Related papers: Multidimensional Terahertz Probes of Quantum Mater…
Terahertz two-dimensional coherent spectroscopy (THz-2DCS) is transforming our ability to probe, visualize, and control quantum materials far from equilibrium. This emerging technique brings multi-dimensional resolution to the ultrafast…
Two distinct measurement schemes have emerged for the new technique of two-dimensional terahertz spectroscopy (2DTS), complicating the literature. Here, we argue that the 'conventional' measurement scheme derived from nuclear magnetic…
Recently, two-dimensional terahertz spectroscopy (2DTS) has attracted increasing attention for studying complex solids. A number of recent studies have applied 2DTS either with long pulses or away from any material resonances, situations…
Ultra-fast and multi-dimensional spectroscopy gives a powerful looking glass into the dynamics of molecular systems. In particular two-dimensional electronic spectroscopy (2DES) provides a probe of coherence and the flow of energy within…
Quantum sensing is highly attractive for accessing spectral regions in which the detection of photons is technically challenging: sample information is gained in the spectral region of interest and transferred via entanglement into another…
Nonlinear terahertz (THz) spectroscopy relies on the interaction of matter with few-cycle THz pulses of electric field amplitudes up to megavolts/centimeter (MV/cm). In condensed-phase molecular systems, both resonant interactions with…
Terahertz spectroscopy allows for identifying different isomers of materials, for drug discrimination as well as for detecting hazardous substances. As many dielectric materials used for packaging are transparent in the terahertz spectral…
Light-matter interactions are key in providing fundamental information about materials. Even in the linear-response regime, the spectroscopic response of a material encodes in it many properties of the ground state as well as of its…
Two-level systems (TLS) of unclear physical origin are a major contributor to decoherence in superconducting qubits. The interactions of individual TLS with a qubit can be detected via various spectroscopic methods, most of which have…
Recently developed terahertz (THz) two-dimensional coherent spectroscopy (2DCS) is a powerful technique to obtain materials information in a fashion qualitatively different from other spectroscopies. Here, we utilized THz 2DCS to…
Double-quantum two-dimensional coherent spectroscopy (MDCS) is a powerful optical method that is used to study optical properties of atomic and complex molecular systems and semiconductor materials. Double-quantum 2D spectra and…
Non-destructive testing is an important technique for detecting defects in multi-layer materials, enabling the evaluation of structural integrity without causing damage on test materials. Terahertz time-domain spectroscopy (THz-TDS) offers…
Two-dimensional terahertz spectroscopy (2DTS) is a low-frequency analogue of two-dimensional optical spectroscopy that is rapidly maturing as a probe of a wide variety of condensed matter systems. However, a persistent problem of 2DTS is…
Ultrafast two-dimensional spectroscopy utilizes correlated multiple light-matter interactions for retrieving dynamic features that may otherwise be hidden under the linear spectrum. Its extension to the terahertz regime of the…
Quantum imaging with undetected photons spatially transfers amplitude and phase information from one spectral region of physical interest to another spectral region that is easy to detect. The photon energy of the two spectral regions can,…
Recent studies have shown that the nonlinear optical response of crystalline systems is fundamentally a quantum geometric property. In this work, we propose two-dimensional coherent spectroscopy (2DCS), which measures the nonlinear…
Interactions between particles in quantum many-body systems play a crucial role in determining the electric, magnetic, optical, and thermal properties of the system. The recent progress in the laser-pulse technique has enabled the…
Two-dimensional coherent spectroscopy (2DCS) is an established method for characterizing molecules and has been proposed in the THz regime as a new tool for probing exotic excitations of quantum magnets; however, the precise nature of the…
Terahertz time-domain spectroscopy (THz-TDS) provides a powerful platform for investigating low-energy excitations in quantum materials. Because these materials are often limited in size, experimental setups typically rely on tightly…
Defects in solid-state materials play a central role in determining coherence, stability, and performance in quantum technologies. Although narrowband techniques can probe specific resonances with high precision, a broadband spectroscopic…