Related papers: Terahertz-Induced Nonlinear Response in ZnTe
The nonlinear interaction between Near-Infrared (NIR) and Terahertz pulses is principally investigated as a means for the detection of radiation in the hardly accessible THz spectral region. Most studies have targeted second-order nonlinear…
We use an open-aperture Z-scan technique to show how intense few-cycle terahertz pulses can experience a nonlinear bleaching of absorption in an n-doped semiconductor due to terahertz-electric-field-driven intervalley scattering of…
We present a method to measure quadratic Terahertz optical nonlinearities in Terahertz time-domain spectroscopy. We use a rotating linear polarizer (a polarizing chopper) to modulate the amplitude of the incident THz pulse train. We use a…
Intense few cycle terahertz pulses exhibit complex non-linear behavior under interaction with heavily n-doped Si. Fast increase in the transmission of a 700 fs pulse (central frequency 1.5 THz) through the Si sample (low field transmission…
Nonlinear terahertz (THz) spectroscopy relies on the interaction of matter with few-cycle THz pulses of electric field amplitudes up to megavolts/centimeter (MV/cm). In condensed-phase molecular systems, both resonant interactions with…
We explore the dynamics of a system where input spectra in the optical domain with very disparate center frequencies are strongly coupled via highly phase-matched, cascaded second-order nonlinear processes driven by terahertz radiation. The…
Collinear phase-matched optical rectification is studied in ZnGeP$_{2}$ pumped with near-infrared light. The pump-intensity dependence is presented for three crystal lengths (0.3, 1.0 and 3.0 mm) to determine the effects of linear optical…
Transmission through photoexcited semiconductors is used to temporally and spectrally shape a Terahertz pulse. By adjusting the optical pump-THz probe delay, we experimentally introduce a polar asymmetry in the pulse profile as high as 92%.…
Strong optical pulses at mid-infrared and terahertz frequencies have recently emerged as a powerful tool to manipulate and control the solid state and especially complex condensed matter systems with strongly correlated electrons. The…
Controlling light polarization is one of the most essential routines in modern optical technology. Since the demonstration of optical pulse shaping by spatial light modulators and its potential in controlling the quantum reaction pathways,…
Interactions of few-cycle terahertz pulses with the induced optical polarization in a quantum-well microcavity reveal that the lower and higher exciton-polariton modes together with the optically forbidden 2p-exciton state form a unique…
The induced terahertz response of semiconductor systems is investigated with a microscopic theory. In agreement with recent terahertz experiments, the developed theory fully explains the ultrafast build up of the plasmon resonance and the…
Recently developed terahertz (THz) two-dimensional coherent spectroscopy (2DCS) is a powerful technique to obtain materials information in a fashion qualitatively different from other spectroscopies. Here, we utilized THz 2DCS to…
Nonlinear responses to intense terahertz (THz) fields provide unique insights into complex dynamics of contemporary material systems. However, the interpretation of the obtained data, in particular, distinguishing genuine ionic oscillations…
We report the first coherent excitation of intramolecular vibrational modes via the nonlinear interaction of a TeraHertz (THz) light field with molecular liquids. A terahertz-terahertz-Raman pulse sequence prepares the coherences with a…
We report on the first experimental observation of a very strong nonlinear response in crystalline quartz in the terahertz (THz) frequency region through THz time-domain spectroscopy (THz-TDS). Theoretical modelling is presented and…
Femtosecond laser pulses interacting with LiNbO3 has been widely applied in intense terahertz generation, excitation and imaging of phonon polaritons and modulating light. It is of great importance to study the nonlinearities induced by…
The effect of terahertz (THz) pulse generation has revolutionized broadband coherent spectroscopy and imaging at THz frequencies. However, THz pulses typically lack spatial structure, whereas structured beams are becoming essential for…
We have systematically investigated the spatial and temporal dynamics of crystallization that occurs in the phase-change material Ge2Sb2Te5 upon irradiation with an intense THz pulse. THz pump and optical probe spectroscopy revealed that…
Coherent radiation with frequencies ranging from 0.3 to 30 THz has recently become accessible by femtosecond laser technology. Terahertz (THz) waves have already found many applications in spectroscopy and imaging, and they can be…