Related papers: Quantum Electrodynamics Coupled-Cluster Theory: Ex…
Under appropriate conditions, superconducting electronic circuits behave quantum mechanically, with properties that can be designed and controlled at will. We have realized an experiment in which a superconducting two-level system, playing…
We investigate the power-dependent photoluminescence spectra from a strongly coupled quantum dot-cavity system using a quantum master equation technique that accounts for incoherent pumping, pure dephasing, and fermion or boson statistics.…
Quantum mechanical effects at the macroscopic level were first explored in Josephson junction-based superconducting circuits in the 1980's. In the last twenty years, the emergence of quantum information science has intensified research…
We introduce a model of quantum magnetism induced by the non-perturbative exchange of microwave photons between distant superconducting qubits. By interconnecting qubits and cavities, we obtain a spin-boson lattice model that exhibits a…
We introduce a new equation-of-motion coupled-cluster method based on a pair coupled-cluster doubles (pCCD) reference, termed frozen-pair EOM-CCSD (EOM-fpCCSD). This approach combines the computational efficiency of the pCCD ansatz with a…
Constant-potential molecular dynamics (MD) simulations are indispensable for understanding the capacitance, structure, and dynamics of electrical double layers (EDLs) at the atomistic level. However, the classical constant-potential method,…
Cavity quantum electrodynamics (cavity QED) enables the control of light-matter interactions at the single-photon level, rendering it a key component of many quantum technologies. Its practical realization, however, is complex since it…
We present a quantum theory for a fully coupled hybrid optomechanical system where all mutual couplings between a two-level atom, a confined photon mode and a mechanical oscillator mode are considered. In such a configuration, new quantum…
In cavity quantum electrodynamics (QED), light-matter interaction is probed at its most fundamental level, where individual atoms are coupled to single photons stored in three-dimensional cavities. This unique possibility to experimentally…
A new perturbative approach to canonical equation-of-motion coupled-cluster theory is presented using coupled-cluster perturbation theory. A second-order M{\o}ller-Plesset partitioning of the Hamiltonian is used to obtain the well known…
We study universal quantum computation in the cavity quantum electrodynamics (CQED) framework exploiting two orthonormal two-photon generalized binomial states as qubit and dispersive interactions of Rydberg atoms with high-$Q$ cavities. We…
We develop coupled-cluster theory for systems of electrons strongly coupled to photons, providing a promising theoretical tool in polaritonic chemistry with a perspective of application to all types of fermion-boson coupled systems. We show…
We present an exact ansatz for the eigenstate problem of mixed fermion-boson systems that can be implemented on quantum devices. Based on a generalization of the electronic contracted Schr\"odinger equation (CSE), our approach guides a…
High-dimensional quantum information processing has emerged as a promising avenue to transcend hardware limitations and advance the frontiers of quantum technologies. Harnessing the untapped potential of the so-called qudits necessitates…
Condensed matter physics and quantum electrodynamics (QED) have been long considered as distinct disciplines. This situation is changing by the progress in cavity QED materials. Motivated by these advances we aim to bridge these fields by…
The squeezed photons, as a quantum-correlated light with reduced noise, have emerged as a great resource for sensing the structures of matter. Here we study the transient absorption (TA) scheme using the squeezed photons whose spectral…
Macroscopic quantum electrodynamics (MQED) provides a unified framework to describe quantum electromagnetic fields in the presence of arbitrary macroscopic environments. Central to this theory is the field correlation, which governs both…
We study light-mediated interactions between spatially separated molecules using real-time quantum electrodynamical time-dependent density functional theory based on the Pauli-Fierz Hamiltonian. An ultrashort delta-kick excitation…
We propose a scheme of increasing quantum correlations for the cavity quantum electrodynamics system consisting of two noninteracting two-level atoms each locally interacting with its own quantized field mode by bang-bang pulses. We…
We systematically study the interaction between two quantized optical fields and a cyclic atomic ensemble driven by a classic optical field. This so-called atomic cyclic ensemble consists of three-level atoms with Delta-type transitions due…