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We have observed short-lived optical birefringence in a CH$_3$NH$_3$PbBr$_3$ single crystal induced by a powerful nearly single-cycle terahertz pulse. Apart from the instantaneous contribution that follows the profile of the squared pump…

Materials Science · Physics 2022-05-10 A. A. Melnikov , V. E. Anikeeva , O. I. Semenova , S. V. Chekalin

We have observed optical birefringence in liquids induced by single-cycle THz pulses with field strengths exceeding 100 kV/cm. The induced change in polarization is proportional to the square of the THz electric field. The time-dependent…

Other Condensed Matter · Physics 2015-05-13 Matthias C. Hoffmann , Nathaniel C. Brandt , Harold Y. Hwang , Ka-Lo Yeh , Keith A. Nelson

We propose and experimentally prove efficient high-resolution electro-optic sampling measurement of broadband terahertz waveforms in a LiNbO$_3$ crystal in the configuration with the probe laser beam propagating along the optical axis of…

Polarization control of terahertz wave is a challenging subject in terahertz science and technology. Here, we report a simple method to control polarization state of the terahertz wave in terahertz generation process. At room temperature,…

Materials Science · Physics 2015-10-28 R. Takeda , N. Kida , M. Sotome , H. Okamoto

The spin-splitting energy bands induced by the relativistic spin-orbit interaction in solids provide a new opportunity to manipulate the spin-polarized electrons on the sub-picosecond time scale. Here, we report one such example in a bulk…

Strongly Correlated Electrons · Physics 2018-04-11 Yuto Kinoshita , Noriaki Kida , Tatsuya Miyamoto , Manabu Kanou , Takao Sasagawa , Hiroshi Okamoto

We report multicycle, narrowband, terahertz radiation at 14.8 THz produced by phase-matched optical rectification of femtosecond laser pulses in bulk lithium niobate (LiNbO$_3$) crystals. Our experiment and simulation show that the output…

Optics · Physics 2020-07-15 Dogeun Jang , Ki-Yong Kim

We report on the emission of terahertz radiation by irradiation of femtosecond laser pulses in non-centrosymmetric paraelectric and ferroelectric phases of Co$_3$B$_7$O$_{13}$I boracite. The Generation of the terahertz waves in both phases…

Materials Science · Physics 2015-06-22 Y. Kinoshita , N. Kida , M. Sotome , R. Takeda , N. Abe , M. Saito , T. Arima , H. Okamoto

Measuring terahertz waveforms in terahertz spectroscopy often relies on electrooptic sampling employing a ZnTe crystal. Although the nonlinearities in such zincblende semiconductors induced by intense terahertz pulses have been studied at…

We detected broadband coherent terahertz (THz) emission from multiferroic BiFeO3 after illuminating a high-quality bulk single ferroelectric domain crystal with a ~100 fs optical pulse. The dependence of the emitted THz waveform on the…

Materials Science · Physics 2009-11-13 D. Talbayev , Seongsu Lee , S. -W. Cheong , A. J. Taylor

Crystal field (CF) excitations in the ground multiplet $^3H_6$ of Tm$^{3+}$ ions were investigated using terahertz transmission spectra of magnetoelectric TmAl$_3$(BO$_3$)$_4$ and Tm$_{0.05}$Yb$_{0.1}$Y$_{0.85}$Al$_3$(BO$_3$)$_4$. These…

We have studied the ultrafast optical response of a PbSe crystal to an intense picosecond terahertz pulse with a peak electric field strength of up to $\sim$ 500 kV/cm. The reflectivity anisotropy signal contains oscillations at the…

Materials Science · Physics 2024-12-10 A. A. Melnikov , Yu. G. Selivanov , D. G. Poydashev , S. V. Chekalin

We report the Terahertz optical properties of the Vanadium doped [100] \b{eta}-Ga2O3 using Terahertz Time-Domain Spectroscopy (THz-TDS). The V-doped \b{eta}-Ga2O3 crystal shows strong birefringence in the 0.2-2.4 THz range. Further, phase…

A previous work, ref. 2 experimentally confirmed that measured special polarization characteristic features of a three-dimensional terahertz (THz) photonic-crystal did not apparently apply to general physical- and optical- basic rules. It…

Optics · Physics 2019-03-20 Chikara Sakurai

Intense few cycle terahertz pulses exhibit complex non-linear behavior under interaction with heavily n-doped Si. Fast increase in the transmission of a 700 fs pulse (central frequency 1.5 THz) through the Si sample (low field transmission…

Ultrafast electron microscopy provides a movie-like access to structural dynamics of materials in space and time, but fundamental atomic motions or electron dynamics are, so far, too quick to be resolved. Here we report the all-optical…

Optics · Physics 2024-02-27 J. Kuttruff , D. Nabben , A. C. Zimmermann , A. Ryabov , P. Baum

The dynamical processes associated with electric field manipulation of the polarization in a ferroelectric remain largely unknown but fundamentally determine the speed and functionality of ferroelectric materials and devices. Here we apply…

The angular dependence of terahertz (THz) emission from birefringent crystals can differ significantly from that of cubic crystals. Here we consider optical rectification in uniaxial birefringent materials, such as chalcopyrite crystals.…

A previous work [1] experimentally confirmed that the special polarization characteristic features of a three-dimensional terahertz (THz) photonic crystal with a silicon inverse diamond structure whose lattice point shape was vacant regular…

Optics · Physics 2019-05-20 Chikara Sakurai

This work presents the results for the Faraday rotation in pure and Cr-doped lead germanate crystals studied in the course of proper ferroelectric phase transition. We show that the increment of the Faraday rotation appearing at the phase…

Materials Science · Physics 2007-06-19 D. Adamenko , I. Klymiv , V. M. Duda , R. Vlokh , O. Vlokh

Terahertz (THz) radiation has been observed from multiferroic BiFeO$_3$ thin films via ultrafast modulation of spontaneous polarization upon carrier excitation with illumination of femtosecond laser pulses. The radiated THz pulses from…

Strongly Correlated Electrons · Physics 2016-08-31 Kouhei Takahashi , Noriaki Kida , Masayoshi Tonouchi
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