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The radioisotope Th-229 is renowned for its extraordinarily low-energy, long-lived nuclear first-excited state. This isomeric state can be excited by VUV lasers and the transition from the ground state has been proposed as a reference…

Solid-state $^{229}$Th nuclear clocks are set to provide new opportunities for precision metrology and fundamental physics. Taking advantage of a nuclear transition's inherent low sensitivity to its environment, orders of magnitude more…

While the $^{229}$Th nuclear isomer has recently been observed and laser-excited, converting optical nuclear manipulation into a chip-scale solid-state frequency standard remains an open challenge. Here, we present a nanophotonic platform…

The recent demonstration of laser excitation of the $\approx 8$ eV isomeric state of Thorium-229 is a significant step towards a nuclear clock. The low excitation energy likely results from a cancellation between electromagnetic and strong…

High Energy Physics - Phenomenology · Physics 2025-09-16 Andrea Caputo , Doron Gazit , Hans-Werner Hammer , Joachim Kopp , Gil Paz , Gilad Perez , Konstantin Springmann

When Th nuclei are doped in CaF$_2$ crystals, a set of electronic defect states appears in the crystal bandgap which would otherwise provide complete transparency to vacuum-ultraviolet radiation. The coupling of these defect states to the 8…

Optical atomic clocks$^{1,2}$ use electronic energy levels to precisely keep track of time. A clock based on nuclear energy levels promises a next-generation platform for precision metrology and fundamental physics studies. Thorium-229…

Calcium monofluoride (CaF) molecules are loaded into an optical dipole trap (ODT) and subsequently laser cooled within the trap. Starting with magneto-optical trapping, we sub-Doppler cool CaF and then load $150(30)$ CaF molecules into an…

Thorium ions exhibit unique nuclear properties with high relevance for testing symmetries of nature, and Paul traps feature an ideal experimental platform for performing high precision quantum logic spectroscopy. Loading of stable or…

Solid-state $^{229}$Th nuclear clocks require a host material whose band gap is larger than the 8.4 eV nuclear transition energy. As such, excitation of the $^{229}$Th nuclear state has so far only been demonstrated in metal fluorides,…

We report the sympathetic cooling and Coulomb crystallization of molecular ions above the surface of an ion-trap chip. N$_2^+$ and CaH$^+$ ions were confined in a surface-electrode radiofrequency ion trap and cooled by the interaction with…

Atomic Physics · Physics 2014-08-13 A. Mokhberi , S. Willitsch

With an expected energy of 7.6(5) eV, $^{229}$Th possesses the lowest excited nuclear state in the landscape of all presently known nuclei. The energy corresponds to a wavelength of about 160 nm and would conceptually allow for an optical…

Instrumentation and Detectors · Physics 2017-04-27 Benedict Seiferle , Lars von der Wense , Mustapha Laatiaoui , Peter G. Thirolf

Deep laser cooling of atoms, ions, and molecules facilitates the study of fundamental physics as well as applied research. In this work, we report on the narrow-line laser cooling of thulium atoms at the wavelength of $506.2\,\textrm{nm}$…

We report non-destructive imaging of optically trapped calcium monofluoride (CaF) molecules using in-situ $\Lambda$-enhanced gray molasses cooling. $200$ times more fluorescence is obtained compared to destructive on-resonance imaging, and…

Sympathetic cooling of Th$^{3+}$ ions is demonstrated in an experiment where $^{229}$Th and $^{230}$Th are extracted from uranium recoil ion sources and are confined in a linear Paul trap together with laser-cooled $^{88}$Sr$^+$ ions.…

Atomic Physics · Physics 2024-03-26 G. Zitzer , J. Tiedau , M. V. Okhapkin , K. Zhang , C. Mokry , J. Runke , Ch. E. Düllmann , E. Peik

Harnessing the potential wide-ranging quantum science applications of molecules will require control of their interactions. Here, we use microwave radiation to directly engineer and tune the interaction potentials between ultracold calcium…

The 7.6-eV-isomer of Thorium-229 offers the opportunity to perform high resolution laser spectroscopy of a nuclear transition. We give a brief review of the investigations of this isomer. The nuclear resonance connecting ground state and…

Optics · Physics 2017-08-23 E. Peik , K. Zimmermann , M. Okhapkin , Chr. Tamm

Thorium-doped LiCaAlF$_6$ and LiSrAlF$_6$ (Th:LiCAF and Th:LiSAF) are promising crystals for a solid-state nuclear clock based on the 8 eV transition in $^{229}$Th; however, their complex crystal structures complicate understanding the…

Materials Science · Physics 2026-01-13 Martin Pimon , Tobias Kirschbaum , Thorsten Schumm , Adriana Pálffy , Andreas Grüneis

The nucleus of 229Thorium presents a unique isomer state of very low energy and long lifetime, current estimates are around 7.8 eV and seconds to hours respectively. This nuclear transitions therefore is a promising candidate for a novel…

Atomic Physics · Physics 2013-04-18 G. A. Kazakov , M. Schreitl , G. Winkler , J. H. Sterba , G. Steinhauser , T. Schumm

We demonstrate the ability to load, cool and detect singly-charged calcium ions in a surface electrode trap using only visible and infrared lasers for the trapped-ion control. As opposed to the standard methods of cooling using…

Atomic Physics · Physics 2017-07-27 F. Lindenfelser , M. Marinelli , V. Negnevitsky , S. Ragg , J. P. Home

We investigate the dynamics of an ion sympathetically cooled by another laser-cooled ion or small ion crystal. To this end, we develop simple models of the cooling dynamics in the limit of weak Coulomb interactions. Experimentally, we…

Quantum Physics · Physics 2015-10-02 M. Guggemos , D. Heinrich , O. A. Herrera-Sancho , R. Blatt , C. F. Roos