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We proposed a mechanism to generate giant anisotropic second harmonic nonlinear response via double resonance effect, achieved through band nesting via electronic bandstructure engineering. The ideal band setup would be a triplet of nested…

The spatial-temporal beam quality of laser sources is crucial for applications such as nonlinear spectroscopy and master oscillator power amplification systems. However, the temporal stability remains challenged by issues like line-width…

Optics · Physics 2026-01-21 Siyu Chen , Jun Ye , Lei Du , Wenwen Cheng , Jiangming Xu , Rongtao Su , Pu Zhou , Zongfu Jiang

We theoretically investigate photo-excitation of electron-hole pairs and high harmonic generation in the bulk of zinc oxide (ZnO) subjected to intense femto-second laser pulses with mid-infrared wavelength. The main microscopic mechanism of…

Optics · Physics 2025-07-15 Boyan Obreshkov , Tzveta Apostolova

Second harmonic generation in nonlinear materials can be greatly enhanced by realizing doubly-resonant cavities with high quality factors. However, fulfilling such doubly resonant condition in photonic crystal (PhC) cavities is a…

Intense, single-cycle terahertz (THz) pulses offer a promising approach for understanding and controlling the properties of a material on an ultrafast time scale. In particular, resonantly exciting phonons leads to a better understanding of…

Strongly Correlated Electrons · Physics 2016-10-05 P. Bowlan , J. Bowlan , S. A. Trugman , R. Valdes Aguilar , J. Qi , X. Liu , J. Furdyna , M. Dobrowolska , A. J. Taylor , D. A. Yarotski , R. P. Prasankumar

We observe strongly anisotropic third-harmonic generation mediated by resonant sum-frequency driving of Raman phonons with THz light, extending light-induced dual control of structural and optical properties in solids. Either strong…

Optics · Physics 2024-05-03 Jiaoyang Zheng , Guru Khalsa , Jeffrey Moses

We conduct a theoretical and numerical study on the second-harmonic (SH) optical response of a nano-structured metamaterial composed of a periodic array of inclusions. Both the inclusions and their surrounding matrix are made of…

Mesoscale and Nanoscale Physics · Physics 2019-03-13 Ulises R. Meza , Bernardo S. Mendoza , W. Luis Mochán

Comparative analysis of second harmonic generation in ordinary and backward-wave settings is presented. Extraordinary properties of frequency doubling nonlinear optical reflectivity and pulse shaping through phase matching of ordinary and…

Optics · Physics 2016-02-02 Alexander K. Popov , Sergey A. Myslivets

We experimentally investigate second harmonic generation from strongly coupled localized and propagative phonon polariton modes in arrays of silicon carbide nanopillars. Our results clearly demonstrate the hybrid nature of the system's…

We investigate second-order nonlinear processes in a system of two coupled identical optical micro-resonators. The double resonance and phase-matching conditions are simultaneously obtained thanks to the frequency splitting induced by the…

Optics · Physics 2025-10-03 Yannick Dumeige , Yoan Léger

Nonlinear interactions of spin-waves and their quanta, magnons, have emerged as prominent candidates for interference-based technology, ranging from quantum transduction to antiferromagnetic spintronics. Yet magnon multiplication in the…

Strongly Correlated Electrons · Physics 2024-04-09 C. Huang , L. Luo , M. Mootz , J. Shang , P. Man , L. Su , I. E. Perakis , Y. X. Yao , A. Wu , J. Wang

We experimentally observe the generation of magnon harmonics and subharmonics in an on-chip surface acoustic wave resonator incorporating a thin Co$_{20}$Fe$_{60}$B$_{20}$ film, using micro-focused Brillouin light scattering. In our…

We use ultrafast laser pulses to experimentally demonstrate that the second-order optical response of bulk single crystals of the topological insulator Bi$_2$Se$_3$ is sensitive to its surface electrons. By performing surface doping…

Materials Science · Physics 2011-02-02 D. Hsieh , J. W. McIver , D. H. Torchinsky , D. R. Gardner , Y. S. Lee , N. Gedik

Plasmonic dimer antennas create strong field enhancement by squeezing light into a nanoscale gap. These optical hotspots are highly attractive for boosting nonlinear processes, such as harmonic generation, photoelectron emission, and…

Frequency conversion processes, such as second- and third-harmonic generation, are one of the most common effects in nonlinear optics which offer many opportunities for photonics, chemistry, material science, characterization, and…

Optics · Physics 2017-06-26 Alexander Krasnok , Mykhailo Tymchenko , Andrea Alu

Third-harmonic generation (THG) is a key nonlinear optical process for ultrafast imaging, terahertz (THz) signal generation, and symmetry-sensitive probes, often dominating in centrosymmetric materials where lower-order responses vanish.…

Optics · Physics 2026-01-09 Sanjay Sarkar , Debottam Mandal , Amit Agarwal

We report terahertz (THz) second harmonic generation (SHG) in superconductors (SC) with inversion symmetric equilibrium states that forbid even-order nonlinearities. Such SHG signal is observed in single-pulse emission by periodic driving…

Because of the importance of second harmonic generation in some nonlinear media, in this paper, we investigated induced second harmonic generation in diamond where there is no intrinsic second order susceptibility, X(2). The electric field…

Optics · Physics 2015-11-19 Mahboubeh Ghalandari

Second-harmonic generation (SHG) is a fundamental nonlinear optical process widely used in photonics; however, it is strictly forbidden in the bulk of centrosymmetric materials due to their inversion symmetry. Nevertheless, applying an…

Directional harmonic generation is an important property characterizing the ability of nonlinear optical antennas to diffuse the signal in well-defined region of space. Herein, we show how sub-wavelength facets of an organic molecular…

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