Related papers: Nonlinear Terahertz Resonances from Ballistic Elec…
Efficient frequency conversion techniques are crucial to the development of plasmonic metasurfaces for information processing and signal modulation. In principle, nanoscale electric-field confinement in nonlinear materials enables higher…
Dielectric metasurfaces provide a unique platform for efficient harmonic generation and optical wavefront manipulation at the nanoscale. While several approaches are available for performing wavefront shaping, the one exploiting geometric…
The generation of harmonics by atoms interacting with two circularly polarized and frequency related laser fields is addressed through ab initio numerical simulations. A detailed charaterization of a few specific harmonics is given. In…
We demonstrate that the THz generation in air from a dual-color pulse, composed of the fundamental and second-harmonic waves, can be coherently controlled by field-free molecular alignment. By tuning its time delay to properly match various…
We demonstrate efficient second-harmonic generation at moderate input power for thin film Ni81Fe19 undergoing ferromagnetic resonance (FMR). Powers of the generated second-harmonic are shown to be quadratic in input power, with an…
Nonlinear frequency conversion in optics can originate the coherent light at the wavelength where it is hard or unlikely to achieve by directly lasing and is a fundamental topic in science and engineering covering both classical and quantum…
We present a method to measure quadratic Terahertz optical nonlinearities in Terahertz time-domain spectroscopy. We use a rotating linear polarizer (a polarizing chopper) to modulate the amplitude of the incident THz pulse train. We use a…
We introduce a versatile numerical method for modeling light diffraction in periodically patterned photonic structures containing quadratically nonlinear non-centrosymmetric optical materials. Our approach extends the generalized source…
We show that the lack of inversion symmetry in monolayer MoS2 allows strong optical second harmonic generation. Second harmonic of an 810-nm pulse is generated in a mechanically exfoliated monolayer, with a nonlinear susceptibility on the…
Second harmonic generation has been applied to study lattice, electronic and magnetic proprieties in atomically thin materials. However, inversion symmetry breaking is usually required for the materials to generate a large signal. In this…
The terahertz spectral regime, ranging from about 0.1 to 15 THz, is one of the least explored yet most technologically transformative spectral regions. One current challenge is to develop efficient and compact terahertz emitters/detectors…
High harmonic generation (HHG) opens a window on the fundamental science of strong-field light-mater interaction and serves as a key building block for attosecond optics and metrology. Resonantly enhanced HHG from hot spots in…
Nonlinear metamaterials show potential for realizing flat nonlinear optical devices but generally lack in terms of achievable conversion efficiencies. Recent work has focused on enhancing nonlinear processes by utilizing high quality factor…
The anisotropic dispersion and inherent nonlinearity of magnetostatic spin waves in thin films and confined structures provide unique opportunities for implementation in next-generation magnonic devices for data and signal processing. A…
Metallic nanostructures exhibit strong nonlinear-optical response at surface plasmon resonances, where the light-matter coupling efficiency is enhanced. An active modulation of this response can be realized by means of an external magnetic…
We derive the $\mathcal{T}$-matrix formalism tailored for numerical analysis of second-harmonic (SH) generation from arbitrarily shaped particles made of centrosymmetric optical materials. First, the transfer matrix of a single particle is…
The nonlinear response of sub wavelength nano-cavities in thin metal films is investigated. We report the resonant dependence of the Second Harmonic Generation by individual triangular and square holes on shape, size and wavelength. For…
Since de discovery of graphene, the family of 2-dimensional materials has attracted much recent attention. In this work, the nonlinear optical properties of few-layer MoS2 two-dimensional crystals are studied using femtosecond laser pulses.…
Resonant enhancement of high harmonic generation can be obtained in plasmas containing ions with strong radiative transitions resonant with harmonic orders. The mechanism for this enhancement is still debated. We perform the first temporal…
In this article, we analytically study second harmonic (SH) generation from thin metallic films with subwavelength, non-centrosymmetry patterns. Because the thickness of the film is much smaller than the SH wavelength, retardation effects…