Related papers: Coherent Nonlinear Optical Response for High-Inten…
In this work we provide an exact and efficient numerical approach to simulate multi-time correlation functions in the Mahan-Nozi\`{e}res-De Dominicis model, which crudely mimics the spectral properties of doped two-dimensional…
Over the past years, there have been many efforts towards generating interactions between two optical beams so strong that they could be observed at the level of individual photons. Such strong interactions, beyond opening up a new regime…
Feedback is a powerful and ubiquitous technique both in classical and quantum system control. Its standard implementation relies on measuring the state of a system, processing the classical signal, and feeding it back to the system. In…
Quantifying and controlling the coherent dynamics and couplings of optically active excitations in solids is of paramount importance in fundamental research in condensed matter optics and for their prospective optoelectronic applications in…
Nonlinear modal interactions in resonant systems govern a wide range of phenomena, with broad relevance across modern physics and engineering. Yet, experimentally determining the strength of nonlinear coupling in multimode resonators…
The nonlinear response of materials, an increasingly important aspect of light-matter interaction, can be challenging to measure in highly absorbing materials. Here, we introduce an interferometric technique that enables a direct…
Exposing a molecule to intense light pulses may bring this molecule to a nonstationary quantum state, thus launching correlated dynamics of electronic and nuclear subsystems. Although much had been achieved in the understanding of…
We introduce a numerically exact and computationally feasible nonlinear-response theory developed for lossy superconducting quantum circuits based on a framework of quantum dissipation in a minimally extended state space. Starting from the…
Manifesting across all time, mass and length scales, nonlinearities lie at the core of numerous physical phenomena. Next-generation quantum applications, such as quantum sensing, require the combination of nonlinearity with non-classical…
Electronic energy transfer in photosynthesis occurs over a range of time scales and under a variety of intermolecular coupling conditions. Recent work has shown that electronic coupling between chromophores can lead to coherent oscillations…
We adapted a recently proposed framework to characterize the optical response of interacting electrons in solids in order to expedite its computation without compromise in accuracy at the microscopic level. Our formulation is based on…
We employ two-dimensional (2D) coherent, nonlinear spectroscopy to investigate couplings within individual InAs quantum dots (QD) and QD molecules. Swapping pulse ordering in a two-beam sequence permits to distinguish between rephasing and…
A nonlinear interferometry scheme is described theoretically to induce and resolve electron wave- function beating on time scales shorter than the optical cycle of the time-delayed pump and probe pulses. By employing two moderately intense…
The photophysics of $\pi$-conjugated polymers has been of considerable interest over the last three decades because of their organic semiconductor properties. Primary photoexcitations, Frenkel excitons, can be probed optically by means of…
We demonstrate theoretically and experimentally that the nonlinear interaction between excitations whose harmonic energies coincide gives rise to a strong coupling that opens a new coherent ultrafast energy relaxation path. Instead of an…
We present a new type of phase- and frequency-sensitive amplification and attenuation in a cyclically driven three-level superconducting Josephson system. Different from the previous linear theory of pure phase-sensitive amplification, a…
Precision spectroscopy of atomic systems is an invaluable tool for the advancement of our understanding of fundamental interactions and symmetries. Recently, highly charged ions (HCI) have been proposed for sensitive tests of physics beyond…
We study the nonlinear spectra and multi-photon correlation functions for the waveguide output of a two-level system (including realistic dissipation channels) with a time-delayed coherent feedback. We compute these observables by extending…
Optical excitation and control of excitonic wavepackets in organic molecules is the basis to energy conversion processes. To gain insights into such processes, it is essential to establish the relationship between the coherence timescales…
We have implemented a new approach for measuring the time-dependent intensity and phase of ultrashort optical pulses. It is based on the interaction between shaped pulses and atoms, leading to coherent transients.