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We introduce a versatile numerical method for modeling light diffraction in periodically patterned photonic structures containing quadratically nonlinear non-centrosymmetric optical materials. Our approach extends the generalized source…

Optics · Physics 2015-06-23 Martin Weismann , Dominic F. G. Gallagher , Nicolae C. Panoiu

Tunable biphoton quantum entanglement generated from nonlinear processes is highly desirable for cutting-edge quantum technologies, yet its tunability is substantially constrained by the symmetry of material nonlinear tensors. Here, we…

A comparative experimental investigation of the dependence of second harmonic generation (SHG) on applied external voltage between the standard nematic liquid crystalline material and an analogue ferromagnetic nematic liquid crystalline…

Soft Condensed Matter · Physics 2019-09-30 Jure Brence , Luka Cmok , Nerea Sebastian , Alenka Mertelj , Darja Lisjak , Irena Drevensek-Olenik

Graphene is a unique platform for tunable opto-electronic applications thanks to its linear band dispersion, which allows electrical control of resonant light-matter interactions. Tuning the nonlinear optical response of graphene is…

Optical nonlinearity depends on symmetry and symmetries vanish in the presence of defects. Vaccancy defects in centrosymmetric crystals and thin films are a well-known source of even-order optical nonlinearity, e.g. causing second harmonic…

Optics · Physics 2022-03-02 Jie Xu , Eric Plum

Recent experiments and calculations in topological semimetals have observed anomalously strong second-order optical nonlinearity, but yet whether the enhancement also occurs at surfaces of topological semimetals in general remains an open…

We propose a computational framework to extract non-linear response functions from real-time simulations in the presence of more than one external field. We apply this approach to the calculation of sum frequency generation (SFG) and…

Materials Science · Physics 2025-11-19 Mike N. Pionteck , Myrta Grüning , Simone Sanna , Claudio Attaccalite

Nonlinear optical generation from a crystalline material can reveal the symmetries of both its lattice structure and underlying ordered electronic phases and can therefore be exploited as a complementary technique to diffraction based…

Strongly Correlated Electrons · Physics 2014-11-04 D. H. Torchinsky , H. Chu , T. Qi , G. Cao , D. Hsieh

Nonlinear phenomena are inherent in most systems in nature. Second or higher-order harmonic generations, three-wave and four-wave mixing are typical phenomena in nonlinear optics. To obtain a nonzero signal for second-harmonic generation in…

Mesoscale and Nanoscale Physics · Physics 2019-04-29 Zhou Li , Franco Nori

Using symmetry arguments we show how optical second harmonic generation (SHG) can be used to detect antiferromagnetism at surfaces and in thin films. Based on the group theoretical analysis of the nonlinear electric susceptibility we…

Condensed Matter · Physics 2007-05-23 A. Daehn , W. Huebner , K. H. Bennemann

Silicon photonics lacks a second-order nonlinear optical response in general because the typical constituent materials are centro-symmetric and lack inversion symmetry, which prohibits second-order nonlinear processes such as second…

Optics · Physics 2022-07-21 Xiyuan Lu , Gregory Moille , Ashutosh Rao , Daron Westly , Kartik Srinivasan

Second-harmonic generation (SHG) is a second-order nonlinear optical process that is not allowed in media with inversion sym-metry. However, due to the broken symmetry at the surface, surface SHG still occurs, but is generally small. We…

Second-order optical nonlinear effects (second-harmonic and sum-frequency generation) are demonstrated in the telecommunication band by periodic poling of thin films of lithium niobate wafer-bonded on silicon substrates and rib-loaded with…

The nonlinear magneto-plasmonics aims to utilize plasmonic excitations to control the mechanisms and taylor the efficiencies of the non-linear light frequency conversion at the nanoscale. We investigate the mechanisms of magnetic second…

We develop a multipolar theory of second-harmonic generation (SHG) by dielectric nanoparticles made of noncentrosymmetric materials with bulk quadratic nonlinearity. We specifically analyze two regimes of optical excitation: illumination by…

Nonlinear spectroscopy with quantum entangled photons is an emerging field of research that holds the promise to achieve a superior signal-to-noise ratio and effectively isolate many-body interactions. Photon sources used for this purpose…

Nonlinear light-matter interactions in structured materials are the source of exciting properties and enable vanguard applications in photonics. However, the magnitude of nonlinear effects is generally small, thus requiring high optical…

Materials Science · Physics 2022-03-22 Fadil Iyikanat , Andrea Konečná , F. Javier García de Abajo

Nonlinear optics, and particularly second harmonic generation (SHG), is increasingly used in many modern disciplines from material characterization in physical sciences to bio-imaging in medicine and optical signal processing in information…

Strongly Correlated Electrons · Physics 2021-03-17 G. van der Laan , S. W. Lovesey

High harmonic generation (HHG) is an extremely nonlinear effect, where a medium is driven by a strong laser field, generating coherent broadband radiation with photon energies ranging up to the X-ray and pulse durations reaching attosecond…

Optics · Physics 2020-10-20 Alexey Gorlach , Ofer Neufeld , Nicholas Rivera , Oren Cohen , Ido Kaminer

Recent years have witnessed significant developments in the study of nonlinear properties of various optical materials at the nanoscale. However, in most cases experimental results on harmonic generation from nanostructured materials are…