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We introduce a novel class of localized atomic environment representations, based upon the Coulomb matrix. By combining these functions with the Gaussian approximation potential approach, we present LC-GAP, a new system for generating…

Machine Learning · Statistics 2016-12-07 James Barker , Johannes Bulin , Jan Hamaekers , Sonja Mathias

In this paper I propose a new model for representing the formation energies of multicomponent crystalline alloys as a function of atom types. In the cases when displacements of atoms from their equilibrium positions are not large, the…

Computational Physics · Physics 2017-08-02 Alexander Shapeev

Identifying the chemical structure from a graphical representation, or image, of a molecule is a challenging pattern recognition task that would greatly benefit drug development. Yet, existing methods for chemical structure recognition do…

Computer Vision and Pattern Recognition · Computer Science 2024-04-03 Martijn Oldenhof , Edward De Brouwer , Adam Arany , Yves Moreau

Machine-learning of atomic-scale properties amounts to extracting correlations between structure, composition and the quantity that one wants to predict. Representing the input structure in a way that best reflects such correlations makes…

Chemical Physics · Physics 2021-02-02 Michael J. Willatt , Félix Musil , Michele Ceriotti

The high-throughput screening of periodic inorganic solids using machine learning methods requires atomic positions to encode structural and compositional details into appropriate material descriptors. These atomic positions are not…

Materials Science · Physics 2018-12-26 Ankit Jain , Thomas Bligaard

Machine-learning models are increasingly used to predict properties of atoms in chemical systems. There have been major advances in developing descriptors and regression frameworks for this task, typically starting from (relatively) small…

Chemical Physics · Physics 2022-11-30 John L. A. Gardner , Zoé Faure Beaulieu , Volker L. Deringer

We elaborate on a general method that we recently introduced for characterizing the "natural" structures in complex physical systems via a multiscale network based approach for the data mining of such structures. The approach is based on…

Materials Science · Physics 2015-03-18 P. Ronhovde , S. Chakrabarty , D. Hu , M. Sahu , K. F. Kelton , N. A. Mauro , K . K. Sahu , Z. Nussinov

Conditioning image generation on specific features of the desired output is a key ingredient of modern generative models. However, existing approaches lack a general and unified way of representing structural and semantic conditioning at…

Computer Vision and Pattern Recognition · Computer Science 2024-07-08 Luca Butera , Andrea Cini , Alberto Ferrante , Cesare Alippi

We present an algorithm for generating all derivative superstructures--for arbitrary parent structures and for any number of atom types. This algorithm enumerates superlattices and atomic configurations in a geometry-independent way. The…

Materials Science · Physics 2014-12-18 Gus L. W. Hart , Rodney W. Forcade

The constant demand for new functional materials calls for efficient strategies to accelerate the materials design and discovery. In addressing this challenge, machine learning generative models can offer promising opportunities since they…

Materials Science · Physics 2020-06-24 Sungwon Kim , Juhwan Noh , Geun Ho Gu , Alán Aspuru-Guzik , Yousung Jung

Sequential weak measurements allow the direct extraction of individual density-matrix elements instead of globally reconstructing the whole density matrix, opening a new avenue for the characterization of quantum systems. Nevertheless, the…

As in many other fields, the rapid rise of generative artificial intelligence is reshaping materials discovery by offering new ways to propose crystal structures and, in some cases, even predict desired properties. This review provides a…

We develop a representation theory of categories as a means to explore characteristic structures in algebra. Characteristic structures play a critical role in isomorphism testing of groups and algebras, and their construction and…

Group Theory · Mathematics 2025-11-20 Peter A. Brooksbank , Heiko Dietrich , Joshua Maglione , E. A. O'Brien , James B. Wilson

The development of high-resolution imaging methods such as electron and scanning probe microscopy and atomic probe tomography have provided a wealth of information on structure and functionalities of solids. The availability of this data in…

Materials Science · Physics 2022-11-08 Sergei V. Kalinin , Ayana Ghosh , Rama Vasudevan , Maxim Ziatdinov

The most successful and popular machine learning models of atomic-scale properties derive their transferability from a locality ansatz. The properties of a large molecule or a bulk material are written as a sum over contributions that…

Chemical Physics · Physics 2020-01-08 Andrea Grisafi , Michele Ceriotti

Neural network potentials are a powerful tool for atomistic simulations, allowing to accurately reproduce \textit{ab initio} potential energy surfaces with computational performance approaching classical force fields. A central component of…

Disordered Systems and Neural Networks · Physics 2023-12-27 Johannes Sandberg , Thomas Voigtmann , Emilie Devijver , Noel Jakse

We utilize connections between molecular coarse-graining approaches and implicit generative models in machine learning to describe a new framework for systematic molecular coarse-graining (CG). Focus is placed on the formalism encompassing…

Chemical Physics · Physics 2020-09-11 Aleksander E. P. Durumeric , Gregory A. Voth

The nearest prototype classification is a less computationally intensive replacement for the $k$-NN method, especially when large datasets are considered. In metric spaces, centroids are often used as prototypes to represent whole clusters.…

Machine Learning · Computer Science 2021-07-06 Jaroslav Hlaváč , Martin Kopp , Jan Kohout

Foundational machine learning interatomic potentials that can accurately and efficiently model a vast range of materials are critical for accelerating atomistic discovery. We introduce universal potentials based on the graph atomic cluster…

Materials Science · Physics 2026-01-06 Yury Lysogorskiy , Anton Bochkarev , Ralf Drautz

A novel Genetic Algorithm is described that is suitable for determining the global minimum energy configurations of crystal structures and which can also be used as a polymorph search technique. This algorithm requires no prior assumptions…

Other Condensed Matter · Physics 2007-05-23 N. L. Abraham , M. I. J. Probert