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In this technical review we give an introduction to optical spectroscopy for layered materials as a powerful, non-invasive tool to access details of the electronic band structure and crystal quality. Potential applications in photonics and…

Materials Science · Physics 2020-12-18 Shivangi Shree , Ioannis Paradisanos , Xavier Marie , Cedric Robert , Bernhard Urbaszek

Proposals to determine biomolecular structures from diffraction experiments using femtosecond X-ray free-electron laser (XFEL) pulses involve a conflict between the incident brightness required to achieve diffraction-limited atomic…

Optics · Physics 2015-05-19 Harry M. Quiney , Keith A. Nugent

We study the elastic scattering of atomic argon by a electron in the presence of a bichromatic laser field. The numerical calculation is done in the first Born approximation (FBA) for a simple screening electric potential. With the help of…

Atomic and Molecular Clusters · Physics 2008-10-09 Bin Zhou , Shu-Min Li

In a recent publication, Dalen, and Selst{\o}, Phys. Rev. A {\bf 111}, 033116 (2025), it was demonstrated how converged photo electron spectra could be determined using a complex absorbing potential on a truncated numerical domain…

Quantum Physics · Physics 2025-10-14 Selstø Sølve , Bendik Steinsvåg Dalen

The high beam current and sub-angstrom resolution of aberration-corrected scanning transmission electron microscopes has enabled electron energy loss spectroscopic (EELS) mapping with atomic resolution. These spectral maps are often…

Materials Science · Physics 2023-07-19 Paul Cueva , Robert Hovden , Julia A. Mundy , Huolin L. Xin , David A. Muller

Plasmonics, the science and technology of the interaction of light with metallic objects, is fundamentally changing the way we can detect, generate and manipulate light. Although the field is progressing swiftly, thanks to the availability…

We study a nonlinear Schr\"odinger equation which arises as an effective single particle model in X-ray Free Electron Lasers (XFEL). This equation appears as a first-principles model for the beam-matter interactions that would take place in…

Numerical Analysis · Mathematics 2014-06-18 Paolo Antonelli , Agissilaos Athanassoulis , Zhongyi Huang , Peter A. Markowich

The holographic mask technique is used to create freely moving electrons with quantized angular momentum. With electron optical elements they can be focused to vortices with diameters below the nanometer range. The understanding of these…

Materials Science · Physics 2013-04-09 P. Schattschneider , M. Stöger-Pollach , S. Löffler , A. Steiger-Thirsfeld , J. Hell , J. Verbeeck

It is shown in the case of proton scattering on an electron gas target that the Closed Time Path formalism can handle final state interactions of the target in equilibrium in a simple and natural manner. The leading order cross section is…

High Energy Physics - Phenomenology · Physics 2013-06-18 F. Mansouri , J. Polonyi , K. Zazoua , N. Zekri

Spatially resolved electron energy-loss spectroscopy (EELS) in a scanning transmission electron microscope (STEM) has been used to investigate as fluidic phase in nanoubbles embedded in a metallic Pd90Pt10 matrix. Using the 1s->2p…

Materials Science · Physics 2016-08-14 D. Taverna , M. Kociak , O. Stéphan , A. Fabre , E. Finot , B. Décamps , C. Colliex

We theoretically demonstrate the ability of electron beams to probe the nonlinear photonic response with nanometer spatial resolution, well beyond the capabilities of existing optical techniques. Although the interaction of electron beams…

Mesoscale and Nanoscale Physics · Physics 2020-12-30 Andrea Konečná , Valerio Di Giulio , Vahagn Mkhitaryan , Claus Ropers , F. Javier García de Abajo

The electronic properties of two-dimensional (2D) materials depend sensitively on the underlying atomic arrangement down to the monolayer level. Here we present a novel strategy for the determination of the band gap and complex dielectric…

Compact radio sources have been observed to undergo large, frequency dependent changes in intensity due to lensing by structures in the interstellar medium, in so-called "extreme scattering events" (ESEs). While the study of astrophysical…

High Energy Astrophysical Phenomena · Physics 2022-06-22 Dylan L. Jow , Ue-Li Pen

Electron energy loss spectroscopy (EELS) has been established as a powerful analytical technique for investigating the oxidation state, band structure, and dielectric properties of materials with exceptional spatial resolution. Inspired by…

The first experimental data from single-particle scattering experiments from free electron lasers (FELs) are now becoming available. The first such experiments are being performed on relatively large objects such as viruses, which produce…

Biomolecules · Quantitative Biology 2015-05-28 Dilano Saldin , Hin-Cheuck Poon , Peter Schwander , Miraj Uddin , Marius Schmidt

In this work we present a theoretical study of EELS (electron-energy-loss spectroscopy) experiments on the ${\rm C}_{60}$ molecule. Our treatment of the problem is based on the simple two-fluid model originally proposed for the description…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 D. A. Gorokhov , R. A. Suris , V. V. Cheianov

The highly energetic electrons in a transmission electron microscope (TEM) can alter or even completely destroy the structure of samples before sufficient information can be obtained. This is especially problematic in the case of zeolites,…

Materials Science · Physics 2021-05-05 Abner Velazco , Daen Jannis , Armand Béché , Johan Verbeeck

The recent theoretical and experimental activities in positronium (Ps) scattering by atoms and molecules are reviewed with special emphasis at low energies. We critically compare the results of different groups $-$ theoretical and…

Chemical Physics · Physics 2009-11-07 Sadhan K. Adhikari

Single-cycle optical pulses with a controlled electromagnetic waveform allow to steer the motion of low-energy electrons in atoms, molecules, nanostructures or condensed-matter on attosecond dimensions in time. However, high-energy…

Optics · Physics 2020-11-11 Yuya Morimoto , Peter Baum

X-ray near-field speckle-based phase-sensing approaches provide efficient means to characterise optical elements. Here, we present a theoretical review of several of these speckle methods in the frame of optical characterisation and provide…