrobel , M. A. Garrett , J. J. Condon , R. Morganti

We present an absolute distance measurement interferometer based on a two wavelength interferometer and a variable synthetic wavelength technique. The wavelength scanning range was 12 GHz, realized with a phase accuracy of 1.0 m{\lambda} by…

Instrumentation and Detectors · Physics 2014-02-25 Yoshiyuki Kuramoto , Hiroshi Okuda

We present a reliable, narrow linewidth (100 kHz) continuous-wave optical parametric oscillator (OPO) suitable for high-resolution spectroscopy applications. The OPO is based on a periodically-poled lithium-niobate crystal and features a…

We have combined high resolution VLBI Space Observatory Programme (VSOP) data at 1.6 and 4.8 GHz with Very Long Baseline Array (VLBA) data at higher frequencies and with similar resolutions to study the spectral properties of the core of…

Astrophysics · Physics 2015-06-24 Richard Dodson , Philip G. Edwards , Hisashi Hirabayashi

We demonstrate a 13-fold speed improvement in broadband cantilever-enhanced photoacoustic spectroscopy (CEPAS) by combining it with phase-controlled Fourier-transform spectroscopy (PC-FTS) instead of traditional Fourier-transform infrared…

Optics · Physics 2022-12-21 Santeri Larnimaa , Mikhail Roiz , Markku Vainio

There is an increasing demand for precise molecular spectroscopy, in particular in the mid-infrared fingerprint window that hosts a considerable number of vibrational signatures, whether it be for modeling our atmosphere, interpreting…

Molecular diagnostics are a primary tool of modern chemistry, enabling researchers to map chemical reaction pathways and rates to better design and control chemical systems. Many chemical reactions are complex and fast, and existing…

Mid-infrared spectroscopy probes molecular vibrations to identify chemical species and functional groups. Therefore, mid-infrared hyperspectral imaging is one of the most powerful and promising candidates for chemical imaging using optical…

Optics · Physics 2023-07-06 Yue Zhao , Shota Kusama , Yuji Furutani , Wei-Hong Huang , Chih-Wei Luo , Takao Fuji

We describe a possible new technique for precise wavelength calibration of high-resolution astronomical spectrographs using femtosecond-pulsed mode-locked lasers controlled by stable oscillators such as atomic clocks. Such `frequency combs'…

Nuclear Magnetic Resonance (NMR) spectroscopy is an important bio-engineering tool to determine the metabolic concentrations, molecule structures and so on. The data acquisition time, however, is very long in multi-dimensional NMR. To…

We demonstrate dual-comb spectroscopy based on difference frequency generation of frequency-agile near-infrared frequency combs, produced with the help of electro-optic modulators. The combs have a remarkably flat intensity distribution and…